Synergistic photoinduction of ferroptosis and apoptosis by a mitochondria-targeted iridium complex for bladder cancer therapy DOI Creative Commons

J Zheng,

Aijing Zhang, Qinglong Du

и другие.

Journal of Colloid and Interface Science, Год журнала: 2024, Номер 683, С. 420 - 431

Опубликована: Дек. 12, 2024

Bladder cancer (BC) is one of the most common malignant tumors urinary system, and has a high recurrence rate treatment resistance. Recent results indicate that mitochondrial metabolism influences therapeutic outcomes BC. Mitochondria-targeted photosensitizer (PS) promising anticancer approach may overcome limitations conventional BC treatments. Herein, two mitochondria-targeted iridium(III) PSs, Ir-Mito1 Ir-Mito2, have been designed for treatment. Mechanically, Ir-Mito2 induced decrease in membrane potential via white light activation, further triggering reduction B-cell lymphoma 2 protein (Bcl-2)/Bcl-associated X (Bax) ratio increment cleaved caspase3. Meanwhile, glutathione, deactivation glutathione peroxidase 4 (GPX4), increase acyl-CoA synthetase long chain family member (ACSL4), accumulation lipid peroxide resulted synergistically activating ferroptosis apoptosis. The demonstrated exhibited excellent antitumor efficacy with superior biosafety vivo. This work on light-activated mitochondrial-targeted PS provides an innovative platform

Язык: Английский

Emerging engineered nanozymes: current status and future perspectives in cancer treatments DOI Creative Commons
Jiajia Zheng,

Weili Peng,

Houhui Shi

и другие.

Nanoscale Advances, Год журнала: 2025, Номер unknown

Опубликована: Янв. 1, 2025

Composite nanozymes are composed of enzymes with similar or different catalytic capabilities and have higher activity than a single enzyme. In recent years, composite emerged as novel nanomaterial platforms for multiple applications in various research fields, where they used to produce oxygen, consume glutathione, toxic reactive oxygen species (ROS) cancer therapy. The therapeutic approach using is known chemo-dynamic therapy (CDT). Some also show special photothermal conversion effects, enabling them be combined pioneering treatments, such photodynamic (PDT), (PTT) sonodynamic (SDT), enhance the anti-cancer effects. this study, classification performances reviewed, along their advantages synthesis methods. Furthermore, treatment cancers emphasized, prospective challenges future discussed.

Язык: Английский

Процитировано

1

Nanozyme-Based Strategies in Cancer Immunotherapy: Overcoming Resistance to Enhance Therapeutic Efficacy DOI Creative Commons
Guangjian Hou, Yukun Xu, Chunhua Wang

и другие.

Aging and Disease, Год журнала: 2025, Номер unknown, С. 0 - 0

Опубликована: Янв. 1, 2025

Nanozymes, which are nanomaterials that replicate the catalytic activities of natural enzymes in biological systems, have recently demonstrated considerable potential improving cancer immunotherapy by altering tumor microenvironment. Nanozyme-driven immune responses represent an innovative therapeutic modality with high effectiveness and minimal side effects. These nanozymes activate system to specifically recognize destroy cells. Combined immunotherapeutic agents, can amplify anti-cancer integrating remodeling immunogenic cell death (ICD). This review offers a thorough discussion about various involved immunity, including those mimicking catalase (CAT), superoxide dismutase (SOD), peroxidase (POD), oxidase (OXD). It also discusses challenges future directions for translating nanozyme platforms into clinical applications, enhancing susceptibility cells immunotherapy. Nanozyme-based strategies substantial oncology, offering new effective options management.

Язык: Английский

Процитировано

0

Porous Fe/Cu Nanoreactor with Dual Insurance Design for Precision Chemotherapy and Chemodynamic Therapy DOI
Xianyu Zhu,

Lingli Gao,

Yanbo Zheng

и другие.

Advanced Healthcare Materials, Год журнала: 2025, Номер unknown

Опубликована: Март 24, 2025

Abstract Poor prognosis and chemotherapy response stem from difficulties in precise targeting the lack of effective synergistic treatments. Nanozymes show promising potential tumor chemodynamic therapy (CDT) by catalyzing hydrogen peroxide (H₂O₂) decomposition glutathione depletion microenvironment (TME). However, integrating with CDT remains challenging. In this study, a porous Fe/Cu bimetallic nanozyme carrier (FeCuNPs) is developed for co‐loading humanized 3F8 anti‐GD2 disialoganglioside antibody (3F8) novel pyridazinone‐based chemotherapeutic agent (IMB), forming nanoreactor (3F8@FeCuNPs@IMB) targeted CDT. The responds specifically to acidic TME as primary insurance, allowing controlled release IMB at site. coating on surface acts secondary minimizing drug leakage during delivery process ensuring chemotherapy. Furthermore, FeCuNPs act peroxidase‐like (POD) oxidase‐like (GSHOX) enzymes, hydroxyl radical (•OH) generation depleting excess GSH, enhancing results vitro vivo indicate that dual insurance designed 3F8@FeCuNPs@IMB offers prospect targeted, precise, combination against melanoma.

Язык: Английский

Процитировано

0

NIR‐II D–A–D‐Type Small‐Molecule Coordination with Carboxylatopillar[5]Arene: a Multifunctional Phototheranostic for Low‐Temperature NIR‐II Photothermal/Platinum‐Based/Chemodynamic Combination Cancer Immunotherapy DOI

Miaomiao Ding,

Hao Chen,

Liuliang He

и другие.

Small, Год журнала: 2025, Номер unknown

Опубликована: Апрель 21, 2025

Abstract Low‐temperature second near‐infrared region (NIR‐II) photothermal therapy (PTT) has shown significant potential in minimizing damage to normal tissues and reducing inflammation. However, it still faces challenge of insufficient immune response. Thus, a multifunctional phototheranostic nanoparticle (BDPB/Pt/Fe@P[5]) is developed by co‐loading BDPB, CDHPt, Fe 2 ⁺ with pH‐sensitive lipid DSPE‐PEOz2K. The carboxylatopillar[5]arene (CP[5]) used construct this exhibits strong host–guest recognition pyridine salts, alleviating aggregation caused quench (ACQ) effect enhancing the NIR‐II emission donor–acceptor–donor (D–A–D)‐type organic small molecule (BDPB). CP[5] provides suitable vehicles for encapsulating platinum (IV) prodrugs (CDHPt) ions via metal coordination controllable reactive oxygen species (ROS) release. Under low‐intensity laser irradiation an acidic tumor microenvironment, nanoparticles degrade, releasing CDHPt platinum‐based chemodynamic (CDT). facilitates direct production superoxide anions (O₂·⁻) from O₂ partially converts into highly cytotoxic hydroxyl radicals, thereby promoting Fenton reaction process. therapeutic efficacy further synergized immunogenic cell death (ICD) effect.

Язык: Английский

Процитировано

0

Nanozyme-based therapeutic strategies for rheumatoid arthritis DOI

Jucong Zhang,

Chenxi Wang,

Xiaochuan Wu

и другие.

Journal of Controlled Release, Год журнала: 2024, Номер 377, С. 716 - 734

Опубликована: Дек. 3, 2024

Язык: Английский

Процитировано

2

Synergistic photoinduction of ferroptosis and apoptosis by a mitochondria-targeted iridium complex for bladder cancer therapy DOI Creative Commons

J Zheng,

Aijing Zhang, Qinglong Du

и другие.

Journal of Colloid and Interface Science, Год журнала: 2024, Номер 683, С. 420 - 431

Опубликована: Дек. 12, 2024

Bladder cancer (BC) is one of the most common malignant tumors urinary system, and has a high recurrence rate treatment resistance. Recent results indicate that mitochondrial metabolism influences therapeutic outcomes BC. Mitochondria-targeted photosensitizer (PS) promising anticancer approach may overcome limitations conventional BC treatments. Herein, two mitochondria-targeted iridium(III) PSs, Ir-Mito1 Ir-Mito2, have been designed for treatment. Mechanically, Ir-Mito2 induced decrease in membrane potential via white light activation, further triggering reduction B-cell lymphoma 2 protein (Bcl-2)/Bcl-associated X (Bax) ratio increment cleaved caspase3. Meanwhile, glutathione, deactivation glutathione peroxidase 4 (GPX4), increase acyl-CoA synthetase long chain family member (ACSL4), accumulation lipid peroxide resulted synergistically activating ferroptosis apoptosis. The demonstrated exhibited excellent antitumor efficacy with superior biosafety vivo. This work on light-activated mitochondrial-targeted PS provides an innovative platform

Язык: Английский

Процитировано

0