Dough‐Kneading‐Inspired Universal Mixing Strategy for Mass Production of Multi‐Stimuli‐Responsive Hydrogels DOI
Wen‐Yao Huang, Chen Yao, Jingjing Xiao

и другие.

Advanced Functional Materials, Год журнала: 2025, Номер unknown

Опубликована: Май 5, 2025

Abstract Inspired by dough kneading, a straightforward and versatile mixing strategy is proposed for the safe, rapid, large‐scale production of smart hydrogels. This approach achieved directly blending gel powders with an appropriate amount swelling agent. The applied possess strong adhesion, enabling them to function as both glue bonding different hydrogels healing agents repairing damaged hydrogels, while their recyclability reusability help lower costs minimize environmental impact. resulting hydrogel, featuring unique internal heterogeneous porous structure, exhibits fast response speed, excellent recoverability, high fatigue resistance. Mechanical tests reveal that this hydrogel robust, capable resisting large elongations (>400%) without breaking, enduring multiple compressions (53%, 10 cycles) crushing, maintaining integrity during prolonged immersion (≈1032 h). Through precise control composition spatial distribution replaceable agents, enables customizable architectures selective shape‐morphing functionality under programmed stimuli. Overall, scalable paradigm establishes eco‐conscious manufacturing platform high‐throughput synthesis stimuli‐responsive materials, positioning it key enabler next‐generation soft devices.

Язык: Английский

Cartilage Lubrication from the Perspective of Wettability DOI

Xuhao Yang,

Feng Gao, Wenlong Song

и другие.

ACS Nano, Год журнала: 2025, Номер unknown

Опубликована: Апрель 2, 2025

Cartilage exhibits an extremely low friction and very wearability within the liquid environment of joint. It is also capable switching wettability between superhydrophilicity hydrophobicity in both wetting dry conditions (specific experimental operations or open wounds). Therefore, understanding cartilage lubrication from perspective provides inspiration for design artificial sections with motion soft actuators coefficients (COF). In this review, articular introduced discussed view wettability. First, basic principles are described a focus on compositions cartilage, particular relationship phospholipid layers supramolecular synergy synovial fluid cartilage. Subsequently, under different stimuli (such as shear, pH, temperature, electric field) insights into lubrication. Finally, we present comprehensive summary delineate challenges domain assisting researchers formulating viable concepts efficient substitution smart lubricating devices.

Язык: Английский

Процитировано

0

Supramolecular Polyzwitterionic Nanoparticles with Engineered pH‐Responsiveness and Cartilage‐Penetration for Osteoarthritis Therapy DOI

Shaopei Ding,

Peng Yu, Peng Xu

и другие.

Advanced Functional Materials, Год журнала: 2025, Номер unknown

Опубликована: Апрель 27, 2025

Abstract Abnormal friction forces, compact matrix structure, and dynamic acidic microenvironment in osteoarthritis (OA) make it difficult to remodel cartilage regeneration by integrating prominent inflammatory responses anabolism. Here, pH‐responsive PSBMA‐ b ‐PColBP@KGN nanoparticles (PSPK NPs) are developed a simple supramolecular assembly process. PSPK NPs found reduce the coefficient of (0.028) under high loading pressure (10.41 MPa). The synergistic effect KGN release coupling deep penetration promotes generation microenvironment. Further, vivo studies confirm potential restoring homeostasis, as evidenced reduced osteophyte volume, aligned structures, abundant matrix. This study provides novel insights into effects release, penetration, hydration lubrication on OA treatment, offering strategy for design tissue‐adaptive promote tissue inflammation‐related diseases.

Язык: Английский

Процитировано

0

Dough‐Kneading‐Inspired Universal Mixing Strategy for Mass Production of Multi‐Stimuli‐Responsive Hydrogels DOI
Wen‐Yao Huang, Chen Yao, Jingjing Xiao

и другие.

Advanced Functional Materials, Год журнала: 2025, Номер unknown

Опубликована: Май 5, 2025

Abstract Inspired by dough kneading, a straightforward and versatile mixing strategy is proposed for the safe, rapid, large‐scale production of smart hydrogels. This approach achieved directly blending gel powders with an appropriate amount swelling agent. The applied possess strong adhesion, enabling them to function as both glue bonding different hydrogels healing agents repairing damaged hydrogels, while their recyclability reusability help lower costs minimize environmental impact. resulting hydrogel, featuring unique internal heterogeneous porous structure, exhibits fast response speed, excellent recoverability, high fatigue resistance. Mechanical tests reveal that this hydrogel robust, capable resisting large elongations (>400%) without breaking, enduring multiple compressions (53%, 10 cycles) crushing, maintaining integrity during prolonged immersion (≈1032 h). Through precise control composition spatial distribution replaceable agents, enables customizable architectures selective shape‐morphing functionality under programmed stimuli. Overall, scalable paradigm establishes eco‐conscious manufacturing platform high‐throughput synthesis stimuli‐responsive materials, positioning it key enabler next‐generation soft devices.

Язык: Английский

Процитировано

0