Journal of Materials Chemistry A,
Год журнала:
2024,
Номер
unknown
Опубликована: Дек. 17, 2024
In
this
work,
a
multifunctional,
high-conductivity,
flexible,
anti-freezing
and
self-adhesive
double-network
hydrogel
with
3D
interpenetrating
framework
was
designed
for
energy
harvesting
storage
self-powered
round-the-clock
sensing.
Abstract
The
rapid
advancement
in
attractive
platforms
such
as
biomedicine
and
human‐machine
interaction
has
generated
urgent
demands
for
intelligent
materials
with
high
strength,
flexibility,
self‐healing
capabilities.
However,
existing
ability
are
challenged
by
a
trade‐off
between
low
elastic
modulus,
healing
due
to
the
inherent
strength
of
noncovalent
bonding.
Here,
drawing
inspiration
from
human
fibroblasts,
monomer
trapping
synthesis
strategy
is
presented
based
on
dissociation
reconfiguration
amphiphilic
ionic
restrictors
(7000‐times
volume
trapping)
develop
eutectogel.
Benefiting
nanoconfinement
dynamic
interfacial
interactions,
molecular
chain
backbone
formed
confined
domains
mechanically
reinforced
while
preserving
soft
movement
resulting
eutectogels
demonstrate
superior
mechanical
properties
(1799%
2753%
higher
tensile
toughness
than
pure
polymerized
deep
eutectic
solvent),
excellent
efficiency
(>90%),
tangential
modulus
(0.367
MPa
during
working
stage),
sensitively
monitor
activities.
This
poised
offer
new
perspective
developing
wearable
electronics
tailored
body
motion.
ACS Applied Materials & Interfaces,
Год журнала:
2025,
Номер
17(6), С. 9115 - 9124
Опубликована: Янв. 30, 2025
Wearable
temperature-sensitive
electronic
skin
enables
robots
to
rapidly
detect
environmental
changes
and
respond
intelligently,
thereby
reducing
temperature-related
mechanical
failures.
Additionally,
this
can
measure
record
the
temperature
of
external
objects,
broadening
its
potential
applications
in
medical
field.
In
study,
we
designed
a
thermally
sensitive
artificial
ionic
using
liquids
(ILs)
as
solvents
carbon
nanotubes
(CNTs)
conductive
fillers.
The
incorporation
ILs
into
polymer
network
enhances
thermal
stability,
while
CNTs
establish
dual
conduction
pathways
(CNTs-CNTs
CNTs-polymer
chain
segments),
leading
rapid
response
times
only
16
s.
initiation
IL
dissociation
at
elevated
temperatures
boosts
carrier
density,
resulting
substantial
improvement
sensitivity
(5%/°C).
Furthermore,
displays
remarkable
self-healing
properties
(90%),
extending
lifespan
practical
applications.
This
kind
stably
sense
wearer's
body
provide
an
ideal
long-term
stable
new
functional
material
for
development
human
such
robots.
Despite
the
rapid
development
of
stretchable
electronic
devices
for
various
applications
in
biomedicine
and
healthcare,
coupling
between
multiple
input
signals
remains
an
obstacle
multimodal
sensing
before
use
practical
environments.
This
work
introduces
a
fully
integrated
stretchable,
rechargeable,
hybrid
device
that
combines
decoupled
sensors
with
flexible
wireless
powering
transmitting
module
emotion
recognition.
Through
optimized
structural
design
material
selection,
can
provide
continuous
real-time
monitoring
biaxial
strain,
temperature,
humidity,
heart
rate,
SpO2
levels.
With
stacked
bilayer
both
circuit,
rechargeable
system
showcases
reduced
footprint
improved
comfort.
A
neural
network
model
is
also
demonstrated
to
allow
high-precision
facial
expression
By
measured
data
mobile
cloud,
healthcare
professionals
evaluate
psychological
health
emotional
support
through
telemedicine
when
needed.
ACS Applied Materials & Interfaces,
Год журнала:
2025,
Номер
unknown
Опубликована: Март 27, 2025
Fabric
electrodes
are
an
important
part
of
long-term
medical-health-monitoring
garments,
but
sweat
corrosion
can
greatly
affect
their
longevity
and
stability.
In
this
study,
the
metal
fabric
biopotential
sensor
was
chemically
modified
with
3-mercaptopropyltrimethoxysilane
(MPTS).
Ag/AgCl
formed
on
electrode
surface
by
constant
voltage
deposition.
Ag/AgCl/3-Mercaptopropyltrimethoxysilane/silver-plated
nylon
(Ag/AgCl/MPTS/SPNE),
Ag/AgCl/3-mercaptopropyltrimethoxysilane/silver-plated
copper
wire
(Ag/AgCl/MPTS/SPCWE),
Ag/AgCl/3-mercaptopropyltrimethoxysilane/sterling
silver
yarn
(Ag/AgCl/MPTS/SSYE)
were
prepared.
Molecular
dynamics
(MD)
simulations
using
Forcite
performed
to
investigate
anticorrosion
mechanism
MPTS.
The
effects
MPTS
dip-coating
time
chlorination
parameters
electrochemical
properties
investigated.
resistance
tested
in
simulated
NaCl
solutions.
We
analyzed
suitability
softness
test,
abrasion
washing
motion
noise
test.
Ag/AgCl/MPTS/SSYE
provides
optimal
resistance,
comfort,
electrical
properties.
It
be
used
for
wearable
applications
such
as
electrocardiogram
(ECG)
signals,
electromyogram
(EMG)
neuromuscular
stimulation
(NMES).
Journal of Materials Chemistry C,
Год журнала:
2025,
Номер
unknown
Опубликована: Янв. 1, 2025
Flexible
conductive
elastomer
materials
are
promising
for
applications
in
wearable,
flexible
sensor
devices,
human
motion
monitoring,
and
other
fields.