I2/H2O2 Mediated Synthesis and Photophysical Properties of Imidazole‐Fused Heterocycles via [4+1] Cyclization Approach DOI
Haonan Li,

Chenping Gao,

Qingjie Liu

и другие.

ChemistrySelect, Год журнала: 2024, Номер 9(36)

Опубликована: Сен. 1, 2024

Abstract An efficient I 2 (10 mmol %)/H O mediated oxidative formal [4+1] cyclization of 2‐pyridinemethylamine or o ‐phenylenediamine (2‐aminobenzenethiol) with benzaldehyde via C−N bond formation has been developed. This strategy provides a straightforward approach to imidazo[1,5‐ ]pyridines, iodo‐substituted ]pyridines and benzimidazole (benzothiazole) derivatives in yields ranging from 60 % 98 %, respectively. Several heterocyclic products exhibit promising blue luminous performance satisfactory fluorescence quantum up 64 large Stokes shifts, longer lifetime (7.35 ns). The band gap energies obtained DFT are also consistent the absorption spectra.

Язык: Английский

Synthesis and site selective C–H functionalization of imidazo-[1,2-a]pyridines DOI
Javeed Ahmad Tali, G. Ravi Kumar, Bhupesh Sharma

и другие.

Organic & Biomolecular Chemistry, Год журнала: 2023, Номер 21(36), С. 7267 - 7289

Опубликована: Янв. 1, 2023

Herein we disclose the synthesis and an overview of all functionalization reactions at each carbon atom, viz , C2, C3, C5, C6, C7 C8 imidazo[1,2- a ]pyridine.

Язык: Английский

Процитировано

18

Structural insight into imidazopyridines and benzimidazoles: the importance of the hydrogen bond, π-stacking interactions and intramolecular charge transfer effect for fluorescence DOI
Haonan Li,

Chenping Gao,

Zhibin Li

и другие.

CrystEngComm, Год журнала: 2024, Номер unknown

Опубликована: Янв. 1, 2024

An investigation of the impact N-position, H-bond and π-stacking for fluorescence in imidazopyridine benzimidazole derivatives.

Язык: Английский

Процитировано

2

Recent Advances in the Electrochemical Functionalization of Imidazoheterocycles DOI
Sifeng Li

Advanced Synthesis & Catalysis, Год журнала: 2024, Номер unknown

Опубликована: Окт. 18, 2024

Abstract Imidazoheterocycles have extensive applications in the pharmaceutical industry and agrochemicals. A comprehensive overview has been provided on current advancements electrochemical functionalization of imidazo‐fused heterocycles, which classified into ten different types reactions. Electrochemical synthesis emerged as a highly effective method for producing organic molecules, especially context sustainable development. Employing electrons traceless oxidant, several C−H reactions heterocycles achieved at either C3 or C5 positions. Electrons may serve reducing agent to synthesize pyridine rings that are partially fully saturated imidazo[1,2‐ ]pyridines. The purpose review is attract interest scientific community promote additional research imidazoheterocycles using methods.

Язык: Английский

Процитировано

1

An efficient and environment-friendly halogenation of imidazoheterocycles with Bu4NX (X = Cl, Br and I) using iodobenzene diacetate as oxidant DOI
Minghua Yang,

Ya-Ting Shao,

Wei Zhang

и другие.

Tetrahedron Letters, Год журнала: 2024, Номер 144, С. 155135 - 155135

Опубликована: Июнь 6, 2024

Язык: Английский

Процитировано

0

A time-controlled selective bromination and formylation of 2-arylimidazo[1,2-a]pyridines DOI

Sheiva Iranfar,

Morteza Shiri, Soma Majedi

и другие.

Journal of the Iranian Chemical Society, Год журнала: 2024, Номер 21(9), С. 2469 - 2475

Опубликована: Авг. 19, 2024

Язык: Английский

Процитировано

0

I2/H2O2 Mediated Synthesis and Photophysical Properties of Imidazole‐Fused Heterocycles via [4+1] Cyclization Approach DOI
Haonan Li,

Chenping Gao,

Qingjie Liu

и другие.

ChemistrySelect, Год журнала: 2024, Номер 9(36)

Опубликована: Сен. 1, 2024

Abstract An efficient I 2 (10 mmol %)/H O mediated oxidative formal [4+1] cyclization of 2‐pyridinemethylamine or o ‐phenylenediamine (2‐aminobenzenethiol) with benzaldehyde via C−N bond formation has been developed. This strategy provides a straightforward approach to imidazo[1,5‐ ]pyridines, iodo‐substituted ]pyridines and benzimidazole (benzothiazole) derivatives in yields ranging from 60 % 98 %, respectively. Several heterocyclic products exhibit promising blue luminous performance satisfactory fluorescence quantum up 64 large Stokes shifts, longer lifetime (7.35 ns). The band gap energies obtained DFT are also consistent the absorption spectra.

Язык: Английский

Процитировано

0