Transition metal supported UiO-67 materials and their applications in catalysis DOI Creative Commons
Tingting Li, Yan Li, Jingxin Mao

и другие.

Frontiers in Chemistry, Год журнала: 2025, Номер 13

Опубликована: Май 30, 2025

Metal-organic frameworks (MOFs) have emerged as promising platforms for heterogeneous catalysis due to their tunable structures and high specific surface areas. Results indicate that modified composite MOFs not only exhibit superior water stability but also demonstrate broader applicability in catalysis, such Fenton-like oxidation, Morita-Baylis-Hillman reactions, ethylene dimerization, various photoelectrochemical processes. Among them, UiO-67, a zirconium-based MOF, has attracted extensive attention its exceptional chemical stability, catalytic activity, well-defined microporous structure. This review introduces composites formed by different types of single multi-metal loadings on UiO-67 demonstrated performance. It emphasizes the structure-performance relationships these composites, highlighting how metal loading spatial distribution influence reactivity stability. The current application status existing challenges series materials derivatives are systematically reviewed. By integrating experimental results mechanistic insights, this work underscores transformative potential meeting demands sustainable catalysis.

Язык: Английский

pH-responsive drug carriers MIL-125(Ti)-NH2 and MIL-125(Ti) for delivering colorectal cancer therapeutics 5-fluorouracil DOI
Jindrayani Nyoo Putro, Felycia Edi Soetaredjo, Maria Yuliana

и другие.

Journal of Porous Materials, Год журнала: 2025, Номер unknown

Опубликована: Фев. 1, 2025

Язык: Английский

Процитировано

1

Multifunctional sorafenib-loaded MXene for enhanced cancer therapy: In vitro and in vivo study based on chemotherapy/photothermal therapy approach DOI
Shehab Elbeltagi, Mohammed Al‐Zharani, Fahd A. Nasr

и другие.

International Journal of Pharmaceutics, Год журнала: 2025, Номер unknown, С. 125492 - 125492

Опубликована: Март 1, 2025

Язык: Английский

Процитировано

1

Enrichment of Trace Selenium in Water Based on Metal−Organic Framework Materials and Reversed−Phase Ultra−High−Performance Liquid Chromatography−Diode Array Determination DOI Creative Commons

H. Cai,

Hongmei Guo, Hantao Jing

и другие.

Separations, Год журнала: 2025, Номер 12(3), С. 62 - 62

Опубликована: Март 9, 2025

A method for the determination of trace selenium in water enriched by metal–organic−framework material (MIL−125−NH2) and reversed−phase ultra−high−performance liquid chromatography−diode array detection (UPLC−DAD) was established. The MIL−125−NH2 material, synthesized microwave method, characterized SEM, XRD, FT−IR. added to sample enrich selenium, desorbed with dilute HCl, then derivative reaction 0.1 mol·L−1 4−nitro−o−phenylenediamine performed produce piaselenole. After extraction cyclohexane, retention time spectrogram were qualitatively detected a detector, peak area quantitatively detected. pH, time, amount extractant, other conditions derivation enrichment optimized experiment, methodology verified under conditions. results showed that linear correlation coefficient R2 0.9998, limit 0.13 μg·L−1 without close ICP−MS after 10−fold 0.013 μg·L−1, RSD 0.7~2.7%, recovery 87.8~102.1%, range 2~1000 μg·L−1. Therefore, can be applied tap water, river mountain spring packaged drinking industrial sewage.

Язык: Английский

Процитировано

0

Enhancing Methanol/Water Activation for Photothermal Hydrogen Production: Modulation of Cu-pyridine Sites in UiO-67 Metal-Organic Frameworks DOI
Shuting Liu,

Ziyu Zengcai,

Jingyao Yang

и другие.

Applied Catalysis B Environment and Energy, Год журнала: 2025, Номер unknown, С. 125376 - 125376

Опубликована: Апрель 1, 2025

Язык: Английский

Процитировано

0

A flexible electrochemical sensor based on paper cellulose fibers network loaded with Mn3O4-UiO-67 for Ultrasensitive detection of methylmercury (MeHg) DOI
Yu Ye, Shunmu Zeng,

Wen Xia

и другие.

Microchemical Journal, Год журнала: 2025, Номер unknown, С. 113778 - 113778

Опубликована: Апрель 1, 2025

Язык: Английский

Процитировано

0

Advances in Green Synthesis and Photo-/Electrocatalytic Applications of Zirconium-Based MOFs: A Review DOI Creative Commons
Tian Zhao, Shilin Peng, Jian Yu

и другие.

Organics, Год журнала: 2025, Номер 6(2), С. 22 - 22

Опубликована: Май 9, 2025

Metal–organic frameworks (MOFs), particularly zirconium-based (Zr-MOFs), have gained significant attention in recent years due to their unique structural and functional properties. This review focuses on eco-friendly synthetic methods for producing Zr-MOFs, addressing the environmental impacts costs associated with conventional synthesis, which often relies hazardous reagents harsh conditions. We explore various green synthesis strategies, including selection of raw materials (such as using zirconium acetate), organic ligands (recycling waste ligand synthesis), (solvothermal, microwave-assisted, ultrasound-assisted, electrochemical, mechanochemical approaches). Additionally, application Zr-MOFs photocatalysis electrocatalysis is examined, highlighting potential purification energy conversion. Despite progress made laboratory settings, challenges remain achieving cost-effectiveness, material stability, scalability industrial applications. Future research should concentrate enhancing efficiency, optimizing catalytic properties, investigating structure–property relationships, expanding applications novel reactions, thus ensuring can contribute sustainable development chemical science technology.

Язык: Английский

Процитировано

0

Transition metal supported UiO-67 materials and their applications in catalysis DOI Creative Commons
Tingting Li, Yan Li, Jingxin Mao

и другие.

Frontiers in Chemistry, Год журнала: 2025, Номер 13

Опубликована: Май 30, 2025

Metal-organic frameworks (MOFs) have emerged as promising platforms for heterogeneous catalysis due to their tunable structures and high specific surface areas. Results indicate that modified composite MOFs not only exhibit superior water stability but also demonstrate broader applicability in catalysis, such Fenton-like oxidation, Morita-Baylis-Hillman reactions, ethylene dimerization, various photoelectrochemical processes. Among them, UiO-67, a zirconium-based MOF, has attracted extensive attention its exceptional chemical stability, catalytic activity, well-defined microporous structure. This review introduces composites formed by different types of single multi-metal loadings on UiO-67 demonstrated performance. It emphasizes the structure-performance relationships these composites, highlighting how metal loading spatial distribution influence reactivity stability. The current application status existing challenges series materials derivatives are systematically reviewed. By integrating experimental results mechanistic insights, this work underscores transformative potential meeting demands sustainable catalysis.

Язык: Английский

Процитировано

0