The
conventional
Slippery
Liquid
Infused
Porous
Surface
(SLIPS)
encounters
challenges
such
as
silicone
oil
leakage
and
complex
manufacturing
of
rough
substrate
structures.
Thus,
it
is
crucial
to
develop
a
lubricant
that
highly
adaptable
less
prone
loss
for
surface
structures;
temperature-controlled
method
infusing
oleogel
into
superhydrophobic
(SHS)
presented
in
this
paper.
This
approach
draws
inspiration
from
the
characteristics
Nepenthes
pitcher
plant
structures,
albeit
without
need
intricate
pore-making
or
nanowire
It
demonstrated
resulting
has
exceptional
fog
harvesting
capability,
with
efficiency
0.3222
g
cm
ACS Applied Materials & Interfaces,
Год журнала:
2024,
Номер
16(26), С. 34089 - 34099
Опубликована: Июнь 18, 2024
Slippery
liquid-infused
porous
surfaces
(SLIPSs)
have
great
potential
to
replace
traditional
antifouling
coatings
due
their
efficient,
green,
and
broad-spectrum
performance.
However,
the
lubricant
dissipation
problem
of
SLIPS
severely
restricts
its
further
development
application,
robust
continues
be
extremely
challenging.
Here,
a
composite
phase-change
layer
consisting
paraffin,
silicone
oil,
MXene
is
designed
readily
construct
stable
NIR-responsive
self-healing
solid
slippery
surface
(PCSSS).
Collective
results
showed
that
PCSSS
could
rapidly
achieve
transformation
complete
under
NIR
irradiation
keep
after
high-speed
water
flushing,
centrifugation,
ultrasonic
treatment.
The
performance
evaluated
by
protein,
bacteria,
algae
antiadhesion
tests
demonstrated
adhesion
inhibition
rate
was
as
high
99.99%.
Moreover,
EIS
potentiodynamic
polarization
experiments
indicated
had
exceptional
corrosion
resistance
(|
Advanced Functional Materials,
Год журнала:
2024,
Номер
unknown
Опубликована: Дек. 15, 2024
Abstract
Organic
protective
coatings
encounter
significant
challenges
in
the
face
of
mechanical
damage,
weathering
degradation,
and
corrosion
activities.
Developing
that
feature
both
autonomous
damage
reporting
enhanced
durability
is
a
promising
yet
challenging
endeavor.
In
this
study,
inspired
by
“damage
coloration”
lurid
bolete,
multifunctional
smart
coating
integrating
color/fluorescence
reporting,
resistance,
active
protection
capabilities
developed
incorporating
microcapsules
encapsulated
with
crystal
violet
lactone
(CVL)
cerium
oxide
(CeO
2
)
nanoparticles
into
polyurethane
(PU)
resins.
CVL,
damage‐reporting
indicator
exhibiting
color
fluorescence
emission,
within
PU/poly‐(urea
formaldehyde)
(PU/UF)
microcapsules.
CVL
released
from
upon
localized
enhancement
under
UV
irradiation
an
intense
blue
coloration
resulting
chromogenic
reaction
CeO
nanoparticles.
addition
to
initiating
confer
outstanding
resistance
matrix
through
their
absorption
inhibition
properties.
The
performance
improvement
composite
terms
verified
situ
transmittance
testing
real‐time
atmospheric
monitoring.
Polymers for Advanced Technologies,
Год журнала:
2025,
Номер
36(3)
Опубликована: Март 1, 2025
ABSTRACT
Ship
surface
fouling
poses
serious
constraints
on
ship
navigation
and
the
marine
environment.
Now
that
traditionally
harmful
antifouling
coatings
have
been
banned
worldwide,
development
of
new
for
ships
are
environmentally
friendly
functionally
stable
is
imminent.
Low
energy
with
structural
biomimetic
properties
safest,
most
friendly,
effective
breakthrough
in
preventing
deposits
hull
surfaces.
This
article
first
explains
mechanism
coatings,
comprehensively
describes
morphology
bionic
microstructure,
summarizes
construction
method
structure.
On
this
basis,
low
fluorine‐containing
silicone‐containing
materials,
as
well
current
application
ships,
analyzed.
In
addition,
stimulus–response
coatings.
reviews
research
progress
based
structures
recent
years,
presents
challenges
future
directions
field,
provides
unique
insights
to
further
optimize
performance
these
ACS Applied Materials & Interfaces,
Год журнала:
2025,
Номер
unknown
Опубликована: Март 19, 2025
Eco-friendly,
flexible,
and
fluorine-free
antismudge
coatings
have
broad
applications
in
soft
substrates
such
as
fabrics,
premium
leather,
synthetic
flexible
electronic
devices.
However,
developing
possessing
both
excellent
durability
desirable
softness
stretchability
remains
a
formidable
challenge.
Herein,
two
waterborne
silicone-based
emulsions
were
prepared
via
emulsion
inversion
point
method,
using
high-molecular-weight
divinyl-terminated
poly(dimethylsiloxane)
(ViPDMSVi)
methyl
vinyl
MQ
resin
raw
materials,
respectively,
with
polyether-modified
silicone
(D(PDMS)PE)
compounding
sodium
dodecyl
sulfate
(SDS)
emulsifiers.
Subsequently,
poly(methylhydrosiloxane)
(PHSE)
was
utilized
cross-linking
agent,
highly
comprehensive
coating
successfully
fabricated
through
hydrosilylation
among
the
three
types
of
emulsions.
Owing
to
rational
structural
design
aqueous-based
strategy,
achieves
integration
high
mechanical
properties
(≥3.5
MPa
tensile
strength
214%
elongation)
stretchability,
outstanding
flexibility
(the
glass
transition
temperature
below
-105
°C),
transparency,
self-cleaning,
performance.
Moreover,
exceptional
is
evidenced
by
maintaining
after
rigorous
treatments,
24
h
UV
irradiation,
immersion
acid,
alkali,
salt
solutions
for
h,
500
cycles
abrasion
under
load
1000
g,
etc.
This
work
provides
feasible
pathway
manufacturing
high-performance
suitable
green
sustainable
manner.
ACS Applied Materials & Interfaces,
Год журнала:
2025,
Номер
unknown
Опубликована: Март 23, 2025
Oxidative
stress
derived
from
excess
reactive
oxygen
radicals
(ROS)
induces
cellular
damage,
apoptosis,
and
necrosis,
thus
effective
biofouling
control
by
directly
inhibiting
primary
membrane
formation.
However,
the
oxidative
produced
that
does
not
rely
on
additional
energy
still
is
a
challenge.
Herein,
an
oxidative-stress-mediated
marine
antifouling
polyurea
coating
prepared
leveraging
strong
electron
absorption
effect
of
C═N.
Given
structure
urethane
bond,
reversible
reaction
barrier
dynamic
bond
can
be
reduced,
thereby
enabling
to
broken
without
need
for
energy.
The
alkyl
radical
(R·)
originating
oxime-urethane
mediate
induction
in
cells
microbial
death,
preserving
exceptional
properties
resisting
most
organism
adhere
substrates.
Notably,
indicates
satisfactory
antibacterial
antialgae
performance
exhibits
8
months
field
performance.
In
addition,
investigated
theoretical
calculation,
interface
behavior
molecular
dynamics
simulation.
This
work
presents
pioneering
example
construction
coating,
which
might
judicious
design
strategy
environmentally
friendly
coating.
Advanced Functional Materials,
Год журнала:
2025,
Номер
unknown
Опубликована: Апрель 30, 2025
Abstract
Healable
antifouling
materials
contribute
a
paradigm
shift
for
extending
marine
infrastructure
lifespan
by
forming
continuable
biofouling
barriers.
However,
achieving
sustainable
performance
in
extreme
mechanical
stresses
remains
challenging
due
to
the
difficulty
of
integrating
stiffness,
toughness,
and
healing
with
efficacy.
Inspired
meniscus,
which
facilitates
efficient
load
absorption
distribution
ability
through
remarkable
resilience
accurate
intercalation
between
thigh
calf
bones,
structural‐bioinspired
segmented
network
strategy
is
proposed.
This
approach
integrates
secondary
meniscus‐inspired
bisphenol
segments
into
primary,
reorganizing
rigid
phases
optimizing
crosslinking
primary
ensure
uniform
stress
dissipation
augment
molecular
dynamism.
design
yields
212.32%
increase
Young’
s
modulus
(362.42
MPa),
55.62%
improvement
toughness
(169.52
MJ
m
−
3
),
an
enhancement
self‐healing
efficiency
from
72.81%
98.75%.
establishes
new
principle
durable
healable
materials,
combining
enhanced
properties
resistance
against
biofouling.
Advanced Materials,
Год журнала:
2025,
Номер
unknown
Опубликована: Май 16, 2025
Abstract
The
exceptional
underwater
adhesion
and
self‐healing
capabilities
of
mussels
have
fascinated
researchers
for
over
two
decades.
Extensive
studies
shown
that
these
remarkable
properties
arise
from
a
series
reversible
dynamic
molecular
interactions
involving
mussel
foot
proteins.
Inspired
by
interaction
strategies,
numerous
functional
materials
exhibiting
strong
performance
been
successfully
developed.
This
review
systematically
explores
the
nanomechanical
mechanisms
mussel‐inspired
interactions,
mainly
revealed
direct
force
measurement
techniques
such
as
surface
forces
apparatus
atomic
microscopy.
development
materials,
including
coacervates,
coatings,
hydrogels,
with
properties,
is
then
summarized.
Furthermore,
macroscopic
material
performances
are
correlated
underlying
mechanisms,
providing
valuable
insights
rational
design
next‐generation
enhanced
properties.
