Batteries,
Год журнала:
2023,
Номер
9(4), С. 228 - 228
Опубликована: Апрель 17, 2023
Solid-state
lithium
batteries
have
attracted
considerable
research
attention
for
their
potential
advantages
over
conventional
liquid
electrolyte
batteries.
The
discovery
of
solid-state
electrolytes
(SSEs)
is
still
undergoing
to
solve
the
remaining
challenges,
and
machine
learning
(ML)
approaches
could
potentially
accelerate
process
significantly.
This
review
introduces
common
ML
techniques
employed
in
materials
an
overview
applications
SSE
discovery,
with
perspectives
on
key
issues
future
outlooks.
Nano-Micro Letters,
Год журнала:
2024,
Номер
16(1)
Опубликована: Фев. 21, 2024
Polymer
solid-state
lithium
batteries
(SSLB)
are
regarded
as
a
promising
energy
storage
technology
to
meet
growing
demand
due
their
high
density
and
safety.
Ion
conductivity,
interface
stability
battery
assembly
process
still
the
main
challenges
hurdle
commercialization
of
SSLB.
As
component
SSLB,
poly(1,3-dioxolane)
(PDOL)-based
solid
polymer
electrolytes
polymerized
in-situ
becoming
candidate
electrolyte,
for
ion
conductivity
at
room
temperature,
good
electrochemical
performances,
simple
process.
This
review
analyzes
opportunities
PDOL
toward
practical
application
The
focuses
include
exploring
polymerization
mechanism
DOL,
performance
composite
electrolytes,
PDOL.
Furthermore,
we
provide
perspective
on
future
research
directions
that
need
be
emphasized
PDOL-based
in
exploration
these
schemes
facilitates
comprehensive
profound
understanding
electrolyte
provides
new
ideas
boost
them
batteries.
Advanced Energy Materials,
Год журнала:
2023,
Номер
13(30)
Опубликована: Июнь 25, 2023
Abstract
Although
there
are
various
strategies
for
solid‐state
polymer
lithium
batteries
(SSPLBs)
manufacturing,
the
most
promising
is
in
situ
polymerization
process.
The
process
inherits
good
liquid
electrolyte/electrode
interfacial
contact
and
compatible
with
existing
lithium‐ion
manufacturing
processes,
making
it
easy
to
achieve
scale‐up
production.
However,
of
current
studies
on
based
lab‐level
coin
cells,
while
practical
pouch
cells
much
less
studied.
There
a
huge
difference
between
SSPLBs
SSPLBs.
Here,
as
complement
reports
reviews,
systematic
review
challenges
design
principles
fabricating
provided
enable
comprehensive
understanding
strategic
guidance
applications.
This
thoroughly
discusses
recent
advances
regarding
fabrication
using
presents
future
outlook
by
processes.
Furthermore,
critical
issues
electrode
materials
highlighted
during
process,
an
attempt
made
call
more
attention
performance
Advanced Functional Materials,
Год журнала:
2023,
Номер
33(49)
Опубликована: Авг. 3, 2023
Abstract
In
the
development
of
all‐solid‐state
lithium
batteries
(ASSLB),
progress
is
made
with
solid‐state
electrolytes;
however,
challenges
regarding
compatibility
and
stability
still
exist
solid
electrodes.
These
issues
result
in
a
low
battery
capacity
short
cycle
life,
which
limit
commercial
application
ASSLBs.
This
review
summarizes
recent
research
on
electrodes
ASSLBs
including
solid–solid
interface
phenomena
such
as
between
electrode
materials
electrolytes.
The
mechanical
problems
electrodes,
fracture,
brittleness,
deformation
materials,
are
also
discussed,
corresponding
methods
to
measure
stress
provided.
addition,
strategies
for
mitigating
stress‐related
examined.
Finally,
fabrication
process
introduced
their
future
developments,
exploration
new
design
more
intelligent
structures,
proposed.
Advanced Materials,
Год журнала:
2024,
Номер
36(21)
Опубликована: Фев. 19, 2024
Abstract
All‐solid‐state
lithium
batteries
(ASSLBs)
face
critical
challenges
of
low
cathode
loading
and
poor
rate
performances,
which
handicaps
their
energy/power
densities.
The
widely‐accepted
aim
high
ionic
conductivity
interfacial
resistance
seems
insufficient
to
overcome
these
challenges.
Here,
it
is
revealed
that
an
efficient
ion
percolating
network
in
the
exerts
a
more
influence
on
electrochemical
performance
ASSLBs.
By
constructing
vertical
alignment
Li
0.35
La
0.55
TiO
3
nanowires
(LLTO
NWs)
solid‐state
through
magnetic
manipulation,
increases
twice
compared
with
consisted
randomly
distributed
LLTO
NWs.
all‐solid‐state
LiFePO
4
/Li
cells
using
poly(ethylene
oxide)
as
electrolyte
able
deliver
capacities
151
mAh
g
−1
(2
C)
100
(5
at
60
°C,
room‐temperature
capacity
108
can
be
achieved
charging
2
C.
Furthermore,
cell
reach
areal
cm
−2
even
practical
LFP
20
mg
.
universality
this
strategy
also
presented
showing
demonstration
LiNi
0.8
Co
0.1
Mn
O
cathodes.
This
work
offers
new
pathways
for
designing
ASSLBs
improved
Chemical Reviews,
Год журнала:
2025,
Номер
unknown
Опубликована: Фев. 4, 2025
Solid-state
batteries
(SSBs)
could
offer
improved
energy
density
and
safety,
but
the
evolution
degradation
of
electrode
materials
interfaces
within
SSBs
are
distinct
from
conventional
with
liquid
electrolytes
represent
a
barrier
to
performance
improvement.
Over
past
decade,
variety
imaging,
scattering,
spectroscopic
characterization
methods
has
been
developed
or
used
for
characterizing
unique
aspects
in
SSBs.
These
efforts
have
yielded
new
understanding
behavior
lithium
metal
anodes,
alloy
composite
cathodes,
these
various
solid-state
(SSEs).
This
review
provides
comprehensive
overview
strategies
applied
SSBs,
it
presents
mechanistic
SSB
that
derived
methods.
knowledge
critical
advancing
technology
will
continue
guide
engineering
toward
practical
performance.
Energy & Environmental Science,
Год журнала:
2023,
Номер
17(1), С. 344 - 353
Опубликована: Ноя. 22, 2023
We
construct
an
efficient
Li
+
transport
network
in
a
high
loading
cathode
using
carbon
coated
1.4
Al
0.4
Ti
1.6
(PO
4
)
3
nanowires,
which
has
strong
adsorption
for
[Li(DMF)
x
]
of
PVDF-based
SPEs
to
promote
its
uniform
diffusion
and
stability
cathode.