Electrochemical Cell Designs for Efficient Carbon Dioxide Reduction and Water Electrolysis: Status and Perspectives DOI Creative Commons
Zhangsen Chen, Lei Zhang, Shuhui Sun

и другие.

Advanced Materials, Год журнала: 2025, Номер unknown

Опубликована: Май 30, 2025

Abstract Integrating renewable electricity and concentrated CO 2 from direct air capture, electrochemical reduction reactions (eCO RR) offer a promising pathway for converting into fuel chemicals, enabling the closure of carbon loop in sustainable manner. The clean H produced via hydrogen evolution reaction (HER) during water electrolysis can replace traditional fossil fuels without additional emissions. Achieving large‐scale high‐efficiency eCO RR HER requires development rational electrolyzer designs, which are crucial industrial implementation. This review examines recent innovations system designs RR, HER, latest advances situ cell operando characterization reactions. It focuses on improvements flow patterns, membrane electrode assemblies, electrolyte engineering to maximize catalytic activities at level. Besides, discusses optimizing counter‐anodic improve energy efficiency electrolysis, offering insights design systems with efficient utilization. Furthermore, it explores integration other (e.g., cells), highlighting their potential role decarbonization future processes. Finally, summary, challenge, outlook industrial‐scale concluded.

Язык: Английский

Mesoporous carbon materials doped with Co, Fe and nitrogen as oxygen reduction reaction electrocatalysts for anion-exchange membrane fuel cell DOI

Johanna Katariina Piir,

Jaana Lilloja, Maike Käärik

и другие.

Electrochimica Acta, Год журнала: 2025, Номер unknown, С. 146226 - 146226

Опубликована: Апрель 1, 2025

Язык: Английский

Процитировано

0

Advanced Development of High‐Entropy Alloys in Catalytic Applications DOI
Zhenfeng Zhu, Zijun Li, Zihe Liu

и другие.

Small Methods, Год журнала: 2025, Номер unknown

Опубликована: Апрель 15, 2025

Abstract Conventional alloys have long been limited by their simple compositions, which make it difficult to meet the requirements of modern catalysis applications. In contrast, high‐entropy (HEAs), characterized multi‐principal elements in near‐equimolar ratios, become a transformative paradigm materials science since inception 2004. The unique core effects HEAs, including effect, severe‐lattice distortion sluggish‐diffusion and cocktail endow them with superior catalytic properties activity, selectivity, durability. However, rapid advanced development comprehensive review applications is imperative foster deeper understanding. this review, capability commencing from entropy‐driven mechanism HEAs systematically explored. Then, are comprehensively analyzed diverse fields, energy conversion, chemical industries, environmental remediation, emphasizing remarkable capabilities Finally, pivotal challenges outlined synthesis methods, mechanistic elucidation, green manufacturing, propose future directions such as database establishment machine‐learning‐assisted design. By addressing knowledge gaps inspiring innovative strategies, aims accelerate translation into practical solutions for sustainable future.

Язык: Английский

Процитировано

0

Microporous poly(aryl piperidinium) hydroxide exchange membranes with multi-directional branched structure for high performance fuel cells DOI
Jian Gao, Jialin Zhao,

Shiyao Sun

и другие.

Journal of Colloid and Interface Science, Год журнала: 2025, Номер unknown, С. 137676 - 137676

Опубликована: Апрель 1, 2025

Язык: Английский

Процитировано

0

Amphoteric Metal Ion‐Coordinated Chitosan Membranes for Efficient Hydroxide Ion Transport DOI
Jikang Wang, Jiaxing Zhang,

Jinghui Wang

и другие.

Chemistry - An Asian Journal, Год журнала: 2025, Номер unknown

Опубликована: Апрель 30, 2025

Hydroxide exchange membranes (HEMs) have attracted extensive attention in energy-related fields, such as fuel cells and water electrolysis, primarily due to their suitability for alkaline environments. However, the practical application of is hindered significantly by limited conductivity. In this study, a series amphoteric metal ion-coordinated chitosan (CTS-AM) with enhanced hydroxide ion conductivity are reported. The CTS-AM prepared using simple soaking-drying method, exhibiting excellent mechanical strength thermal stability strong coordination bonds between ions chains. To best our knowledge, Zn2+ coordinated membrane achieved highest-ever reported 82.0 ± 5.4 mS cm-1 at 25 °C 100% RH, value increasing 301.0 6.7 operating temperature (80 °C) RH. Through combined structural analysis theoretical calculations, we propose that formation nanochannels lowered barrier electron transfer responsible high conductivities membranes. This study presents viable approach design fabrication high-performance HEMs energy storage devices other applications.

Язык: Английский

Процитировано

0

Polyethylene terephthalate (PET) waste in Electrochemical applications DOI Creative Commons
Varun Donnakatte Neelalochana, Paolo Scardi, Narges Ataollahi

и другие.

Journal of environmental chemical engineering, Год журнала: 2025, Номер unknown, С. 116823 - 116823

Опубликована: Апрель 1, 2025

Язык: Английский

Процитировано

0

Holistic nanoarchitectonic design of hierarchically structured oxygen reduction reaction catalyst DOI
Atanu Panda, Abin Sebastian, Ravi Nandan

и другие.

Chemical Engineering Journal, Год журнала: 2025, Номер unknown, С. 163959 - 163959

Опубликована: Май 1, 2025

Язык: Английский

Процитировано

0

Electrochemical Cell Designs for Efficient Carbon Dioxide Reduction and Water Electrolysis: Status and Perspectives DOI Creative Commons
Zhangsen Chen, Lei Zhang, Shuhui Sun

и другие.

Advanced Materials, Год журнала: 2025, Номер unknown

Опубликована: Май 30, 2025

Abstract Integrating renewable electricity and concentrated CO 2 from direct air capture, electrochemical reduction reactions (eCO RR) offer a promising pathway for converting into fuel chemicals, enabling the closure of carbon loop in sustainable manner. The clean H produced via hydrogen evolution reaction (HER) during water electrolysis can replace traditional fossil fuels without additional emissions. Achieving large‐scale high‐efficiency eCO RR HER requires development rational electrolyzer designs, which are crucial industrial implementation. This review examines recent innovations system designs RR, HER, latest advances situ cell operando characterization reactions. It focuses on improvements flow patterns, membrane electrode assemblies, electrolyte engineering to maximize catalytic activities at level. Besides, discusses optimizing counter‐anodic improve energy efficiency electrolysis, offering insights design systems with efficient utilization. Furthermore, it explores integration other (e.g., cells), highlighting their potential role decarbonization future processes. Finally, summary, challenge, outlook industrial‐scale concluded.

Язык: Английский

Процитировано

0