Journal of Materials Chemistry A,
Год журнала:
2023,
Номер
12(1), С. 128 - 143
Опубликована: Ноя. 20, 2023
Due
to
the
synergistic
effect
of
field
redistribution
and
Fermi
level's
moving,
an
ESD
31.07
J
cm
−3
with
η
80.03%
was
obtained
in
SZS,
which
is
best
performance
cellulose-based
dielectric
capacitors
authors'
knowledge.
The
rapid
rise
of
triboelectric
nanogenerators
(TENGs),
which
are
emerging
energy
conversion
devices
in
advanced
electronics
and
wearable
sensing
systems,
has
elevated
the
interest
high-performance
multifunctional
materials.
Among
them,
cellulosic
materials,
affording
high
efficiency,
biodegradability,
customizability,
becoming
a
new
front-runner.
inherently
low
dielectric
constant
limits
increase
surface
charge
density.
However,
owing
to
its
unique
structure
excellent
processability,
cellulose
shows
great
potential
for
modulation,
providing
strong
impetus
applications
era
Internet
Things
artificial
intelligence.
This
review
aims
provide
comprehensive
insights
into
fabrication
dielectric-enhanced
materials
via
modulation.
exceptional
advantages
research
progress
highlighted.
effects
constant,
polarization,
percolation
threshold
on
density
systematically
investigated,
theoretical
basis
Typical
characterization
methods
introduced,
their
technical
characteristics
analyzed.
Furthermore,
performance
enhancements
endowed
by
including
more
efficient
harvesting,
electronics,
impedance
matching
material
strategies,
introduced.
Finally,
challenges
future
opportunities
modulation
summarized.
Advanced Materials,
Год журнала:
2024,
Номер
36(16)
Опубликована: Янв. 6, 2024
Abstract
Electronic
waste
is
a
growing
threat
to
the
global
environment
and
human
health,
raising
particular
concerns.
Triboelectric
devices
synthesized
from
sustainable
degradable
materials
are
promising
electronic
alternative,
but
mechanical
mismatch
at
interface
between
polymer
substrate
electrodes
remains
unresolved
in
practical
applications.
This
study
uses
sulfhydryl
silanization
reaction
chemical
selectivity
site
specificity
of
thiol–disulfide
exchange
dynamic
covalent
chemistry
prepare
tough
monolithic‐integrated
triboelectric
bioplastic.
The
stress
dissipated
by
bond
adaptation
interaction,
which
makes
dielectric
layer
conductive
have
good
adhesion
effect
(220.55
kPa).
interfacial
interlocking
with
gives
bioplastic
excellent
tensile
strength
(87.4
MPa)
fracture
toughness
(33.3
MJ
m
−3
).
Even
when
subjected
tension
force
10
000
times
its
weight,
it
still
maintains
stable
output
no
visible
cracks.
provides
new
insights
into
design
reliable
environmentally
friendly
self‐powered
devices,
significant
for
development
flexible
wearable
electronics.
Nano-Micro Letters,
Год журнала:
2024,
Номер
16(1)
Опубликована: Апрель 9, 2024
Rapid
advancements
in
flexible
electronics
technology
propel
soft
tactile
sensing
devices
toward
high-level
biointegration,
even
attaining
perception
capabilities
surpassing
human
skin.
However,
the
inherent
mechanical
mismatch
resulting
from
deficient
biomimetic
properties
of
materials
poses
a
challenge
to
application
wearable
human-machine
interaction.
Inspired
by
innate
biphasic
structure
subcutaneous
tissue,
this
study
discloses
skin-compliant
iontronic
triboelectric
gel
via
phase
separation
induced
competitive
hydrogen
bonding.
Solvent-nonsolvent
interactions
are
used
construct
bonding
systems
trigger
separation,
and
soft-hard
alternating
phase-locked
confers
with
Young's
modulus
(6.8-281.9
kPa)
high
tensile
(880%)
compatible
The
abundance
reactive
hydroxyl
groups
gives
excellent
tribopositive
self-adhesive
(peel
strength
>
70
N
m
Nano-Micro Letters,
Год журнала:
2024,
Номер
16(1)
Опубликована: Май 31, 2024
Abstract
The
rapid
development
of
the
Internet
Things
and
artificial
intelligence
technologies
has
increased
need
for
wearable,
portable,
self-powered
flexible
sensing
devices.
Triboelectric
nanogenerators
(TENGs)
based
on
gel
materials
(with
excellent
conductivity,
mechanical
tunability,
environmental
adaptability,
biocompatibility)
are
considered
an
advanced
approach
developing
a
new
generation
sensors.
This
review
comprehensively
summarizes
recent
advances
in
gel-based
TENGs
sensors,
covering
their
principles,
properties,
applications.
Based
requirements
working
mechanism
characteristic
advantages
gels
introduced.
Design
strategies
performance
optimization
hydrogel-,
organogel-,
aerogel-based
systematically
summarized.
In
addition,
applications
human
motion
sensing,
tactile
health
monitoring,
human–machine
interaction,
other
related
fields
Finally,
challenges
discussed,
feasible
proposed
to
guide
future
research.
Nano Letters,
Год журнала:
2024,
Номер
24(23), С. 7125 - 7133
Опубликована: Май 29, 2024
Wearable
sensors
are
experiencing
vibrant
growth
in
the
fields
of
health
monitoring
systems
and
human
motion
detection,
with
comfort
becoming
a
significant
research
direction
for
wearable
sensing
devices.
However,
weak
moisture-wicking
capability
sensor
materials
leads
to
liquid
retention,
severely
restricting
sensors.
This
study
employs
pattern-guided
alignment
strategy
construct
microhill
arrays,
endowing
triboelectric
directional
capability.
Within
2.25
s,
can
quickly
directionally
remove
droplets,
driven
by
Laplace
pressure
differences
wettability
gradient.
The
exhibit
excellent
performance,
enabling
rapid
response/recovery
(29.1/37.0
ms),
thereby
achieving
real-time
online
respiration
movement
states.
work
addresses
long-standing
challenge
insufficient
driving
force
flexible
electronic
materials,
holding
implications
enhancing
application
potential
skin
Nano Letters,
Год журнала:
2024,
Номер
24(25), С. 7809 - 7818
Опубликована: Июнь 14, 2024
Noncontact
sensing
technology
serves
as
a
pivotal
medium
for
seamless
data
acquisition
and
intelligent
perception
in
the
era
of
Internet
Things
(IoT),
bringing
innovative
interactive
experiences
to
wearable
human–machine
interaction
networks.
However,
pervasive
limitations
current
noncontact
devices
posed
by
harsh
environmental
conditions
hinder
precision
stability
signals.
In
this
study,
triboelectric
nanopaper
prepared
phase-directed
assembly
strategy
is
presented,
which
possesses
low
charge
transfer
mobility
(1618
cm2
V–1
s–1)
exceptional
high-temperature
stability.
Wearable
self-powered
sensors
constructed
from
operate
stably
under
high
temperatures
(200
°C).
Furthermore,
temperature
warning
system
workers
hazardous
environments
demonstrated,
capable
nonintrusively
identifying
harmful
thermal
stimuli
detecting
motion
status.
This
research
not
only
establishes
technological
foundation
accurate
stable
but
also
promotes
sustainable
development
IoT
extreme
environments.