How to Deal with Charge in the Ranking of Lewis Acidity: Critical Evaluation of an Extensive Set of Cationic Lewis Acids DOI Creative Commons
Philipp Erdmann, Manuel Schmitt, Lukas M. Sigmund

и другие.

Angewandte Chemie, Год журнала: 2024, Номер 136(22)

Опубликована: Март 13, 2024

Abstract The quantification of Lewis acidity is fundamental and applied importance in chemistry. However, if neutral charged acids are compared, a coherent ranking has been elusive, severe uncertainties were accepted. With this study, we present systematic computational analysis base affinities 784 mono‐, di‐ tricationic their comparison with 149 representative acids. Evaluating vacuum fluoride ion (FIA) reveals charge‐caused clustering that prohibits any meaningful ranking. Instead, solvation‐corrected FIA solv identified as metric overcomes charge sensitivity balanced manner, allowing for evaluation across varying states. Analyzing the impact molecular volume on solvation‐induced damping provides rationales trends guidelines choice or design cationic condensed phase. Exploring alternative scales, explicit counteranion effects, selected experimental case studies reaffirms advantages most versatile practical approach quantitative general (thermodynamic) acidity.

Язык: Английский

How to Deal with Charge in the Ranking of Lewis Acidity: Critical Evaluation of an Extensive Set of Cationic Lewis Acids DOI Creative Commons
Philipp Erdmann, Manuel Schmitt, Lukas M. Sigmund

и другие.

Angewandte Chemie International Edition, Год журнала: 2024, Номер 63(22)

Опубликована: Март 13, 2024

The quantification of Lewis acidity is fundamental and applied importance in chemistry. However, if neutral charged acids are compared, a coherent ranking has been elusive, severe uncertainties were accepted. With this study, we present systematic computational analysis base affinities 784 mono-, di- tricationic their comparison with 149 representative acids. Evaluating vacuum fluoride ion (FIA) reveals charge-caused clustering that prohibits any meaningful ranking. Instead, solvation-corrected FIA

Язык: Английский

Процитировано

12

Recent advances in bismuth oxyfluoride-based photocatalysts for energy and environmental remediation DOI
Vinoth Kumar Selvaraj, Alagarsamy Pandikumar

Materials Today Chemistry, Год журнала: 2024, Номер 36, С. 101924 - 101924

Опубликована: Янв. 24, 2024

Язык: Английский

Процитировано

10

Surface decorated metal carbonyl clusters: bridging organometallic molecular clusters and atomically precise ligated nanoclusters DOI Creative Commons
Cristiana Cesari, Cristina Femoni, Francesca Forti

и другие.

Dalton Transactions, Год журнала: 2025, Номер unknown

Опубликована: Янв. 1, 2025

In this Frontier Article, the work carried out within our research group in Bologna field of surface decorated metal carbonyl clusters will be outlined and put a...

Язык: Английский

Процитировано

1

[K2(Bi@Pd12@Bi20)]4–: An Endohedral Inorganic Fullerene with Spherical Aromaticity DOI
Cong‐Cong Shu, Dariusz W. Szczepanik, Alvaro Muñoz‐Castro

и другие.

Journal of the American Chemical Society, Год журнала: 2024, Номер 146(20), С. 14166 - 14173

Опубликована: Май 8, 2024

Inorganic fullerene clusters have attracted widespread attention due to their highly symmetrical geometric structures and intrinsic electronic properties. However, cage-like composed of heavy metal elements with high symmetry are rarely reported, synthesis is also challenging. In this study, we present the a [K2(Bi@Pd12@Bi20)]4- cluster that incorporates {Bi20} cage pseudo-Ih symmetry, making it largest main group compound bismuth element date. Magnetic characterization theoretical calculations suggest spin state overall quartet. Quantum chemical reveal [Bi20]3- has similar configuration C606- [Bi@Pd12@Bi20]6- exhibits unique open-shell aromatic character.

Язык: Английский

Процитировано

4

Interfacial linkage modulated amorphous molybdenum sulfide/bismuth halide perovskite heterojunction for enhanced visible-light-driven photocatalytic hydrogen evolution DOI Creative Commons
He Zhao, Rossella Greco, Rafal Sliz

и другие.

Applied Catalysis B Environment and Energy, Год журнала: 2024, Номер 358, С. 124454 - 124454

Опубликована: Июль 29, 2024

Photocatalytic hydrogen evolution is a promising approach for direct solar-to-fuel conversion. Although significant research efforts have been put on the development of lead-free metal halide perovskites to reach excellent optoelectronic properties, their rational design efficient heterojunction photocatalytic systems still poses challenges. Here, we report new strategy tailor interface hybrid tri(dimethylammonium) hexaiodobismuthate (DMA3BiI6) and amorphous molybdenum sulfide (a-MoSx) heterojunctions. Specifically, a-MoSx was prepared with abundant apical S2– or bridging S22– ligands allow coupling DMA3BiI6 via an interfacial Mo–S–Bi linkage. The as-obtained heterostructures were found show improved visible-light-driven in hydroiodic acid splitting under mild conditions reaching superior rate around 750 µmol g−1 h−1 apparent quantum efficiency (AQE) 13.0 % at 420 nm. high activity kept after long-term performance test 3 days.

Язык: Английский

Процитировано

4

Bismuth(III)-Catalyzed Oxidative Cross-Coupling of 3-Hydroxycarbazoles with Arenols under an Oxygen Atmosphere DOI
Kengo Kasama,

Yuta Koike,

Haoyang Dai

и другие.

Organic Letters, Год журнала: 2023, Номер 25(35), С. 6501 - 6505

Опубликована: Авг. 28, 2023

A Bi(OTf)3-catalyzed oxidative cross-coupling reaction of 3-hydroxycarbazoles with arenols was developed under mild conditions. Both substrates were used in a 1:1 molar ratio the presence catalytic amount Bi(OTf)3. The carried out an oxygen atmosphere at 30 °C to afford C1-symmetric hydroxybiaryls good yields (up 94%) high chemo- and regioselectivity.

Язык: Английский

Процитировано

1

How to Deal with Charge in the Ranking of Lewis Acidity: Critical Evaluation of an Extensive Set of Cationic Lewis Acids DOI Creative Commons
Philipp Erdmann, Manuel Schmitt, Lukas M. Sigmund

и другие.

Angewandte Chemie, Год журнала: 2024, Номер 136(22)

Опубликована: Март 13, 2024

Abstract The quantification of Lewis acidity is fundamental and applied importance in chemistry. However, if neutral charged acids are compared, a coherent ranking has been elusive, severe uncertainties were accepted. With this study, we present systematic computational analysis base affinities 784 mono‐, di‐ tricationic their comparison with 149 representative acids. Evaluating vacuum fluoride ion (FIA) reveals charge‐caused clustering that prohibits any meaningful ranking. Instead, solvation‐corrected FIA solv identified as metric overcomes charge sensitivity balanced manner, allowing for evaluation across varying states. Analyzing the impact molecular volume on solvation‐induced damping provides rationales trends guidelines choice or design cationic condensed phase. Exploring alternative scales, explicit counteranion effects, selected experimental case studies reaffirms advantages most versatile practical approach quantitative general (thermodynamic) acidity.

Язык: Английский

Процитировано

0