Advanced Functional Materials,
Год журнала:
2025,
Номер
unknown
Опубликована: Март 5, 2025
Abstract
Electrocatalytic
water
splitting
has
emerged
as
a
key
method
for
large‐scale
production
of
green
hydrogen.
Constructing
efficient,
durable,
and
low‐cost
electrocatalysts
the
hydrogen
evolution
reaction
at
high
current
densities
is
prerequisite
practical
industrial
applications
splitting.
Recently,
non‐noble
metal‐based
self‐supporting
electrodes
have
been
explored
density
due
to
their
cost‐effective,
conductivity
metal
substrate,
robust
interfacial
binding
between
catalyst
strong
mechanical
stability.
In
this
review,
recently
reported
(Ni,
Fe,
Cu,
Co,
Ti,
Mo,
alloy)
electrode
applied
are
comprehensively
summarized,
classified,
discussed.
Five
fundamental
design
principles
such
intrinsic
activity,
abundant
active
sites,
fast
electron
transfer,
mass
transport,
stability
proposed
discussed
achieve
high‐performance
under
densities.
Furthermore,
various
modification
strategies
including
heteroatom
doping,
morphology
engineering,
interface
phase
strain
engineering
enhance
catalytic
activity
durability
electrode.
Finally,
challenges
prospects
designing
efficient
stable
in
future
This
comprehensive
overview
will
provide
valuable
insight
guidance
development
production.
Dalton Transactions,
Год журнала:
2024,
Номер
53(37), С. 15390 - 15402
Опубликована: Янв. 1, 2024
The
choice
of
solid
3D
substrates
to
design
electrocatalysts
significantly
impacts
the
efficiency
and
effectiveness
self-supported
used
in
water
splitting.
These
are
pivotal
boosting
performance
by
providing
structural
support,
facilitating
electron
transport,
increasing
active
surface
area.
This
improvement
leads
higher
catalytic
better
stability,
ultimately
optimizing
electrocatalytic
process.
interaction
between
substrate
electrocatalyst
can
also
affect
intrinsic
properties
catalyst,
further
influencing
its
performance.
Therefore,
understanding
use
is
vital
for
advancing
water-splitting
technologies.
article
explores
critical
role
enhancing
activity
materials
By
examining
recent
developments
research
this
region,
we
target
showcase
a
comprehensive
how
different
influence
highlight
future
directions
these
systems
applications.
