Synergistic Interfacial Dipole and π-Conjugation Effects Enable Efficient Tin Perovskite Solar Cells DOI

Feng Yang,

Kun Wang, Yang Yang

и другие.

Nano Letters, Год журнала: 2025, Номер unknown

Опубликована: Март 31, 2025

Tin perovskites are considered promising candidates for realizing high-performance, lead-free perovskite solar cells (PSCs). Despite prominent progress made through bulk optimization, unsatisfactory interfaces between tin and charge transport layers critical obstacles to boosting device performance. Herein, we address this issue by introducing piperazine dihydroiodide (PDI) ferrocene (Fc) at the interface of perovskite/C60 synergistically improve interfacial transport. Specifically, PD+ interacts with formamidinium ions (FA+) form an dipole, Fc establishes π-π conjugation C60. These effects significantly electron extraction reduce energy losses. As a result, efficiency PSCs is remarkably improved from 10.62% 13.65%, accompanied enhanced stability. This work highlights importance modulation in toward efficient eco-friendly photovoltaics.

Язык: Английский

Key degradation mechanisms of perovskite solar cells and strategies for enhanced stability: issues and prospects DOI Creative Commons
Md. Helal Miah, Md. Bulu Rahman, Mohammad Nur‐E‐Alam

и другие.

RSC Advances, Год журнала: 2025, Номер 15(1), С. 628 - 654

Опубликована: Янв. 1, 2025

Insights into the factors and mechanisms of degradation, along with potential solutions.

Язык: Английский

Процитировано

2

Isomerizing Passivators in Perovskite Solar Cells: The Impact of Molecular Spatial Configuration DOI
Fazheng Qiu, Jiayi Sun, Haoliang Cheng

и другие.

ACS Materials Letters, Год журнала: 2025, Номер unknown, С. 544 - 552

Опубликована: Янв. 9, 2025

Язык: Английский

Процитировано

1

Fluorine-substituted bifunctional molecules for enhanced perovskite solar cell performance DOI

Murali Ravi,

Mengde Zhai,

Ziyang Xia

и другие.

Chemical Engineering Journal, Год журнала: 2025, Номер unknown, С. 159876 - 159876

Опубликована: Янв. 1, 2025

Язык: Английский

Процитировано

1

Bilayer interfacial engineering with PEAI/OAI for synergistic defect passivation in high-performance perovskite solar cells DOI

Chentai Cao,

Yuli Tao,

Quan Yang

и другие.

Journal of Semiconductors, Год журнала: 2025, Номер 46(5), С. 052805 - 052805

Опубликована: Май 1, 2025

Abstract Interfacial defects and environmental instability at perovskite surfaces pose significant challenges for inverted solar cells (PSCs). Surface post-treatment strategies have emerged as a viable approach to improve film quality passivate defects. Although organic molecules can both grain boundaries via hydrogen or covalent bonding, their limited adsorption specificity often results in incomplete defect neutralization. In this work, we introduce bilayer passivation employing phenethylammonium iodide (PEAI) n-octylammonium (OAI) concurrently mitigate non-radiative recombination stability. PEAI passivates undercoordinated Pb 2+ surfaces, effectively eliminating deep-level traps suppressing losses. Meanwhile, OAI forms hydrophobic barrier on the surface through its long alkyl chains, inhibiting moisture penetration without compromising interfacial charge transport. As result, exhibits significantly enhanced optoelectronic performance stability, achieving champion power conversion efficiency (PCE) of 24.48%.

Язык: Английский

Процитировано

1

Tailoring Organic Cation Structures in DJ 2D Perovskite: Impacts on Performance of 2D/3D Heterojunction Perovskite Solar Cells DOI
Xiaobo Zhang, Wencai Zhou, Yongcai He

и другие.

Materials Today Communications, Год журнала: 2025, Номер unknown, С. 111842 - 111842

Опубликована: Фев. 1, 2025

Язык: Английский

Процитировано

0

Synergistic Interfacial Dipole and π-Conjugation Effects Enable Efficient Tin Perovskite Solar Cells DOI

Feng Yang,

Kun Wang, Yang Yang

и другие.

Nano Letters, Год журнала: 2025, Номер unknown

Опубликована: Март 31, 2025

Tin perovskites are considered promising candidates for realizing high-performance, lead-free perovskite solar cells (PSCs). Despite prominent progress made through bulk optimization, unsatisfactory interfaces between tin and charge transport layers critical obstacles to boosting device performance. Herein, we address this issue by introducing piperazine dihydroiodide (PDI) ferrocene (Fc) at the interface of perovskite/C60 synergistically improve interfacial transport. Specifically, PD+ interacts with formamidinium ions (FA+) form an dipole, Fc establishes π-π conjugation C60. These effects significantly electron extraction reduce energy losses. As a result, efficiency PSCs is remarkably improved from 10.62% 13.65%, accompanied enhanced stability. This work highlights importance modulation in toward efficient eco-friendly photovoltaics.

Язык: Английский

Процитировано

0