Advanced Functional Materials,
Год журнала:
2024,
Номер
35(1)
Опубликована: Окт. 31, 2024
Abstract
The
use
of
all‐solid‐state
lithium
metal
batteries
(ASSLMBs)
has
garnered
significant
attention
as
a
promising
solution
for
advanced
energy
storage
systems.
By
employing
non‐flammable
solid
electrolytes
in
ASSLMBs,
their
safety
profile
is
enhanced,
and
the
anode
allows
higher
density
compared
to
traditional
lithium‐ion
batteries.
To
fully
realize
potential
solid‐state
(SSEs)
must
meet
several
requirements.
These
include
high
ionic
conductivity
Li
+
transference
number,
smooth
interfacial
contact
between
SSEs
electrodes,
low
manufacturing
cost,
excellent
electrochemical
stability,
effective
suppression
dendrite
formation.
This
paper
delves
into
essential
requirements
enable
successful
implementation
ASSLMBs.
Additionally,
representative
state‐of‐the‐art
examples
developed
past
5
years,
showcasing
latest
advancements
SSE
materials
highlighting
unique
properties
are
discussed.
Finally,
provides
an
outlook
on
achieving
balanced
improved
addressing
failure
mechanisms
solutions,
critical
challenges
such
reversibility
plating/stripping
thermal
runaway,
characterization
techniques,
composite
SSEs,
computational
studies,
ASS
lithium–sulfur
lithium–oxygen
With
this
consideration,
ASSLMBs
can
be
realized.
Advanced Functional Materials,
Год журнала:
2023,
Номер
33(42)
Опубликована: Июнь 20, 2023
Abstract
In
recent
years,
metal‐organic
frameworks,
especially
MOF‐based
derivatives,
have
been
regarded
as
one
of
the
best
candidate
electrode
materials
for
next
generation
advanced
materials,
due
to
high
porosity,
large
surface
area,
modifiable
functional
groups
well
controllable
chemical
composition.
This
review
presents
corresponding
synthesis
methods,
structural
design,
and
electrochemical
performance
MOF‐derived
including
metal
oxides,
sulfides,
phosphides,
carbon
in
high‐performance
lithium‐ion
batteries.
Subsequently,
problems
that
exist
current
application
derivatives
electrodes
batteries
are
discussed
along
with
possible
feasible
solutions.
At
last,
some
reasonable
pathways
strategies
design
MOF
also
suggested.
Chemical Engineering Journal Advances,
Год журнала:
2024,
Номер
18, С. 100589 - 100589
Опубликована: Янв. 29, 2024
Reduce
environmental
impacts
and
guarantee
a
steady
supply
of
critical
chemicals
by
practising
sustainable
waste
management
chemical
production.
By
advancing
circular
economy
ideas
decreasing
dependency
on
finite
resources,
this
research
has
the
potential
to
alter
industrial
landscape
radically.
The
technological,
economic,
regulatory,
social
barriers
material
recovery
production
are
explored
in
paper.
key
resolving
these
issues
is
identification
solutions
that
both
economically
viable
environmentally
benign.
This
paper
introduces
Chemical
Production
Waste
Material
Recovery
Framework
(CP&WMRF),
which
incorporates
innovative
recycling
upcycling
methods,
manufacturing
processes,
incorporation
digital
technologies
like
artificial
intelligence
(AI)
machine
learning
(ML)
maximize
efficiency
with
resources
employed.
It
possible
reduce
energy
use
Interfaces
help
CP&WMRF.
Chemicals
can
be
manufactured
using
feedstocks
as
an
alternative
fossil
fuels.
system
standardizes
how
e-waste
recycled
recovered
metals
materials
used.
To
prove
viability
they
require
simulation
modeling
tools.
assessments
decision-makers
understand
benefits
drawbacks
proposed
terms
their
performance,
effect,
economic
viability.
When
pitted
against
AI-ML,
achieved
94.2
%,
CP&WMRF's
96.2%
result
reveals
significant
edge.
AI-ML
less
efficient,
score
93.8
%.
field
sustainability
analysis,
95.2%,
higher
than
AI-ML's
decent
lower
93.2%.
impressive
97.5%
CP&WMRF
resource
substantially
surpasses
92.8%
ascribed
AI-ML.
remarkable
success
optimizing
recovery,
98.7%,
91.5%
associated
present
establishes
framework
for
revolutionary
move
toward
green
chemistry
integrating
all-encompassing
applications,
rigorous
analysis.
