Surfaces and Interfaces, Год журнала: 2025, Номер unknown, С. 106342 - 106342
Опубликована: Март 1, 2025
Язык: Английский
Surfaces and Interfaces, Год журнала: 2025, Номер unknown, С. 106342 - 106342
Опубликована: Март 1, 2025
Язык: Английский
Materials Today Chemistry, Год журнала: 2025, Номер 44, С. 102608 - 102608
Опубликована: Фев. 27, 2025
Язык: Английский
Процитировано
0Applied Catalysis O Open, Год журнала: 2025, Номер unknown, С. 207036 - 207036
Опубликована: Март 1, 2025
Язык: Английский
Процитировано
0Microchemical Journal, Год журнала: 2025, Номер unknown, С. 113392 - 113392
Опубликована: Март 1, 2025
Язык: Английский
Процитировано
0ACS Sustainable Chemistry & Engineering, Год журнала: 2025, Номер unknown
Опубликована: Апрель 1, 2025
Electrochemical generation of hydrogen peroxide (H2O2) through the two-electron oxygen reduction reaction (2e– ORR) represents a sustainable development strategy for bulk H2O2 manufacturing, yet crafting efficient catalysts remains substantial challenge. Carbon materials are particularly appealing as electrochemical catalysts, owing to their diverse nanostructures and adjustable attributes. Nonetheless, lack structure–property understanding has hindered progression metal-free carbon electrocatalysts. In this study, we fabricated porous with abundant edge sulfhydryl groups (−SH) determined that 2e– ORR performance is roughly proportional −SH content, outperforming reported in aspects such selectivity (90–98% over broad potential 0.30–0.70 V vs RHE) stability (maintaining 90% during 12 h testing) measured alkaline solution rotating ring-disk electrode setup. Furthermore, flow cell setup, both production rate (2910 mmol gcatalyst–1 h–1) Faraday efficiency (over 80%) surpass most carbon- metal-based Consequently, research illuminates straightforward pathway design specific sulfur configurations carbon-based high-selectivity production.
Язык: Английский
Процитировано
0Surfaces and Interfaces, Год журнала: 2025, Номер unknown, С. 106342 - 106342
Опубликована: Март 1, 2025
Язык: Английский
Процитировано
0