Sustainable carbon sources for green laser-induced graphene: A perspective on fundamental principles, applications, and challenges

Applied Physics Reviews, Год журнала: 2022, Номер 9(4)

Опубликована: Ноя. 10, 2022

Since the discovery of laser-induced graphene (LIG), significant advances have been made to obtain green LIG (gLIG) from abundant, eco-friendly, natural, and organic renewable bio-based carbon sources. Recently, some sustainable cost-effective electronic devices designed with gLIG, resulting in diverse solutions environmental impact caused by waste (e-waste). However, there are still several challenges that must be addressed regarding widespread market implementation gLIG-based products, synthesis practical applications. In this review, we focus on precursor sources, their conversion mechanisms, physical chemical properties applications, along related its implementation, showing future opportunities perspectives promising new material. Various systems based gLIG for energy storage, electrocatalysis, water treatment, sensors reported literature. Additionally, has proposed ink formulation or incorporation into polymer matrices, further expand use non-carbon-based substrates applications which pristine cannot directly used. way, it is possible apply substrates, aiming at emerging wearable edible electronics. Thus, review will bring an overview developments, accordance European Green Deal, United Nations Sustainable Development Goals era internet-of-things, demands components principles efficiency production methods.

Язык: Английский

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Biodegradable Materials for Transient Organic Transistors

Advanced Functional Materials, Год журнала: 2022, Номер 33(6)

Опубликована: Дек. 9, 2022

Abstract Electronic devices that can physically disappear in a controlled manner without harmful by‐products unveil wide range of opportunities medical devices, environmental monitoring, and next‐generation consumer electronics. Their property transience is indispensable for mitigating the global problem electronic waste accumulation. Additionally, transient technologies are biocompatible be biologically resorbed great potential applications temporary implants, since it eliminates need expensive device recovery surgery. Transistors key building blocks modern electronics, their fabrication using organic materials beneficial due to low cost, unprecedented flexibility facile processing. This contribution reviews technological application biodegradable four major classes transistors, namely field‐effect transistors (OFETs), synaptic electrolyte‐gated OFETs, electrochemical transistors. The fundamental biodegradation mechanism discussed detail, followed by perspective various utilized as active semiconductors, dielectrics, electrolytes substrates types transistor devices. comprehensively discusses role all modern‐day highlighting unique properties allow biodegradable, eco‐friendly, sustainable

Язык: Английский

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Review of recent advances and sensing mechanisms in solid-state organic thin-film transistor (OTFT) sensors

Journal of Materials Chemistry C, Год журнала: 2024, Номер 12(16), С. 5654 - 5683

Опубликована: Янв. 1, 2024

Advances in processing of active layers organic thin-film transistor (OTFT)-based chemical and biological sensors have enabled significant developments their performance, achieving part-per-billion molar concentration limits detection.

Язык: Английский

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MOF‐Based Sustainable Memory Devices

Advanced Functional Materials, Год журнала: 2021, Номер 32(5)

Опубликована: Окт. 13, 2021

Abstract Data storage, processing, and communications are the backbone of digital world focus innovation efforts microelectronics industry. Recent raw material shortages, however, have revealed danger sourcing for At a time significant increase in demand data storage systems, it is urgent to consider sustainability resources used devices. By diluting inorganic elements an organic matrix, metal–organic frameworks (MOFs) substantial interest sustainable technologies. Moreover, they shown great potential as active materials electronic, optical, magnetic memory devices, paving way accessible, sustainable, recyclable microelectronic Based on number fundamental studies bistability MOFs, their scalability, recyclability, low energy consumption, MOFs highlighted new generation memristive Finally, considering “green” chemistry specific MOF, flexibility, well market mineral future development MOF‐based devices socio‐economic profits from utilization predicted.

Язык: Английский

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High‐Performance Bioelectronic Circuits Integrated on Biodegradable and Compostable Substrates with Fully Printed Mask‐Less Organic Electrochemical Transistors

Small, Год журнала: 2022, Номер 18(26)

Опубликована: Июнь 1, 2022

Abstract Organic electrochemical transistors (OECTs) rely on volumetric ion‐modulation of the electronic current to provide low‐voltage operation, large signal amplification, enhanced sensing capabilities, and seamless integration with biology. The majority OECT technologies require multistep photolithographic microfabrication methods glass or plastic substrates, which do not an ideal path toward ultralow cost ubiquitous sustainable electronics bioelectronics. At same time, development advanced bioelectronic circuits combining bio‐detection, local processing functionalities urgently demand for technology platforms a monolithic high‐performance iontronic sensors. Here, fully printed mask‐less OECTs fabricated thin‐film biodegradable compostable substrates are proposed. dispensing capillary printing used depositing both high‐ low‐viscosity materials. Fully unipolar inverter gain normalized supply voltage as high 136.6 V −1 , current‐driven sensors ion detection real‐time monitoring sensitivity up 506 mV dec integrated substrates. These universal building blocks top‐performance ever reported demonstrate effectiveness proposed approach can open opportunities next‐generation

Язык: Английский

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Hydrogel‐Based Artificial Synapses for Sustainable Neuromorphic Electronics

Advanced Materials, Год журнала: 2024, Номер 36(38)

Опубликована: Авг. 1, 2024

Hydrogels find widespread applications in biomedicine because of their outstanding biocompatibility, biodegradability, and tunable material properties. can be chemically functionalized or reinforced to respond physical chemical stimulation, which opens up new possibilities the emerging field intelligent bioelectronics. Here, state-of-the-art functional hydrogel-based transistors memristors is reviewed as potential artificial synapses. Within these systems, hydrogels serve semisolid dielectric electrolytes switching layers memristors. These synaptic devices with volatile non-volatile resistive show good adaptability external stimuli for short-term long-term memory effects, some are integrated into arrays neurons; although, there discrepancies performance efficacy. By comparing different respective properties, an outlook provided on a range biocompatible, environment-friendly, sustainable neuromorphic hardware. How energy-efficient information storage processing achieved using neural networks brain-inspired architecture computing described. The development synapses significantly impact fields bionics, biometrics, biosensing.

Язык: Английский

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Revolutionizing Papertronics: Advanced Green, Tunable, and Flexible Components and Circuits

Advanced Sustainable Systems, Год журнала: 2024, Номер 8(6)

Опубликована: Фев. 28, 2024

Abstract Papertronics introduce a sustainable, cost‐effective revolution in electronics, especially for the Internet of Things. This research overcomes traditional challenges paper's porosity, which has impeded electronic component fabrication and performance. A novel approach that harnesses natural capillary action, combined with hydrophobic wax patterning, to achieve precise vertical integration components is introduced. method marks significant departure from conventional surface deposition techniques. study demonstrates successful creation tunable resistors, capacitors, field‐effect transistors, embedded within single sheet paper. Contrary previous assumptions use paper, its rough porous texture as strategic advantage, facilitating intricate leveraged. Machine learning algorithms play an important role predicting enhancing performance these papertronic components. innovation facilitates development compact printed circuit boards increased density, enabling diverse analog digital circuits either or multi‐layer paper formats. The resulting systems exceed benchmarks, offering eco‐friendly disposal through biodegradability incineration. These breakthroughs establish papertronics feasible, alternative electronics industry, permitting widespread adoption continuous sustainable solutions.

Язык: Английский

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Photo-crosslinked polymer dielectrics enabling flexible organic transistor synapses with excellent linearity for neuromorphic applications

Chemical Engineering Journal, Год журнала: 2025, Номер unknown, С. 160538 - 160538

Опубликована: Фев. 1, 2025

Язык: Английский

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Surface Functionalization with (3-Glycidyloxypropyl)trimethoxysilane (GOPS) as an Alternative to Blending for Enhancing the Aqueous Stability and Electronic Performance of PEDOT:PSS Thin Films

ACS Applied Materials & Interfaces, Год журнала: 2023, Номер 15(47), С. 54711 - 54720

Опубликована: Ноя. 14, 2023

Organic mixed ionic-electronic conductors, such as poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS), are essential materials for the fabrication of bioelectronic devices due to their unique ability couple and transport ionic electronic charges. The growing interest in has led development organic electrochemical transistors (OECTs) that can operate aqueous solutions transduce signals biological origin into measurable signals. A common challenge with OECTs is maintaining stability performance PEDOT:PSS films operating under conditions. Although conventional approach blending dispersions a cross-linker (3-glycidyloxypropyl)trimethoxysilane (GOPS) helps ensure strong adhesion device substrates, it also impacts morphology thus electrical properties films, which leads significant reduction OECTs. In this study, we instead functionalize only surface substrates GOPS introduce silane monolayer before spin-coating dispersion on substrate. all cases, having blend increased metrics, three times higher conductivity, volumetric capacitance, mobility-capacitance product [μC*] value OECT devices, ultimately leading record 406 ± 39 F cm-1 V-1 s-1 amorphous PEDOT:PSS. This does not come at expense operational stability, both functionalization show similar when subjected pulsed gate bias stress, long-term cycling tests, aging over 150 days. Overall, study establishes novel using blended cross-linker, achieving high-performance conductors stable water bioelectronics.

Язык: Английский

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Green production of plant/collagen-based antibacterial polyvinyl alcohol (PVA) nanocomposite films

Sustainable Chemistry and Pharmacy, Год журнала: 2023, Номер 33, С. 101119 - 101119

Опубликована: Май 26, 2023

Язык: Английский

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