Ruthenium‐Catalyzed Chemoselective Olefin Transfer Hydrogenation of alpha,beta‐Unsaturated Carbonyl Systems By Using EtOH as Hydrogen Source DOI Creative Commons
Martin Albrecht, Alicia Beaufils

ChemCatChem, Год журнала: 2024, Номер unknown

Опубликована: Окт. 30, 2024

Abstract The use of EtOH as hydrogen donor is remarkably under explored in transfer hydrogenation reactions, even though represents an appealing source. With the cationic ruthenium complex [Ru(PYA)(cymene)] + , 1 containing a N,N‐bidentate amino‐functionalized pyridinium amidate (PYA) ligand catalyst precursor, we here demonstrate first example chemoselective room temperature C═C bond α,β‐unsaturated ketones using benign source to yield variety functionalized ketones. reaction proceeds mild conditions with K 2 CO 3 base and conventiently at temperature. A broad substrate scope, including various carbonyl groups, demonstrates general applicability this method. Preliminary mechanistic studies suggest formation alkoxide [ ]–OEt initially formed species, requirement for induce hydride transfer, suggesting protic activation catalyst.

Язык: Английский

Potential industrial and nutritional applications of shrimp by-products: a review DOI Creative Commons

Abuzar,

Hafiz Rizwan Sharif, Mian Kamran Sharif

и другие.

International Journal of Food Properties, Год журнала: 2023, Номер 26(2), С. 3407 - 3432

Опубликована: Дек. 4, 2023

Asia is the largest producer of shrimp, accounting for 70% global cultured production. The market shrimp has a high demand and by-products from processing make up 40–60% whole shrimp. main include head, viscera, shell, pelopods, tail, cephalothorax, exoskeleton. trends future hurdles by-product utilization have been outlined. These are good source protein anti-inflammatory, anti-fungal, anti-oxidant properties. They also enhance immune system bioactive compounds that encourage their use anti-cancerous, anti-hypertensive, various other diseases. waste produced can yield valuable by-products, including astaxanthin, oil, carotenoids, fortified products, nutrient-enriched chitin, protein, flavor enhancers, composite flour. astaxanthin 59.97 µg/g along with carotenoid 68.26 µg/ml dw, chitosan (87%), (47.8%), oil extracted (88.9%) head rich (66%) chitin (6%). help meet growing an increasing population. abundance healthy ingredients found in makes it resource scientists, entrepreneurs, industrialists to develop new products. Additionally, utilizing reduce burden on earth decrease environmental pollution.

Язык: Английский

Процитировано

17

Well-Defined Robust Imidazole-Based Metal–Ligand Cooperative Ru(II)-para-Cymene for Transfer Hydrogenation of Furanic Aldehydes Using Renewable Alcohols DOI
Rahul Daga Patil, Sanjay Pratihar

ACS Sustainable Chemistry & Engineering, Год журнала: 2024, Номер 12(16), С. 6206 - 6219

Опубликована: Апрель 9, 2024

The present study addresses the challenges in catalytic transfer hydrogenation using methanol/ethanol for converting biomass-derived furanic aldehydes to furfuryl alcohols. introduction of air-stable Ru(II)-para-cymene catalysts with imidazole-based metal–ligand cooperativity represents a significant advancement. Spectroscopic, situ monitoring, labeling, and DFT investigations reveal mechanistic details, highlighting role Ru–H generation through dehydrogenation Ru(II)-alkoxide intermediates. Hydride proton transfers are facilitated by interconvertible coordination mode imidazole Ru(II)–para-cymene, which is crucial maintaining catalyst's efficiency selectivity. Notably, pKa N–H coordinated significantly influences reactivity, following specific order depending on attached heterocycle: > pyridine thiazole. This correlates well computed activation barrier generation. catalyst exhibits ease synthesis, stability air moisture, use renewable hydrogen sources, excellent selectivity aldehydes, applicability various potential large-scale processes. These features collectively contribute economic sustainable nature both protocol, providing valuable contribution field hydrogenation.

Язык: Английский

Процитировано

6

The Role of Effective Catalysts for Hydrogen Production: A Performance Evaluation DOI Creative Commons
A. Yağmur Gören, Mert Temiz, Doğan Erdemir

и другие.

Energy, Год журнала: 2024, Номер unknown, С. 134257 - 134257

Опубликована: Дек. 1, 2024

Язык: Английский

Процитировано

3

Chitosan as a Bio-Based Ligand for the Production of Hydrogenation Catalysts DOI Creative Commons
Stefano Paganelli,

Eleonora Brugnera,

Alessandro Di Michele

и другие.

Molecules, Год журнала: 2024, Номер 29(9), С. 2083 - 2083

Опубликована: Май 1, 2024

Bio-based polymers are attracting increasing interest as alternatives to harmful and environmentally concerning non-biodegradable fossil-based products. In particular, bio-based may be employed ligands for the preparation of metal nanoparticles (M(0)NPs). this study, chitosan (CS) was used stabilization Ru(0) Rh(0) (MNPs), prepared by simply mixing RhCl3 × 3H2O or RuCl3 with an aqueous solution CS, followed NaBH4 reduction. The formation M(0)NPs-CS confirmed Fourier Transform Infrared Spectroscopy (FT-IR), Differential Scanning Calorimetry (DSC), Thermal Gravimetric Analysis (TGA), Electron Microscopy (SEM), Energy-Dispersive X-ray (EDX), Transmission (TEM) Diffraction (XRD). Their size estimated below 40 nm Rh(0)-CS 10nm Ru(0)-CS SEM analysis. were hydrogenation (E)-cinnamic aldehyde levulinic acid. Easy recovery liquid-liquid extraction made it possible separate catalyst from reaction Recycling experiments demonstrated that highly efficient up four times in best conditions. data found study show CS is excellent ligand nanoparticles, allowing production some most efficient, selective recyclable catalysts known literature.

Язык: Английский

Процитировано

1

Ruthenium‐Catalyzed Chemoselective Olefin Transfer Hydrogenation of alpha,beta‐Unsaturated Carbonyl Systems By Using EtOH as Hydrogen Source DOI Creative Commons
Martin Albrecht, Alicia Beaufils

ChemCatChem, Год журнала: 2024, Номер unknown

Опубликована: Окт. 30, 2024

Abstract The use of EtOH as hydrogen donor is remarkably under explored in transfer hydrogenation reactions, even though represents an appealing source. With the cationic ruthenium complex [Ru(PYA)(cymene)] + , 1 containing a N,N‐bidentate amino‐functionalized pyridinium amidate (PYA) ligand catalyst precursor, we here demonstrate first example chemoselective room temperature C═C bond α,β‐unsaturated ketones using benign source to yield variety functionalized ketones. reaction proceeds mild conditions with K 2 CO 3 base and conventiently at temperature. A broad substrate scope, including various carbonyl groups, demonstrates general applicability this method. Preliminary mechanistic studies suggest formation alkoxide [ ]–OEt initially formed species, requirement for induce hydride transfer, suggesting protic activation catalyst.

Язык: Английский

Процитировано

1