Effect of Thermal Aging on Polyurethane Degradation and the Influence of Unsaturations in the Hard Segment DOI
Manuel Burelo, Edgar Adrián Franco Urquiza, Enrique Martínez‐Franco

и другие.

Journal of Polymer Science, Год журнала: 2025, Номер unknown

Опубликована: Май 16, 2025

ABSTRACT This research focuses on synthesizing two types of polyurethanes (PUs): one with saturated C–C bonds (SPU) and another unsaturated CC (UPU), primarily in the hard segment. Both PUs underwent thermal aging for 30 days at 150°C an air atmosphere to investigate influence unsaturation their degradation. The samples, both before after aging, were characterized using FT‐IR, XRD, TGA, DSC, mechanical testing, SEM. Additionally, percentage weight loss was measured. Similar changes observed SPU UPU aging. Thermal degradation resulted mass losses approximately 5% 10% UPU, accompanied by chemical alterations PUs, as evidenced FT‐IR. Mechanical testing revealed a decline performance materials, notable reductions yield strength elongation break. exhibited more pronounced properties compared SPU. SEM analysis further confirmed surface materials. Among demonstrated higher susceptibility study provides valuable insights into how diols or polyols used PU synthesis influences resulting material properties. findings also highlight potential implications when exposed temperatures exceeding processing operational limits.

Язык: Английский

Innovative self-repairing binders tackling degradation and de-lithiation challenges: Structure, mechanism, high energy and durability DOI
Farshad Boorboor Ajdari,

Fereshteh Abbasi,

Ali Molaei Aghdam

и другие.

Materials Science and Engineering R Reports, Год журнала: 2024, Номер 160, С. 100830 - 100830

Опубликована: Июль 16, 2024

Язык: Английский

Процитировано

6

Investigation on Dynamic and Static Modulus and Creep of Bio-Based Polyurethane-Modified Asphalt Mixture DOI Open Access
Han Biao,

Yongming Xing,

Chao Li

и другие.

Polymers, Год журнала: 2025, Номер 17(3), С. 359 - 359

Опубликована: Янв. 28, 2025

The superior mechanical qualities of polyurethane have garnered increasing attention for its application in modifying asphalt mixtures. However, needs to use polyols cure, and need be produced by petroleum refining. As we all know, is a non-renewable energy source. In order reduce oil consumption conform the trend green economy, lignin chitin were used instead as curing agents. this paper, biological polyurethane-modified mixture (BPA-16) was designed compared with (PA-16) matrix (MA-16). viscoelastic characteristics three mixtures evaluated using dynamic modulus, static creep tests. interplay between modulus frequency examined, along variations correlation modulus. behavior ultimately examined uniaxial load test. findings indicate that BPA-16 exceeds those PA-16 MA-16 8.7% 30.4% at 25 Hz −20 °C, respectively. At 50 phase angle decreases 26.3% relative MA-16. Lignin chitin, when utilized agents place polyol, can enhance stability low temperatures diminish their temperature sensitivity. A bio-based also maintain better elastic properties wider range. −20–20 moduli BPA-16, are linear, they converted formula different frequencies. failure stages PA-16, not observed during 3600 s duration, exhibiting least strain, indicating resistance permanent deformation PU-modified mixes.

Язык: Английский

Процитировано

0

Enhancing the properties and engineering performance of asphalt binders and mixtures with physicochemically treated waste wind turbine blades DOI
Yi Luo,

Jiasheng Huang,

Yijie Wang

и другие.

Construction and Building Materials, Год журнала: 2025, Номер 473, С. 141023 - 141023

Опубликована: Март 31, 2025

Язык: Английский

Процитировано

0

Biopolymers as bitumen additives: a systematic quantitative literature review DOI
Aytuğ Kumandaş, Erhan Burak Pancar, Neslihan Şahan

и другие.

Road Materials and Pavement Design, Год журнала: 2025, Номер unknown, С. 1 - 58

Опубликована: Апрель 3, 2025

Язык: Английский

Процитировано

0

Performance of PTMEG/CO composite polyurethane and modification mechanism of polyurethane-modified asphalt DOI
Xiao Yang,

Jinxiang Hong,

Zijia Xiong

и другие.

Construction and Building Materials, Год журнала: 2025, Номер 475, С. 141117 - 141117

Опубликована: Апрель 11, 2025

Язык: Английский

Процитировано

0

S‐S Vitrimer Composites via Simplified Fabrication: Recyclable Graphite Flakes Simultaneously Enhance Mechanical‐Thermal Properties and Suppress Disulfide Exchange DOI

Wu Xin,

Chao Yan, Ying Hu

и другие.

Macromolecular Chemistry and Physics, Год журнала: 2025, Номер unknown

Опубликована: Апрель 22, 2025

Abstract Vitrimers are covalently crosslinked networks with dynamic bond exchange, where their behavior is typically regulated by adjusting network structures or incorporating fillers. This study introduces graphite flakes (GFs) into sulfur‐containing. to investigate effects on mechanical properties, stress relaxation, and thermal conductivity. The results demonstrate that adding 10 wt.% GFs increases tensile strength 4.37% compared pure epoxy vitrimer, while higher filler content reduces toughness decelerates relaxation. At 160 °C, the characteristic relaxation time rises from 15.35 s (pure vitrimer) 108.85 (40 wt% composite). Arrhenius prefactor ( τ₀ ) decreases loading, whereas activation energy E a remains nearly unaffected. Additionally, 40 enhance diffusivity 110.17% due oriented phonon transport channels. Chemical recycling via DTT solution achieves complete matrix degradation recovery without damaging GFs. provided valuable insights for optimizing vitrimer composites, particularly in enhancing conductivity modulating properties.

Язык: Английский

Процитировано

0

Sustainable fabrication of porous bio-based polyurethane as triboelectric material realized by dynamic bond and scN2 foaming DOI
Xiaodong Zhang, Zhijun Jiang, Xin Zhang

и другие.

Chemical Engineering Journal, Год журнала: 2025, Номер unknown, С. 163012 - 163012

Опубликована: Апрель 1, 2025

Язык: Английский

Процитировано

0

Polyurethanes synthesized from diisocyanate trimers and polyethylene glycol undergo crosslinking via thermally reversible Diels–Alder reactions DOI
Heru Santoso, Sabrina Aufar Salma, Frita Yuliati

и другие.

Macromolecular Research, Год журнала: 2025, Номер unknown

Опубликована: Май 15, 2025

Язык: Английский

Процитировано

0

Effect of Thermal Aging on Polyurethane Degradation and the Influence of Unsaturations in the Hard Segment DOI
Manuel Burelo, Edgar Adrián Franco Urquiza, Enrique Martínez‐Franco

и другие.

Journal of Polymer Science, Год журнала: 2025, Номер unknown

Опубликована: Май 16, 2025

ABSTRACT This research focuses on synthesizing two types of polyurethanes (PUs): one with saturated C–C bonds (SPU) and another unsaturated CC (UPU), primarily in the hard segment. Both PUs underwent thermal aging for 30 days at 150°C an air atmosphere to investigate influence unsaturation their degradation. The samples, both before after aging, were characterized using FT‐IR, XRD, TGA, DSC, mechanical testing, SEM. Additionally, percentage weight loss was measured. Similar changes observed SPU UPU aging. Thermal degradation resulted mass losses approximately 5% 10% UPU, accompanied by chemical alterations PUs, as evidenced FT‐IR. Mechanical testing revealed a decline performance materials, notable reductions yield strength elongation break. exhibited more pronounced properties compared SPU. SEM analysis further confirmed surface materials. Among demonstrated higher susceptibility study provides valuable insights into how diols or polyols used PU synthesis influences resulting material properties. findings also highlight potential implications when exposed temperatures exceeding processing operational limits.

Язык: Английский

Процитировано

0