Advanced Materials,
Год журнала:
2024,
Номер
36(25)
Опубликована: Апрель 2, 2024
Stretchable
ionic
conductors
are
crucial
for
enabling
advanced
iontronic
devices
to
operate
under
diverse
deformation
conditions.
However,
when
employed
as
interconnects,
existing
struggle
maintain
stable
conduction
strain,
hindering
high-fidelity
signal
transmission.
Here,
it
is
shown
that
strain-insensitive
can
be
achieved
by
creating
a
solid-liquid
bicontinuous
microstructure.
A
fiber
from
polymerization-induced
phase
separation,
which
contains
solid
elastomer
interpenetrated
liquid
ion-conducting
phase,
fabricated.
The
spontaneous
partitioning
of
dissolved
salts
leads
the
formation
robust
self-wrinkled
interface,
fostering
development
highly
tortuous
channels.
Upon
stretch,
these
meandering
channels
straightened,
effectively
enhancing
conductivity
counteract
strain
effect.
Remarkably,
retains
till
fracture,
with
only
7%
resistance
increase
at
200%
strain.
This
approach
presents
promising
avenue
designing
durable
cables
capable
transmission
minimal
strain-induced
distortion.
Nature Communications,
Год журнала:
2024,
Номер
15(1)
Опубликована: Март 15, 2024
Abstract
Developing
fiber
electronics
presents
a
practical
approach
for
establishing
multi-node
distributed
networks
within
the
human
body,
particularly
concerning
triboelectric
fibers.
However,
realizing
monitoring
micro-physiological
activities
remains
challenging
due
to
intrinsic
variability
and
subtle
amplitude
of
physiological
signals,
which
differ
among
individuals
scenarios.
Here,
we
propose
technical
based
on
dynamic
stability
model
sheath-core
fibers,
integrating
micro-flexure-sensitive
enabled
by
nanofiber
buckling
an
ion
conduction
mechanism.
This
scheme
enhances
accuracy
signal
transmission
process,
resulting
in
improved
sensitivity
(detectable
at
ultra-low
curvature
0.1
mm
−1
;
flexure
factor
>21.8%
bending
range
10°.)
robustness
under
micro
flexure.
In
addition,
also
developed
scalable
manufacturing
process
ensured
compatibility
with
modern
weaving
techniques.
By
combining
precise
micro-curvature
detection,
fibers
unlock
their
full
potential
various
diagnoses,
upper
limb
muscle
strength
rehabilitation
training.
Advanced Functional Materials,
Год журнала:
2024,
Номер
34(44)
Опубликована: Июнь 22, 2024
Abstract
Tactile
sensors
have
garnered
considerable
interest
for
their
capacity
to
detect
and
quantify
tactile
information.
The
incorporation
of
microstructural
designs
into
flexible
has
emerged
as
a
potent
strategy
augment
sensitivity
pressure
variations,
thereby
enhancing
linearity,
response
spectrum,
mechanical
robustness.
This
review
underscores
the
imperative
progress
in
microstructured
sensors.
Subsequently,
discourse
transitions
prevalent
materials
employed
fabrication
sensor
electrodes,
encapsulation
layers,
active
sensing
mediums,
elucidating
merits
limitations.
In‐depth
discussions
are
devoted
adorned
with
microstructures,
including
but
not
limited
to,
micropyramids,
microhemispheres,
micropillars,
microporous
configurations,
microcracks,
topological
interconnections,
multilevel
constructs,
random
roughness,
biomimetic
microstructures
inspired
by
flora
fauna,
accompanied
exemplar
studies
from
each
category.
Moreover,
utility
within
realm
intelligent
environments
is
explicated,
highlighting
application
monitoring
physiological
signals,
detection
sliding
motions,
discernment
surface
textures.
culminates
critical
examination
paramount
challenges
predicaments
that
must
be
surmounted
further
development
enhance
functional
performance
sensors,
paving
way
integration
advanced
sensory
systems.
Advanced Materials,
Год журнала:
2024,
Номер
36(21)
Опубликована: Фев. 16, 2024
Abstract
Active
sensing
is
a
fundamental
aspect
of
human
and
animal
interactions
with
the
environment,
providing
essential
information
about
hardness,
texture,
tackiness
objects.
This
ability
stems
from
presence
diverse
mechanoreceptors
in
skin,
capable
detecting
wide
range
stimuli
sensorimotor
control
biological
mechanisms.
In
contrast,
existing
tactile
sensors
for
robotic
applications
typically
excel
identifying
only
limited
types
information,
lacking
versatility
requisite
strategies
to
extract
proactively.
Here,
inspired
by
haptic
perception,
skin‐inspired
artificial
3D
mechanoreceptor
(SENS)
multiple
mechanical
developed
bridge
action
closed‐loop
system
dynamic
exploration.
A
tensor‐based
non‐linear
theoretical
model
established
characterize
deformation
(e.g.,
tensile,
compressive,
shear
deformation)
SENS,
guidance
design
optimization
multimode
properties
high
fidelity.
Based
on
recognizing
objects
improved
accuracy
(≈96%)
further
demonstrated.
exploration
approach
shows
promise
such
as
autonomous
learning,
healthcare,
space
deep‐sea
Advanced Materials,
Год журнала:
2023,
Номер
36(17)
Опубликована: Ноя. 23, 2023
Bioinspired
artificial
skins
integrated
with
reliable
human-machine
interfaces
and
stretchable
electronic
systems
have
attracted
considerable
attention.
However,
the
current
design
faces
difficulties
in
simultaneously
achieving
satisfactory
skin-like
mechanical
compliance
self-powered
multimodal
sensing.
Here,
this
work
reports
a
microphase-separated
bicontinuous
ionogel
which
possesses
properties
mimics
sensing
ability
of
biological
skin
by
ion-driven
stimuli-electricity
conversion.
The
exhibits
excellent
elasticity
ionic
conductivity,
high
toughness,
ultrastretchability,
as
well
Young's
modulus
similar
to
that
human
skin.
Leveraging
ion-polymer
interactions
enabled
selective
ion
transport,
can
output
pulsing
or
continuous
electrical
signals
response
diverse
stimuli
such
strain,
touch
pressure,
temperature
sensitively,
demonstrating
unique
Furthermore,
ionogel-based
I-skin
concurrently
sense
different
decouple
variations
from
voltage
assistance
machine-learning
model.
ease
fabrication,
wide
tunability,
sensing,
environmental
tolerance
ionogels
demonstrate
new
strategy
development
next-generation
soft
smart
mechano-transduction
devices.
Advanced Functional Materials,
Год журнала:
2023,
Номер
33(52)
Опубликована: Сен. 12, 2023
Abstract
Ionogels
have
become
a
popular
material
in
flexible
electronics
and
soft
robotics
based
on
their
excellent
ionic
conductivity,
environmental
tolerance,
electrochemical
stability.
However,
it
remains
challenge
to
develop
an
ionogel
integrated
with
high
strength,
toughness,
self‐healing,
adhesion.
Herein,
novel
strategy
is
established
design
high‐strength
(0.97
MPa)
tensile
(980%),
crack
insensitivity,
self‐healing
the
cosolvent
method.
By
virtue
of
differential
interactions
between
specific
polymer
various
liquids
gradient
polarity,
systems
are
employed
achieve
high‐performance
ionogels
by
simple
one‐step
polymerization.
Gel
permeation
chromatography,
atomic
force
microscopy,
time‐domain
nuclear
magnetism,
density
functional
theoretical
calculation
used
analyze
reasons.
Microphase
separation
can
be
induced
hydrone
or
stretching
enhance
strength
ionogel.
Therefore,
assembled
as
strain
temperature
sensors
monitor
human
movement
person's
body
low
detection
threshold
(0.1
°C)
extreme
environments.
This
concept
creates
new
path
materials
performance,
provide
prospective
regulate
situ
microphase
change
performance
resulting
via
Angewandte Chemie International Edition,
Год журнала:
2023,
Номер
62(33)
Опубликована: Июнь 21, 2023
Designing
deformable
supercapacitors
(D-SCs)
that
have
robust
skeleton
and
smoothly
active
channels
for
charges
kinetic
migration
faradic
storage
are
highly
crucial
wearable
systems.
Here,
we
develop
the
high-performance
D-SCs
made
of
covalent
organic
frameworks(COF)@amino-modified
Ti3
C2
Tx
deposited
on
decorated
nylon
6
(DPA)
film
(COF@N-Ti3
/DPA)
via
layer-by-layer
fabrication.
The
hierarchical
COF@N-Ti3
/DPA
exhibits
admirable
specific
capacitance,
rate
performance
cycling
stability
in
three-electrode
system
due
to
superior
H+
property
large
interfacial
charge
transfer
clarified
by
density
functional
theory
calculations.
Additionally,
solid-state
deliver
favourable
energy
practical
energy-supply
applications.
Particularly,
present
high
stabilities,
with
regard
80.7,
80.6
83.4
%
capacitance
retention
after
5000
bending
cycles,
2000
stretching
cycles
folding
separately.
International Journal of Extreme Manufacturing,
Год журнала:
2023,
Номер
5(3), С. 032013 - 032013
Опубликована: Июнь 15, 2023
Abstract
Nanomaterial-based
flexible
sensors
(NMFSs)
can
be
tightly
attached
to
the
human
skin
or
integrated
with
clothing
monitor
physiological
information,
provide
medical
data,
explore
metaverse
spaces.
Nanomaterials
have
been
widely
incorporated
into
due
their
facile
processing,
material
compatibility,
and
unique
properties.
This
review
highlights
recent
advancements
in
NMFSs
involving
various
nanomaterial
frameworks
such
as
nanoparticles,
nanowires,
nanofilms.
Different
triggering
interaction
interfaces
between
metaverse/virtual
reality
(VR)
applications,
e.g.
skin-mechanics-triggered,
temperature-triggered,
magnetically
triggered,
neural-triggered
interfaces,
are
discussed.
In
context
of
interfacing
physical
virtual
worlds,
machine
learning
(ML)
has
emerged
a
promising
tool
for
processing
sensor
data
controlling
avatars
metaverse/VR
many
ML
algorithms
proposed
technologies.
paper
discusses
advantages,
disadvantages,
prospects
applications.