Homogenizing Electron and Hole Transport Layers in Tin Perovskite Solar Cells to Enhance Photocurrent and Voltage DOI
Qinyu Ning, Donghao Miao, Mingyu Ma

и другие.

ACS Applied Materials & Interfaces, Год журнала: 2025, Номер unknown

Опубликована: Май 23, 2025

Tin perovskite solar cells (TPSCs) are considered as a sustainable alternative to their lead-containing counterparts, offering an ideal bandgap, more stable crystal structure, and better semiconducting properties. However, the fabrication of efficient able TPSCs has been challenging task. Among main components TPSCs, herein, we investigated transport layers interface with layer. Several microscopy techniques revealed inhomogeneity in common hole layer, poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS), electron layer (ETL), indene-C60 bisadduct (ICBA). A hydrogen-bond donor molecule d-sorbitol modified microstructure PEDOT:PSS, increasing its conductivity crystallization density overlying Blending 1% poly(methyl methacrylate) into ICBA rendered uniform ETL, which facilitated across tin perovskite. The photocurrent density, open-circuit voltage, fill factor were all enhanced achieve power conversion efficiency 15.8% excellent short-term stability. Our findings address often-neglected aspect device provide new approach boosting performance reproducibility TPSCs.

Язык: Английский

Improving the Stability of Wide Bandgap Perovskites: Mechanisms, Strategies, and Applications in Tandem Solar Cells DOI

Wenye Jiang,

Yuemin Zhu, Jin Liu

и другие.

Advanced Materials, Год журнала: 2025, Номер unknown

Опубликована: Апрель 7, 2025

Abstract Tandem solar cells (TSCs) based on wide bandgap (WBG) perovskites have gained significant attention for their higher power conversion efficiency (PCE) compared to single‐junction cells. The role of WBG perovskite (PSCs) as the sub‐cell in tandem consists absorbing high‐energy photons and producing open‐circuit voltages ( V OC ). However, PSCs face serious phase separation issues, resulting poor long‐term stability substantial loss TSCs. In response, researchers developed a range strategies mitigate these challenges, showing promising progress, comprehensive review is expected. this review, we discuss mechanism organic–inorganic hybrids all‐inorganic perovskites. Additionally, conduct an in‐depth investigation various enhance stability, including component engineering, additive interface dimension control, solvent encapsulation. Furthermore, application TSCs summarized detail. Finally, perspectives are provided offer guidance development efficient stable field

Язык: Английский

Процитировано

1
Enhancing Interfacial Contact in Perovskite/Silicon Tandem Solar Cells Through TaOX Passivation DOI

Yihan Sun,

Zhiqin Ying, Xin Li

и другие.

Small, Год журнала: 2025, Номер unknown

Опубликована: Май 5, 2025

Abstract Perovskite/silicon tandem solar cells demonstrating tremendous potential for commercialization that position them as a transformative technology in photovoltaics. However, the poor interface contact between perovskite and C 60 has long been critical factor limiting power conversion efficiency (PCE) of top cells. Here, multifunctional inorganic tantalum oxide (TaO X) film passivation layer is introduced, which not only suppresses recombination across but also improves energy level alignment enhances charge extraction at perovskite/C interface. More importantly, TaO X demonstrates exceptional thermal stability, significantly overall stability device. These synergistic effects enable fabrication single‐junction cell with PCE 21.0% bandgap 1.68 eV. Furthermore, when combined double‐sided tunnel passivated silicon bottom cell, 29.5% 1 cm 2 achieved. unencapsulated ‐based devices exhibited improved subjected to ISOS‐L‐1 accelerated aging conditions.

Язык: Английский

Процитировано

0
Homogenizing Electron and Hole Transport Layers in Tin Perovskite Solar Cells to Enhance Photocurrent and Voltage DOI
Qinyu Ning, Donghao Miao, Mingyu Ma

и другие.

ACS Applied Materials & Interfaces, Год журнала: 2025, Номер unknown

Опубликована: Май 23, 2025

Tin perovskite solar cells (TPSCs) are considered as a sustainable alternative to their lead-containing counterparts, offering an ideal bandgap, more stable crystal structure, and better semiconducting properties. However, the fabrication of efficient able TPSCs has been challenging task. Among main components TPSCs, herein, we investigated transport layers interface with layer. Several microscopy techniques revealed inhomogeneity in common hole layer, poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS), electron layer (ETL), indene-C60 bisadduct (ICBA). A hydrogen-bond donor molecule d-sorbitol modified microstructure PEDOT:PSS, increasing its conductivity crystallization density overlying Blending 1% poly(methyl methacrylate) into ICBA rendered uniform ETL, which facilitated across tin perovskite. The photocurrent density, open-circuit voltage, fill factor were all enhanced achieve power conversion efficiency 15.8% excellent short-term stability. Our findings address often-neglected aspect device provide new approach boosting performance reproducibility TPSCs.

Язык: Английский

Процитировано

0