
Carbon Capture Science & Technology, Год журнала: 2024, Номер 13, С. 100313 - 100313
Опубликована: Сен. 26, 2024
Язык: Английский
Carbon Capture Science & Technology, Год журнала: 2024, Номер 13, С. 100313 - 100313
Опубликована: Сен. 26, 2024
Язык: Английский
Advanced Science, Год журнала: 2024, Номер 11(30)
Опубликована: Июнь 13, 2024
Photocatalytic CO
Язык: Английский
Процитировано
19Chemical Reviews, Год журнала: 2024, Номер 124(21), С. 12006 - 12085
Опубликована: Окт. 31, 2024
Catalytic COx (CO and CO2) hydrogenation to valued chemicals is one of the promising approaches address challenges in energy, environment, climate change. H2O an inevitable side product these reactions, where its existence effect are often ignored. In fact, significantly influences catalytic active centers, reaction mechanism, performance, preventing us from a definitive deep understanding on structure-performance relationship authentic catalysts. It necessary, although challenging, clarify provide practical strategies tune concentration distribution optimize influence. this review, we focus how induces structural evolution catalysts assists processes, as well efforts understand underlying mechanism. We summarize discuss some representative tuning for realizing rapid removal or local enrichment around catalysts, along with brief techno-economic analysis life cycle assessment. These fundamental understandings further extended reactions CO CO2 reduction under external field (light, electricity, plasma). also present suggestions prospects deciphering controlling applications.
Язык: Английский
Процитировано
13ACS Catalysis, Год журнала: 2025, Номер unknown, С. 3558 - 3569
Опубликована: Фев. 12, 2025
Язык: Английский
Процитировано
2Journal of Colloid and Interface Science, Год журнала: 2024, Номер 677, С. 1095 - 1106
Опубликована: Авг. 19, 2024
Язык: Английский
Процитировано
9Green Energy & Environment, Год журнала: 2025, Номер unknown
Опубликована: Янв. 1, 2025
Язык: Английский
Процитировано
1Carbon Capture Science & Technology, Год журнала: 2025, Номер unknown, С. 100377 - 100377
Опубликована: Фев. 1, 2025
Язык: Английский
Процитировано
1Nano Energy, Год журнала: 2024, Номер 133, С. 110460 - 110460
Опубликована: Ноя. 9, 2024
Язык: Английский
Процитировано
6Chemical Engineering Journal, Год журнала: 2024, Номер 501, С. 157513 - 157513
Опубликована: Ноя. 8, 2024
Язык: Английский
Процитировано
5Journal of environmental chemical engineering, Год журнала: 2024, Номер unknown, С. 114986 - 114986
Опубликована: Ноя. 1, 2024
Язык: Английский
Процитировано
3ACS Applied Materials & Interfaces, Год журнала: 2025, Номер unknown
Опубликована: Янв. 8, 2025
The replacement of the thermodynamically unfavorable anodic oxygen evolution reaction (OER) with a more favorable organic oxidation reaction, such as benzylamine, has garnered significant interest in hybrid water electrolyzer cells. This approach promises production value-added chemicals alongside hydrogen fuel generation, improving overall energy efficiency. However, achieving high current density for benzylamine without interference from OER remains challenge, limiting practical efficiency cell. In this study, we investigated room temperature method sulfur introduction VNi-layered double hydroxide (LDH) catalyst and its application electrocatalytic oxidation. S-introduction VNi-LDH was found to modulate electronic states nickel vanadium, increasing number active sites, electrochemical surface area, charge transfer properties. resulting S-VNi-LDH achieved 400 mA cm–2 at only 1.39 V vs RHE potential oxidation, avoiding evolution. demonstrated 100% selectivity (Faradaic Efficiency = 98.6%) conversion into benzonitrile within 2.5 h reaction. two-electrode electrolysis system, cell voltage 1.50 when substituted showed consumption 4.67 kWh/m3 H2 1.31 during indicating exceptional stability over five cycles, maintaining 98.6 ± 0.4% FE consistent voltage. also oxidized various amines, including benzylamines secondary (95–97%) faradaic (85.8–98%). study presents an eco-friendly, room-temperature S-doping VNi-LDH, which out performed reported catalysts literature.
Язык: Английский
Процитировано
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