Microenvironment Regulation, Promoting CO2 Conversion to Mono- and Multicarbon Products over Cu-Based Catalysts DOI
Ying‐Ya Liu, Zhichao Sun, Chong Peng

и другие.

Industrial & Engineering Chemistry Research, Год журнала: 2024, Номер unknown

Опубликована: Ноя. 16, 2024

This Review summarizes recent advancements in regulating microenvironments for enhancing CO2 conversion, particularly focusing on copper-based catalysts, which are crucial transforming to valuable chemicals and fuels. We discuss strategies microenvironment regulation, including single-atom catalyst design, particle size/facets/morphology control, confinement effects, interfacial engineering. These approaches influence the efficiency selectivity of conversion by optimizing active site density, controlling reactant/intermediate concentrations, promoting charge-transfer processes. highlight importance mass transfer, electrolyte properties, modifying electrode structures improving conversion. Despite significant progress, challenges remain electrocatalytically achieving high current densities multicarbon products, developing effective quantify contribution catalytic performance. Future research will focus advanced characterization techniques, exploring novel materials synthesis methods, utilizing machine learning theoretical modeling design optimization.

Язык: Английский

Bridge‐Oxygen Bond: An Active Group for Energy Electrocatalysis DOI Open Access
Nana Zhang, Zilan Zhang,

Siwei Yan

и другие.

Advanced Functional Materials, Год журнала: 2025, Номер unknown

Опубликована: Март 20, 2025

Abstract Energy electrocatalytic reactions such as hydrogen evolution reaction, oxygen reduction nitrogen carbon etc., are important to solve the current energy shortage and increasing environmental problems. Developing novel efficient catalyts for these has become an essential urgent issue. Catalysts incorporating bridge‐oxygen bond have received attention due their superior conductivity stability, which favorable optimizing reaction mechanism improving kinetics. This paper provides a comprehensive review encompassing concept of bond, means characterization, activity in electrocatalysis effect on catalytic performance. Through this review, it is expected furnish valuable reference rational design catalysts featuring structure across diverse reactions.

Язык: Английский

Процитировано

1

Engineering interfacial molecular interactions on Ag Hollow fibre gas diffusion electrodes for high efficiency in CO2 conversion to CO DOI

Yizhu Kuang,

Guoliang Chen,

Dimuthu Herath Mudiyanselage

и другие.

Chemistry - A European Journal, Год журнала: 2024, Номер unknown

Опубликована: Окт. 9, 2024

The electrochemical CO

Язык: Английский

Процитировано

2

Controlled Synthesis of Copper Sulfide-associated Catalysts for Electrochemical Reduction of CO2 to Formic Acid and Beyond: A Review DOI Creative Commons
Anirban Mukherjee, Maryam Abdinejad, Susanta Sinha Mahapatra

и другие.

Energy Advances, Год журнала: 2024, Номер unknown

Опубликована: Янв. 1, 2024

This review provides a comprehensive overview of various advanced engineering strategies and controlled synthesis copper–sulfide compounds for enhanced electrochemical CO 2 reduction to valuable products.

Язык: Английский

Процитировано

1

Microenvironment Regulation, Promoting CO2 Conversion to Mono- and Multicarbon Products over Cu-Based Catalysts DOI
Ying‐Ya Liu, Zhichao Sun, Chong Peng

и другие.

Industrial & Engineering Chemistry Research, Год журнала: 2024, Номер unknown

Опубликована: Ноя. 16, 2024

This Review summarizes recent advancements in regulating microenvironments for enhancing CO2 conversion, particularly focusing on copper-based catalysts, which are crucial transforming to valuable chemicals and fuels. We discuss strategies microenvironment regulation, including single-atom catalyst design, particle size/facets/morphology control, confinement effects, interfacial engineering. These approaches influence the efficiency selectivity of conversion by optimizing active site density, controlling reactant/intermediate concentrations, promoting charge-transfer processes. highlight importance mass transfer, electrolyte properties, modifying electrode structures improving conversion. Despite significant progress, challenges remain electrocatalytically achieving high current densities multicarbon products, developing effective quantify contribution catalytic performance. Future research will focus advanced characterization techniques, exploring novel materials synthesis methods, utilizing machine learning theoretical modeling design optimization.

Язык: Английский

Процитировано

1