G-Quadruplex DNAzyme-Based Biocatalysis Combined with an Intelligent Electromagnetic-Actuated Microfluidic Chip for Tetracycline Detection DOI
Li Wang, Wanwan Wang, Shumin Zhang

и другие.

Journal of Agricultural and Food Chemistry, Год журнала: 2024, Номер 73(2), С. 1598 - 1607

Опубликована: Дек. 31, 2024

In this study, we present an intelligent electromagnetic-actuated microfluidic chip integrated with a G-quadruplex DNAzyme-based biocatalysis platform for rapid and sensitive tetracycline (TC) detection. sensing system, TC significantly quenches fluorescent magnetic carbon dots (M-CDs) via the internal filtration effect dynamic quenching (the excitation emission wavelength at 350 440 nm, respectively). Then, on M-CDs-Aptamer is exposed bound hemin to form hemin-G-quadruplex DNAzyme, catalyzing conversion of 3,3',5,5'-tetramethylbenzidine produce blue color. This enables fluorescence/colorimetric detection TC. Importantly, automatic electromagnet-integrated was designed control shuttling materials in each function slot according programmed sequence. Under optimal conditions, limits fluorescence colorimetric methods were 11 43 μmol/L, respectively. The results tilapia (Oreochromis nilotica) comparable those traditional high-performance liquid chromatography. offers excellent performance determination potential portable, trace pollutants food environment.

Язык: Английский

Unsupervised Learning‐Assisted Acoustic‐Driven Nano‐Lens Holography for the Ultrasensitive and Amplification‐Free Detection of Viable Bacteria DOI Creative Commons
Yang Zhou, Junpeng Zhao, Junping Wen

и другие.

Advanced Science, Год журнала: 2024, Номер 12(2)

Опубликована: Ноя. 22, 2024

Abstract Bacterial infection is a crucial factor resulting in public health issues worldwide, often triggering epidemics and even fatalities. The accurate, rapid, convenient detection of viable bacteria an effective method for reducing infections illness outbreaks. Here, unsupervised learning–assisted surface acoustic wave–interdigital transducer‐driven nano‐lens holography biosensing platform developed the ultrasensitive amplification‐free bacteria. monitoring device integrated with effect can achieve holographic imaging polystyrene microsphere probes ultra‐wide field view (∽28.28 mm 2 ), sensitivity limit as low 99 nm. A lightweight learning hologram processing algorithm considerably reduces training time computing hardware requirements, without requiring datasets manual labels. By combining phage–mediated bacterial DNA extraction enhanced CRISPR–Cas12a systems, this strategy successfully achieves Salmonella various real samples, demonstrating accuracy validated qPCR benchmark method. This approach has cost (∽$500) rapid (∽1 h) highly sensitive (∽38 CFU mL −1 allowing emerging powerful tool food safety inspection clinical diagnosis.

Язык: Английский

Процитировано

7

Weight Differences-Based Multi-level Signal Profiling for Homogeneous and Ultrasensitive Intelligent Bioassays DOI

Weiqi Zhao,

Minjie Han,

Xiaolin Huang

и другие.

ACS Nano, Год журнала: 2025, Номер unknown

Опубликована: Март 10, 2025

Current high-sensitivity immunoassay protocols often involve complex signal generation designs or rely on sophisticated signal-loading and readout devices, making it challenging to strike a balance between sensitivity ease of use. In this study, we propose homogeneous-based intelligent analysis strategy called Mata, which uses weight quantify basic immune signals through subunits. We perform nanomagnetic labeling target capture events micrometer-scale polystyrene subunits, enabling magnetically regulated kinetic expression. Signal subunits are classified the multi-level classifier in synergy with developed deep learning recognition models. Subsequently, quantified achieve ultra-high sensitivity. Mata achieves detection 0.61 pg/mL 20 min for interleukin-6 detection, demonstrating comparable conventional digital immunoassays over 22-fold that chemiluminescence reducing time by more than 70%. The entire process relies homogeneous reaction can be performed using standard bright-field optical imaging. This balances high convenient operation has few hardware requirements, presenting promising solution wide accessibility.

Язык: Английский

Процитировано

0

Unraveling the potential of bioengineered microbiome-based strategies to enhance cancer immunotherapy DOI
Muhammad Hamza, Shuai Wang, Yike Liu

и другие.

Microbiological Research, Год журнала: 2025, Номер unknown, С. 128156 - 128156

Опубликована: Март 1, 2025

Язык: Английский

Процитировано

0

Double-emulsion droplet digital CRISPR/Cas12a for amplification-free, absolute quantification of nucleic acids at attomole levels DOI Creative Commons
Yang Zhang, Hangrui Liu, Shi‐Yang Tang

и другие.

Chemical Engineering Journal, Год журнала: 2025, Номер unknown, С. 162098 - 162098

Опубликована: Апрель 1, 2025

Процитировано

0

Deep-Learning-Assisted Microfluidic Immunoassay via Smartphone-Based Imaging Transcoding System for On-Site and Multiplexed Biosensing DOI
Peng Lü, Yang Zhou,

Xiaohu Niu

и другие.

Nano Letters, Год журнала: 2025, Номер unknown

Опубликована: Апрель 9, 2025

Point-of-care testing (POCT) with multiplexed capability, ultrahigh sensitivity, affordable smart devices, and user-friendly operation is critically needed for clinical diagnostics food safety. This study presents a deep-learning-assisted microfluidic immunoassay platform that uses smartphone-based imaging transcoding system, polystyrene microsphere-based encoding, artificial-intelligence-assisted decoding. Microspheres of varying sizes act as multiprobes, their quantities correlating to target concentrations after an immunoreaction separation-filtration within the chip. A smartphone intelligent decoding software captures images multiprobes from chip performs classification, counting, concentration calculations. The "encoding-decoding" strategy integrated design allow these processes be completed in simple steps, eliminating need additional immunomagnetic separation. As proof concept, this successfully detected multiple respiratory viruses antibiotics various real samples high sensitivity 30 min, demonstrating great potential smart, universal toolkit next-generation POCT applications.

Язык: Английский

Процитировано

0

crRNA array-mediated CRISPR/Cas12a coupling with dual RPA for highly sensitive detection of Streptomyces aureofaciens Tü117 from hypertension with multi-signal output DOI
Tingting Zhou,

Gongle Shen,

Zhong Lian

и другие.

Biosensors and Bioelectronics, Год журнала: 2025, Номер 282, С. 117493 - 117493

Опубликована: Апрель 17, 2025

Язык: Английский

Процитировано

0

Detection of Salmonella in food by SG4MB/SRCA based colorimetric biosensor DOI

Xiaoxuan Wang,

Yunzhe Zhang,

Hui Di

и другие.

Journal of Food Composition and Analysis, Год журнала: 2025, Номер unknown, С. 107677 - 107677

Опубликована: Апрель 1, 2025

Язык: Английский

Процитировано

0

G-Quadruplex DNAzyme-Based Biocatalysis Combined with an Intelligent Electromagnetic-Actuated Microfluidic Chip for Tetracycline Detection DOI
Li Wang, Wanwan Wang, Shumin Zhang

и другие.

Journal of Agricultural and Food Chemistry, Год журнала: 2024, Номер 73(2), С. 1598 - 1607

Опубликована: Дек. 31, 2024

In this study, we present an intelligent electromagnetic-actuated microfluidic chip integrated with a G-quadruplex DNAzyme-based biocatalysis platform for rapid and sensitive tetracycline (TC) detection. sensing system, TC significantly quenches fluorescent magnetic carbon dots (M-CDs) via the internal filtration effect dynamic quenching (the excitation emission wavelength at 350 440 nm, respectively). Then, on M-CDs-Aptamer is exposed bound hemin to form hemin-G-quadruplex DNAzyme, catalyzing conversion of 3,3',5,5'-tetramethylbenzidine produce blue color. This enables fluorescence/colorimetric detection TC. Importantly, automatic electromagnet-integrated was designed control shuttling materials in each function slot according programmed sequence. Under optimal conditions, limits fluorescence colorimetric methods were 11 43 μmol/L, respectively. The results tilapia (Oreochromis nilotica) comparable those traditional high-performance liquid chromatography. offers excellent performance determination potential portable, trace pollutants food environment.

Язык: Английский

Процитировано

1