Nonisothermal Crystallization Behavior and Crystallization Morphology of Three‐Arm Polylactic Acid With Different Chain Lengths DOI

Aiqiang Yang,

Le Yue, Yihan Shao

и другие.

Journal of Applied Polymer Science, Год журнала: 2025, Номер unknown

Опубликована: Апрель 15, 2025

ABSTRACT To investigate the effects of chain length on crystallization ability three‐arm polylactic acid (TA‐PLA), a series TA‐PLA samples with different lengths were synthesized by ring‐opening polymerization lactide. Differential scanning calorimetry (DSC) was used to study their nonisothermal behavior, and polarized optical microscope (POM) observe isothermal morphology. The analysis revealed that increase in reduced TA‐PLA. For instance, 12.1 longest only exhibited crystallinity 38.21% at cooling rate 1°C/min, whereas 3.9 reached up 70.75%. Mo equation provided an accurate description kinetics shown simulate process sample successfully. From photographs captured using POM, it evident long chains slowed growth (G) spherical crystals samples. Furthermore, distinct temperature dependencies spherulitic rates.

Язык: Английский

The Biomechanical Properties of A Modified Distraction Device Used in Mandibular Distraction Osteogenesis for Craniofacial Microsomia Patients: A Simulation Finite Element Analysis Study DOI
Anna Liu,

Changjin Huang,

Wei Liu

и другие.

Journal of Craniofacial Surgery, Год журнала: 2025, Номер unknown

Опубликована: Янв. 10, 2025

Objective: Finite element analysis (FEA) of the biomechanical properties modified extraoral distractor device used in mandibular distraction craniofacial microsomia patients. Materials and Methods: models 5 patients under 2 working conditions, instance when is activated participates mastication, were included current study. To conduct FEA, load boundary conditions (35.6 N on for first condition 50 unoperated side, 100 200 both sides second condition) applied. Besides, constraint contact also Results: With or 3 bioabsorbable screws fixing upper plate, maximal displacement mandible was <3 mm stress distributed less than yield strength corresponding materials setting side condition. However, condition, slightly increased, exceeded some Conclusion: In most cases, poly-L-lactic acidscrews could firmly fix without plastic deformation, although situation would be different mastication force too powerful.

Язык: Английский

Процитировано

0

Triazole Drives Hole Localization and Superoxide Radical Formation for Enhancive Photocatalytic Cascade Isomerization/C─C Bond Scission of Biomass to Lactic Acid DOI Open Access
Chenguang Liu,

Jinshu Huang,

Yu Wen

и другие.

Small, Год журнала: 2025, Номер unknown

Опубликована: Янв. 31, 2025

Chemocatalytic synthesis of lactic acid (LA) from biomass sugars involves heat-absorbing multistep cascade reactions mediated by different active sites, often encountering unsatisfactory selectivity. Here, a hole-localized carbon nitride-based photocatalyst (C-CNN) is constructed covalent binding heptazine and triazole skeleton via C─N bonds further conjugated interaction with activated carbon, achieving the complete conversion various to LA (up 98.6% selectivity) at room temperature for 2 h. The introduced electron donor in C-CNN can not only enhance adsorption sugar enhanced aldose-to-ketose isomerization over localized hole (Lewis acid) on skeleton, but also modulate valence band oxidation circumvent formation •OH •O2 ‒ selective C3‒C4 cleavage ketose, thus realizing exclusive LA. Moreover, near-infrared light absorption endowed supply sufficient interface photothermal effect ambient production. Life cycle assessment shows that photocatalytic system has good prospects industrialization terms both energy environment. This work offers novel insights into multidirectional utilization solar value-added through rational modulation sites.

Язык: Английский

Процитировано

0

High-Efficiency and Low-Resistance Melt-Blown/Electrospun PLA Composites for Air Filtration DOI Open Access
Yongmei Guo, Mingdong Wu, Xiaojian Ye

и другие.

Polymers, Год журнала: 2025, Номер 17(3), С. 424 - 424

Опубликована: Фев. 6, 2025

Biodegradable polylactic acid (PLA) was used to fabricate nonwoven fabrics via the melt blowing process, followed by electrospinning deposit a nanofiber membrane. This composite process yielded PLA melt-blown/electrospun materials with excellent filtration performance. The effects of solution concentration and spinning duration on structure material performance were investigated. optimal produced using 10 wt.% prepared solvent mixture dichloromethane (DCM) N, N-dimethylformamide (DMF) in 75/25 weight ratio. parameters included 5 h, 18 kV voltage, 1.5 mL/h flow rate, 12 cm collection distance. resulting achieved efficiency 98.7%, pressure drop 142 Pa, an average pore size μm, contact angle 138.7°. These results provided for preparing materials. study highlights potential hydrophobic composites high low air resistance as environmentally friendly alternatives traditional non-degradable

Язык: Английский

Процитировано

0

Unraveling the Crystallization, Mechanical, and Heat Resistance Properties of Poly(butylene adipate-co-terephthalate) Through the Introduction of Stereocomplex Crystallites DOI Creative Commons
Min Qiao, Tao Zhang, Jing Jiang

и другие.

Crystals, Год журнала: 2025, Номер 15(3), С. 247 - 247

Опубликована: Март 6, 2025

Poly(butylene adipate-co-terephthalate) (PBAT) is a promising degradable polymer for replacing non-degradable traditional plastics to mitigate pollution. However, its low softening temperature and poor hardness impede application. Herein, PBAT stereocomplex polylactide (sc-PLA) blends were fabricated through melt-blending process balance the heat resistance mechanical strength of in this research. The effects PLA content hot embossing on blend properties comprehensively investigated. results demonstrate that sc-crystal PBAT/sc-PLA increased by 493% as rose from 10% 30%. with 15% PLLA PDLA, embossed at 190 °C, exhibited highest sc-PLA crystallinity 23.3% largest fraction sc-crystallites 66%, leading optimal comprehensive performance. Its Vicat (VST) reached 92.2 nonlinear increase trend accordance power-law model between VST mass ratio was obtained. Compared neat PBAT, maximum tensile yield stress 9.7 MPa Young’s modulus 82.5 achieved improved approximately 107% 361%, respectively. This research offers an effective strategy synergistically enhancing PBAT.

Язык: Английский

Процитировано

0

Preparation of piezoelectric β-PLA utilizing a micro-shear field in non-solvent induced phase separation DOI

Qianyu Wei,

Weicheng Gao, Tianze Zhang

и другие.

Chemical Engineering Journal, Год журнала: 2025, Номер unknown, С. 161804 - 161804

Опубликована: Март 1, 2025

Язык: Английский

Процитировано

0

Enhancing Antibacterial and Mechanical Properties of Polylactic Acid Fibers Through Trace Coordination Bonding With Nano‐Cu2O for Sustainable Public Textiles DOI
Tao Ding, Zhang Fei, Yanyan Ma

и другие.

Journal of Applied Polymer Science, Год журнала: 2025, Номер unknown

Опубликована: Апрель 15, 2025

ABSTRACT Public Textiles require high durability and safety, yet common materials like cotton, linen, silk, wool are prone to harboring pathogens experiencing mechanical deterioration due microbial activity. Developing fibers with exceptional antimicrobial properties for is crucial but challenging. Herein, a trace coordination bond crosslinking strategy was proposed prepare nano‐Cu 2 O/polylactic acid (Cu O/PLA) highly antibacterial activity, robustness, recyclability. The dynamic bonds allow uniform dispersion of O in PLA, improving molecular chain interfaces resulting excellent performance (tensile fracture strength 48.75 MPa). combination O's capacity PLA's weak acidity provides superior activity (99.99%) against various pathogens. This enables Cu O/PLA demonstrate an shelf life exceeding 6 months. Additionally, the ease breaking regenerating grants Therefore, this offers novel viable approach preparing nanocomposite PLA properties, addressing challenges faced Textiles.

Язык: Английский

Процитировано

0

Nonisothermal Crystallization Behavior and Crystallization Morphology of Three‐Arm Polylactic Acid With Different Chain Lengths DOI

Aiqiang Yang,

Le Yue, Yihan Shao

и другие.

Journal of Applied Polymer Science, Год журнала: 2025, Номер unknown

Опубликована: Апрель 15, 2025

ABSTRACT To investigate the effects of chain length on crystallization ability three‐arm polylactic acid (TA‐PLA), a series TA‐PLA samples with different lengths were synthesized by ring‐opening polymerization lactide. Differential scanning calorimetry (DSC) was used to study their nonisothermal behavior, and polarized optical microscope (POM) observe isothermal morphology. The analysis revealed that increase in reduced TA‐PLA. For instance, 12.1 longest only exhibited crystallinity 38.21% at cooling rate 1°C/min, whereas 3.9 reached up 70.75%. Mo equation provided an accurate description kinetics shown simulate process sample successfully. From photographs captured using POM, it evident long chains slowed growth (G) spherical crystals samples. Furthermore, distinct temperature dependencies spherulitic rates.

Язык: Английский

Процитировано

0