Self-Healing Thermoset Polyurethanes Driven by Host–Guest Interactions Between α-Cyclodextrin and Poly(ethylene glycol) Monomethyl Ether or Dodecanol Moieties DOI Creative Commons

Ryuji Miyagawa,

Mitsuhiro Shibata

Molecules, Год журнала: 2025, Номер 30(9), С. 1941 - 1941

Опубликована: Апрель 27, 2025

Self-healing thermoset polymers have attracted significant attention because they contribute to resource and energy savings by extending their service life. The reactions between glycerol ethoxylate (GCE), α-cyclodextrin (α-CD), poly(ethylene glycol) monomethyl ether (MPEG), hexamethylene diisocyanate (HDI) at molar ratios of GCE:α-CD:MPEG = a:b:c produced polyurethane networks (GCM-abc, abc 311, 411, 511) containing α-CD MPEG as host guest moieties, respectively. To compare this with GCM-411, 1-dodecanol (DN) was used instead a molecule yield network (GCD-411). Dynamic mechanical analysis revealed the formation polymer network, loss tangent (tan δ) peak temperature (Tα) crosslinking density (νe) decreased increasing GCE fraction for GCMs, Tα νe values GCD were slightly higher than those GCM-411. tensile strength GCMs fraction, GCD-411 that All cured films healed room 24 h, healing efficiency (ησ), based on strength, increased in order GCM-311 < GCM-411 GCM-511 GCD-411. When from 80 °C, ησ 24–38% 45–62%. self-healed thrice treatment gradually each cycle.

Язык: Английский

Solvent-Free Ion-Conductive Xerogels with High Conductivity and Adhesion Enable Multimodal Sensing DOI Creative Commons
Yicheng Zhu,

Yichen Zhou,

Xing Zhang

и другие.

Gels, Год журнала: 2025, Номер 11(4), С. 242 - 242

Опубликована: Март 26, 2025

Ion-conductive gels (ICGs) are essential for achieving human–machine interfaces, bioelectronic applications, or durable wearable sensors. However, traditional solvent-dependent ICGs face bottlenecks such as dehydration-induced failure and challenges in a balance between conductivity mechanical properties. Here, this work developed novel ternary ion-conductive xerogel (PEM-Li ICXG) system based on polyethylene glycol (PEG), poly (2-methoxyethyl acrylate) (PMEA), LiTFSI. PEM-Li ICXGs exhibit high (2.7 × 10−2 S/m), adhesive capability (0.34 MPa), solvent-free characteristics. Remarkably, the incorporation of ions into simultaneously optimizes their performance. We demonstrate application flexible sensors strain temperature sensing. The proposed synthesis strategy is straightforward may further inspire design high-performance ICXGs.

Язык: Английский

Процитировано

0

Eco-friendly, mechanically robust, weather-resistant and rapidly cured polyurea elastomer synthesized by vat photopolymerization 3D printing DOI Creative Commons
Yin Yu, Lisheng Xu, Siqi Liu

и другие.

Composites Part A Applied Science and Manufacturing, Год журнала: 2025, Номер unknown, С. 108985 - 108985

Опубликована: Апрель 1, 2025

Язык: Английский

Процитировано

0

Synthesis of anti-ultraviolet and fluorescent waterborne polyurethanes with highly active plant oil-based internal emulsifiers DOI Creative Commons
Yabin Zhu,

Henghui Deng,

Huizhou Luo

и другие.

Resources Chemicals and Materials, Год журнала: 2025, Номер unknown, С. 100114 - 100114

Опубликована: Апрель 1, 2025

Язык: Английский

Процитировано

0

Self-Healing Thermoset Polyurethanes Driven by Host–Guest Interactions Between α-Cyclodextrin and Poly(ethylene glycol) Monomethyl Ether or Dodecanol Moieties DOI Creative Commons

Ryuji Miyagawa,

Mitsuhiro Shibata

Molecules, Год журнала: 2025, Номер 30(9), С. 1941 - 1941

Опубликована: Апрель 27, 2025

Self-healing thermoset polymers have attracted significant attention because they contribute to resource and energy savings by extending their service life. The reactions between glycerol ethoxylate (GCE), α-cyclodextrin (α-CD), poly(ethylene glycol) monomethyl ether (MPEG), hexamethylene diisocyanate (HDI) at molar ratios of GCE:α-CD:MPEG = a:b:c produced polyurethane networks (GCM-abc, abc 311, 411, 511) containing α-CD MPEG as host guest moieties, respectively. To compare this with GCM-411, 1-dodecanol (DN) was used instead a molecule yield network (GCD-411). Dynamic mechanical analysis revealed the formation polymer network, loss tangent (tan δ) peak temperature (Tα) crosslinking density (νe) decreased increasing GCE fraction for GCMs, Tα νe values GCD were slightly higher than those GCM-411. tensile strength GCMs fraction, GCD-411 that All cured films healed room 24 h, healing efficiency (ησ), based on strength, increased in order GCM-311 < GCM-411 GCM-511 GCD-411. When from 80 °C, ησ 24–38% 45–62%. self-healed thrice treatment gradually each cycle.

Язык: Английский

Процитировано

0