Hybrid-Protected Perovskite Quantum Dot Films with Ultra-High Efficiency and Stability for LED Backlighting DOI Creative Commons
Loan Thi Ngo, Wen‐Tse Huang, Hemant Verma

et al.

ACS Applied Materials & Interfaces, Journal Year: 2024, Volume and Issue: unknown

Published: Nov. 19, 2024

All-inorganic lead halide perovskite quantum dots (PQDs) have emerged as highly promising materials for photonic and optoelectronic devices, solar cells, photocatalysts. However, PQDs encounter instability color separation issues because of ion diffusion. Current strategies mainly address stability in green CsPbBr3 PQDs, with limited focus on the red-mixed their inferior compared PQDs. Our study provides a new dual-protection methodology synthesizing high-efficiency red mixed-halide PQD films. Red CsPb(Br0.4I0.6)3 are embedded silicone resin then incorporated poly(methyl methacrylate) (PMMA) matrix to form PQDs@silicone/PMMA The high photoluminescence yield (PLQY) great recorded pure-red polymer film. ultrabright film was also successfully fabricated an outstanding PLQY beyond 94%. These films exhibited enhanced against thermal environmental degradation, attributed dense protective layer PMMA matrices by formation Si–halide Pb–O bonds, thereby reducing surface defects. Theoretical calculations reveal that combining improves interactions, eliminating uncoordinated Pb2+ enhancing stability. Applied white light-emitting diodes (WLEDs), these demonstrated broad gamut 143.4%, indicating potential efficient WLED backlighting.

Language: Английский

Metal Halide Perovskite as Down‐Conversion Materials for Advanced Display DOI
Xiang Zhang, Nian Liu,

Hainan Du

et al.

Advanced Materials, Journal Year: 2025, Volume and Issue: unknown

Published: May 9, 2025

Abstract Metal halide perovskites have gained worldwide attention as excellent optoelectronic materials. Over the past decade, perovskite‐based color conversion technology has shown significant promise for commercialization, particularly in display applications. Prototypes of displays utilizing this made remarkable achievements. As slightly more than a decade elapsed since discovery metal perovskite light‐emitting diodes, comprehensive review, and outlook is crucial to advance explore its full potential next‐generation displays. To end, paper systematically outlined strategies enhancing material performance patterning fabrication techniques converters. Building on current technological advancements, review also summarizes new chances emerging morphologies. Furthermore, key challenges hindering commercialization converters are pointed out guide future research development. This aims offer valuable insights into advanced

Language: Английский

Citations

0

Efficient Large-Area Quantum Cutting Photoconversion Films for Silicon Solar Cells on Photovoltaic Glass Using Knife Coating DOI
Yue Wang, Donglei Zhou, Wen Feng Xu

et al.

The Journal of Physical Chemistry Letters, Journal Year: 2024, Volume and Issue: 15(28), P. 7236 - 7243

Published: July 8, 2024

Yb3+ doped perovskite nanocrystals (PNCs) serve as efficient photoconverters, exhibiting quantum cutting emission at ∼980 nm, which aligns precisely with the optimal response region of silicon solar cells (SSCs). However, severe nonradiative recombination caused by defects in crystal lattice and film boundaries, along limitations small-scale preparation, restricts their commercial application. Here, we used Ru3+ to mitigate CsPbCl3 PNCs adjusted luminescence, achieving a 175% photoluminescence yield (PLQY). The results show that ions enter lattice, fill lead vacancies, passivate defects. Furthermore, cysteine effectively eliminates surface forming Pb–S bonds, resulting films remarkable 117% PLQY, demonstrating strong photoconversion capabilities. Uniformly knife-coated on 20 × cm2 photovoltaic glass, these increased SSC efficiency from 21.45% 23.15%. This study showcases cost-effective photoconverter scalable coating method boost large-area SSCs.

Language: Английский

Citations

1

CdSe-Based Quantum Dots Assisted Deep Ultraviolet Light Detection and Visualization DOI Creative Commons
Hua Xiao, Mingxin Liu, Jiarui Zhang

et al.

Optics Express, Journal Year: 2024, Volume and Issue: 32(20), P. 35015 - 35015

Published: Sept. 5, 2024

To clarify the positive effect of down-conversion process for ultraviolet (UV) and deep (DUV) light detection visualization, we choose, synthesize, characterize a spectrum direct-bandgap CdSe-based colloidal quantum dot (QD) solvents color-conversion layers (CCLs) across blue, green, yellow, orange, red hues. Their optical absorption, emission, response speeds under various UV DUV wavelength 280 nm, 372 405 nm are evaluated. The blue QD CCL demonstrated highest yield up to 0.68. By integrating this directly onto silicon-based photodiode, responded power 280-nm is significantly enhanced by 27 times; data decreases slightly 23 times when using orange QDs, due comparatively lower yield. For optimal result in communication system, QDs help exhibit 520 mV stimulated with 372-nm light, compared substantial improvement over original 120 mV. This enhancement makes reduces BER, especially at rates below 70 Mb/s, stronger avalanche photodiode (APD) 600 nm. Furthermore, demonstrate potential application patterning have also produced through inkjet printing, showcasing their printability, high stability air, pure color emission illumination. These results underscore significant full-color anti-counterfeiting solutions integration into flexible, printable wearables variety visualization applications.

Language: Английский

Citations

1

Multiparticle Synergistic Electrophoretic Deposition Strategy for High-Efficiency and High-Resolution Displays DOI
Xuefei Li, Jinyang Zhao, Hui Xiao

et al.

ACS Nano, Journal Year: 2024, Volume and Issue: 18(27), P. 17715 - 17724

Published: June 25, 2024

Colloidal nanoparticles offer unique photoelectric properties, making them promising for functional applications. Multiparticle systems exhibit synergistic effects on the properties of their individual components. However, precisely controlled assembly multiparticles to form patterned building blocks solid-state devices remains challenging. Here, we demonstrate a versatile multiparticle electrophoretic deposition (EPD) strategy achieve assembly, high-efficiency, and high-resolution patterns. Through elaborate surface design charge regulation nanoparticles, precise control over particle distribution (gradient or homogeneous structure) in films using EPD technique. The system integrates silicon oxide titanium synergistically enhancing emission efficiency quantum dots high level field. Furthermore, superiority our integrate into large-area full-color display panels with resolution 1000 pixels per inch. results suggest great potential developing expanding diverse

Language: Английский

Citations

0

Effects of Structural Variation in Electrospray Systems on Spray Characteristics DOI Creative Commons

Ji Yeop Kim,

Sang Ji Lee,

Mun Hee Lee

et al.

Soft Matter, Journal Year: 2024, Volume and Issue: 20(34), P. 6791 - 6799

Published: Jan. 1, 2024

Electrospraying is a method of atomizing fluids using high voltage potential difference. Since the atomization electrostatic does not directly charge nozzle but only uses difference, various equipment structures are possible. In case this study, 12 different nozzle, ring electrode, and substrate were configured, data on characteristics electrospray, such as spray modes applied voltage, coating area, current, velocity, factors used in industrial processes, verified. Data provided for generation process uniform continuous electrospray.

Language: Английский

Citations

0

Continuous wave laser fabrication of small pitch/size perovskite pixels realizes high-resolution color conversion micro-LED displays DOI
Teng Ma, Jun Chen, Ziyi Chen

et al.

Nanoscale, Journal Year: 2024, Volume and Issue: unknown

Published: Jan. 1, 2024

As a new generation of display technology, micro-light-emitting diodes (micro-LEDs) have been widely recognized owing to their excellent performance in brightness, contrast ratio, resolution,

Language: Английский

Citations

0

Highly Efficient and Linearly Polarized Light Emission of Micro-LED Integrated with Double-Functional Meta-Grating DOI
Xuzheng Wang, Zhenhuan Tian, Shilun Pei

et al.

Nano Letters, Journal Year: 2024, Volume and Issue: unknown

Published: Dec. 18, 2024

Linearly polarized micro light-emitting diodes (LP-Micro-LEDs) exhibit exceptional potential across diverse fields. The existing methods to introduce polarization initially unpolarized Micro-LEDs and further enhance the degree of are, however, at expense low luminous efficiency. We fabricated a GaN-based blue Micro-LED integrated with Al nanograting specially designed Ag/GaN meta-grating, which overcomes dilemma between efficiency by simultaneously introducing effects mode selection energy recycling. LP-Micro-LED achieves an average extinction ratio (ER) 21.92 dB within ±60°, showing 2.04-fold increase in 1.32-fold ER compared Ag reflector design. This approach opens way toward next generation high-efficiency low-cost optoelectronic devices encryption, displays, optical communication, medicine.

Language: Английский

Citations

0

Silica coating of quantum dots and their applications in optoelectronic fields DOI

Siting Cai,

Xiang Chen, Shuli Wang

et al.

Chinese Chemical Letters, Journal Year: 2024, Volume and Issue: unknown, P. 110798 - 110798

Published: Dec. 1, 2024

Language: Английский

Citations

0

Hybrid-Protected Perovskite Quantum Dot Films with Ultra-High Efficiency and Stability for LED Backlighting DOI Creative Commons
Loan Thi Ngo, Wen‐Tse Huang, Hemant Verma

et al.

ACS Applied Materials & Interfaces, Journal Year: 2024, Volume and Issue: unknown

Published: Nov. 19, 2024

All-inorganic lead halide perovskite quantum dots (PQDs) have emerged as highly promising materials for photonic and optoelectronic devices, solar cells, photocatalysts. However, PQDs encounter instability color separation issues because of ion diffusion. Current strategies mainly address stability in green CsPbBr3 PQDs, with limited focus on the red-mixed their inferior compared PQDs. Our study provides a new dual-protection methodology synthesizing high-efficiency red mixed-halide PQD films. Red CsPb(Br0.4I0.6)3 are embedded silicone resin then incorporated poly(methyl methacrylate) (PMMA) matrix to form PQDs@silicone/PMMA The high photoluminescence yield (PLQY) great recorded pure-red polymer film. ultrabright film was also successfully fabricated an outstanding PLQY beyond 94%. These films exhibited enhanced against thermal environmental degradation, attributed dense protective layer PMMA matrices by formation Si–halide Pb–O bonds, thereby reducing surface defects. Theoretical calculations reveal that combining improves interactions, eliminating uncoordinated Pb2+ enhancing stability. Applied white light-emitting diodes (WLEDs), these demonstrated broad gamut 143.4%, indicating potential efficient WLED backlighting.

Language: Английский

Citations

0