Theoretical Investigation on Indeno-Annulation of O-Formyl-Ynone and P-Bis-O-Formyl-Ynone with Dimethylacetone-1,3-Dicarboxyate for Synthesis of 9‑Fluorenol and Indeno[1,2‑B]Fluorenol DOI
Nan Lü, Chengxia Miao, Xiaozheng Lan

и другие.

Опубликована: Янв. 1, 2023

The mechanism is investigated for indeno-annulation of o-formyl-ynone, p-bis-o-formyl-ynone with DMAD under metal-free. cascade process consists Michael addition, aldol reaction condensation/aromatization. addition initiated by enol form via nucleophilic attack to ynone delivering accumulated diene the first new C−C bond. From ketone isomer, reaction/H transfer proceeds producing second bond and five-membered ring. enol-ketone tautomerism annulation are prior condensation affording third another six-membered fluorenol product given aromatization. positive solvation effect DMSO solution lies in reduction absolute activation energies reaction. exerts more favorable influence on simple CHO at ortho-position than case substituted this indeno-annulation. These results supported Multiwfn analysis FMO specific TSs MBO value vital bonding, breaking.

Язык: Английский

An Approach to Functionally Embellished o-Alkynylbenzoates or Furan-3(2H)-ones from Diynones and DMAD: Controlled Divergence and Product Selectivity DOI
Manas Jyoti Sarma,

K. A. Sudarshana,

Srihari Pabbaraja

и другие.

The Journal of Organic Chemistry, Год журнала: 2023, Номер 88(6), С. 3945 - 3953

Опубликована: Март 2, 2023

The discovery of reaction regime controlled product diversification in a one-pot between diynones and dimethyl-1,3-acetonedicarboxylate (DMAD) to selectively furnish either functionally unique pentasubstituted o-alkynylbenzoates or fully substituted furan-3(2H)-ones is delineated. potential these two versatile platforms enter new utilitarian chemical space has also been explored.

Язык: Английский

Процитировано

12

One-Flask, Telescoped Synthesis of Pyrano[3,2-b]indol-2-ones from O-Nitroynones and β-Ketoesters: Further Advancement to Functionalized Carbazoles DOI

K. A. Sudarshana,

Alagesan Balasubramani, Srihari Pabbaraja

и другие.

The Journal of Organic Chemistry, Год журнала: 2025, Номер unknown

Опубликована: Март 19, 2025

A new general strategy for accessing pyrano[3,2-b]indol-2-ones, a promising fused hybrid heterocyclic system, has been devised from o-nitroynones and β-ketoesters through one-flask cascade process involving tandem Michael addition, intramolecular cyclization, Cadogan-Sundberg reductive cyclization. The utility of this approach further amplified by leveraging the cycloaddition proclivity α-pyrone moiety in pyrano[3,2-b]indol-2-ones toward concise entry to carbazoles. Illustrative synthesis carbazole natural products hyellazole chlorohyellazole is also disclosed.

Язык: Английский

Процитировано

0

Photocatalytic Denitrative Alkenylation of Nitroalkanes DOI
Ayumi Osawa,

K Uemura,

Shuji Murakami

и другие.

Organic Letters, Год журнала: 2024, Номер unknown

Опубликована: Ноя. 25, 2024

Reductive radical generation has become a cornerstone of modern photoredox chemistry. However, the synthesis functionalized precursors remains tedious multistep process. In this study, we focus on potential nitro group as redox-active functional and present denitrative alkenylation nitroalkanes, facilitated by photoreductive alkyl radicals from nitroalkanes. By taking advantage facile α-functionalization successfully generate various radicals, which are subsequently used in reactions.

Язык: Английский

Процитировано

3

Enantioselective Michael addition of malonates to β,γ-unsaturated α-ketoesters catalysed by Cu(ii) complexes bearing binaphthyl–proline hybrid ligands DOI

Shibo Yu,

Qihang Cai,

Jiahui Li

и другие.

Organic & Biomolecular Chemistry, Год журнала: 2023, Номер 21(8), С. 1764 - 1770

Опубликована: Янв. 1, 2023

High yields (up to 96%) and high ee 92%) were achieved for chiral copper(II) complex-catalysed enantioselective Michael addition of malonates β,γ-unsaturated-α-ketoesters. The ligands took advantage both the binaphthyl proline moieties, substituents with different electronic steric features could be tolerated. reactions carried out under mild conditions, a gram scale reaction realised without loss yield enantioselectivity.

Язык: Английский

Процитировано

7

Indeno-Annulation of o-Formyl-Ynones, o-Bis-Ynones, and p-Bis-o-Formyl-Ynones with Dimethyl Acetone-1,3-Dicarboxylate: One Flask Cascade Synthesis of Functionally Endowed 9-Fluorenols and Indeno[1,2-b]fluorenols DOI

Bilal Ahmad Ganaie,

Alagesan Balasubramani, Bilal A. Bhat

и другие.

The Journal of Organic Chemistry, Год журнала: 2023, Номер 88(16), С. 11637 - 11649

Опубликована: Авг. 9, 2023

A mild, scalable, one-pot access to multifunctional 9-fluorenols from o-formyl-ynones and o-bis-ynones on reaction with dimethylacetone-1,3-dicarboxyate through tandem Michael addition-Aldol condensation cascade has been conceptualized executed. The scope utility of this synthetic approach have further amplified for entry into functionally enhanced, higher order fluorenols like pentacyclic indeno[1,2-b]fluorene-6,12-diols indeno[1,2-b]fluorene-6,12-diones the implementation "double indeno-annulation" tactic p-bis-o-formyl ynones dimethylacetone-1,3-dicarboxylate. Besides several green attributes, current is also compatible emerging time energy economy features a swift gateway build complexity.

Язык: Английский

Процитировано

3

Theoretical Investigation on Indeno-annulation of o-formyl-ynone and p-bis-o-formyl-ynone with Dimethylacetone-1,3-dicarboxyate for Synthesis of 9-fluorenol and Indeno[1,2-b]fluorenol DOI Open Access
Nan Lü, Chengxia Miao, Xiaozheng Lan

и другие.

Acta Scientific Pharmaceutical Sciences, Год журнала: 2024, Номер unknown, С. 03 - 13

Опубликована: Фев. 1, 2024

The mechanism is investigated for indeno-annulation of o-formyl-ynone, p-bis-o-formyl-ynone with DMAD under metal-free.The cascade process consists Michael addition, aldol reaction condensation/aromatization.Michael addition initiated by enol form via nucleophilic attack to ynone delivering accumulated diene the first new C-C bond.From ketone isomer, reaction/H transfer proceeds producing second bond and five-membered ring.The enol-ketone tautomerism annulation are prior condensation affording third another six-membered fluorenol product given aromatization.The positive solvation effect DMSO solution lies in reduction absolute activation energies reaction.DMSO exerts more favorable influence on simple CHO at ortho-position than case substituted this indeno-annulation.These results supported Multiwfn analysis FMO specific TSs MBO value vital bonding, breaking.As a prime objective chemical industry, development synthetic methodologies not only essential sustainable production chemicals but also related efficiency, step, cost environmental impact minimize waste ecological footprint [1-3].In pursuit goal, catalysis discipline offering efficient versatile strategies sustainability especially formation multiple bonds presenting productive direction.It enables expansion enrichment domino or tandem processes executed one flask one-pot fashion thus minimizing number purification separation steps [4-6].The construction various polycyclic scaffolds such tactics provides privileged category expeditious delivery functional complex potential drug conjugates involving wide range pharmacological activities [7-9].In field, ynones regarded as promising platforms many reactive sites build [10].The reactions variety multifunctional partner often unraveled space.A was achieved Ru-catalyzed oxidative alkynylation oxetanols, azetidinols bicyclopentanols ynones, which subsequently converted azetidine-, oxetaneand bicyclopentane-bearing isoxazoles, pyrazoles pyrimidines [11].Conjugated alkynones occupied firm position among building blocks.The base-catalyzed substrate-controlled dimerizations aliphatic were focused density theory (DFT) study understand origin selectivity assembly [12].The cyclization diazo compounds promoted DBU has been developed synthesis fused eight-membered oxocino[2,3-c] single step highly regio-and diastereoselective manner [13].

Язык: Английский

Процитировано

0

One flask cascade approach to complex pyrano[2,3-c]pyrazole-pyrazolone hybrid heterocyclic system and its initiatory neurobiological profiling DOI
Alagesan Balasubramani,

K. A. Sudarshana,

Roli Kushwaha

и другие.

Chemical Communications, Год журнала: 2024, Номер 60(64), С. 8443 - 8446

Опубликована: Янв. 1, 2024

A one-pot multicomponent approach towards a hybrid heterocyclic pyrano[2,3-

Язык: Английский

Процитировано

0

Photocatalytic Denitrative Alkenylation of Nitroalkanes DOI Creative Commons
Ayumi Osawa,

K Uemura,

Shuji Murakami

и другие.

Опубликована: Авг. 30, 2024

Reductive radical generation has become a cornerstone of modern photoredox chemistry. However, the synthesis functionalized precursors remains tedious multi-step process. In this study, we focus on potential nitro group as redox-active functional and present denitrative alkenylation nitroalkanes, facilitated by photoreductive alkyl radicals from nitroalkanes. By taking advantage facile α-functionalization successfully generate various radicals, which are subsequently used in reactions.

Язык: Английский

Процитировано

0

Reductive Homologation of Nitroalkanes via Denitrative Aminoalkylation DOI
Ayumi Osawa, M. BALASUBRAMANIAN, Yoshiaki Nakao

и другие.

Organic Letters, Год журнала: 2024, Номер 26(42), С. 9046 - 9050

Опубликована: Окт. 16, 2024

We present the reductive homologation of nitroalkanes through utilization denitrative aminoalkylation reaction. This transformation is accomplished by radical-radical coupling alkyl radicals derived from and persistent aminoalkyl radicals. By capitalizing on diverse α-functionalization nitroalkanes, α,β-multifunctionalized amines can be readily accessed.

Язык: Английский

Процитировано

0

Theoretical Investigation on Indeno-Annulation of O-Formyl-Ynone and P-Bis-O-Formyl-Ynone with Dimethylacetone-1,3-Dicarboxyate for Synthesis of 9‑Fluorenol and Indeno[1,2‑B]Fluorenol DOI
Nan Lü, Chengxia Miao, Xiaozheng Lan

и другие.

Опубликована: Янв. 1, 2023

The mechanism is investigated for indeno-annulation of o-formyl-ynone, p-bis-o-formyl-ynone with DMAD under metal-free. cascade process consists Michael addition, aldol reaction condensation/aromatization. addition initiated by enol form via nucleophilic attack to ynone delivering accumulated diene the first new C−C bond. From ketone isomer, reaction/H transfer proceeds producing second bond and five-membered ring. enol-ketone tautomerism annulation are prior condensation affording third another six-membered fluorenol product given aromatization. positive solvation effect DMSO solution lies in reduction absolute activation energies reaction. exerts more favorable influence on simple CHO at ortho-position than case substituted this indeno-annulation. These results supported Multiwfn analysis FMO specific TSs MBO value vital bonding, breaking.

Язык: Английский

Процитировано

1