A novel thermosensitive porous imprinted polymer for selectively separating ReO4 based on Pickering‐like emulsion polymerization DOI

Xianhang Bu,

Zhengcan Chen,

Xiaoyu Lin

и другие.

Journal of Applied Polymer Science, Год журнала: 2024, Номер 141(42)

Опубликована: Авг. 10, 2024

Abstract In this study, we combined the imprinting technique, temperature‐sensitive polymer, and Pickering emulsion polymerization to prepare a porous imprinted polymer. First, block polymer PDEA‐b‐P (DEA‐co‐AM) was prepared by reversible‐addition fragmentation chain transfer polymerization, then ReO 4 − (ReO ‐TPIP) using Pickering‐like which introduced preparation of The structure morphology were characterized FTIR, SEM‐EDS, BET. adsorption experiments showed that maximum (Q), separation (R), desorption (D) ‐TPIP 0.1568 mmol/g, 3.41, 85.22%, respectively, equilibrium could be reached after 120 min, decreased 0.1212 1.23, 70.01% repeated use for 11 times. These results indicate has good reusability properties. studies conformed zero‐level kinetic model in pre‐adsorption stage, quasi‐one‐level late isothermal process more Langmuir model. addition, secondary leach solution high‐temperature alloys, purity rhenium increased from 35.4119% 53.4812% one adsorption/desorption cycle. provides new material strategy selective purification complex rhenium‐containing solutions industry.

Язык: Английский

Date palm fiber agro-waste biomass for efficient removal of 2,4,6-Trichlorophenol from aqueous solution: Characterization, Kinetics, Isotherms studies and Cost-effective analysis DOI Creative Commons
Nadavala Siva Kumar, Mohammad Asif, Anesh Manjaly Poulose

и другие.

Desalination and Water Treatment, Год журнала: 2024, Номер 318, С. 100405 - 100405

Опубликована: Апрель 1, 2024

This study proposes using date palm biomass to remove emerging industrial contaminants, such as 2,4,6-Trichlorophenol (2,4,6-TCP) from water, promoting sustainable waste utilization and a more cost-effective technology. To investigate the potential of raw fiber Triethylamine-modified fibers (RDPF TEA–MDPF) for 2,4,6-TCP removal in batch adsorption experiments. The residual concentration effluents was examined UV-visible spectroscopy. structural chemical composition modified materials determined various techniques, including BET, FTIR, Elemental analyzer (CHN), Particle size analysis, FESEM-EDX, TGA analysis. optimal pH highest uptake capacity equilibrium studies found be 2.0 RDPF 6.0 TEA-MDPF biomass. sorption kinetics onto both adsorbents excellent, designated by pseudo-second-order (R2 = 0.93–0.99) Elovich models 0.86–0.97). indicates that regulated chemisorption. results experiment exhibited good correlation (R2) between PSO maximum (qm) capacities Langmuir isotherm model remediation aqueous media, which 115.50 mg/g 191.75 TEA-MDPF, respectively. exhibits superior compared RDPF, making it promising candidate contaminated wastewater.

Язык: Английский

Процитировано

4

Effects of hydrodynamic cavitation in removal of polycyclic aromatic hydrocarbons (PAHs) from car-wash wastewater DOI Creative Commons
Agnieszka Montusiewicz, Magdalena Lebiocka, Aleksandra Szaja

и другие.

Desalination and Water Treatment, Год журнала: 2025, Номер unknown, С. 101067 - 101067

Опубликована: Фев. 1, 2025

Язык: Английский

Процитировано

0

Eucalyptus wood waste biochar: a green solution for fluoranthene contamination in wastewater DOI

Yu Shuang Ren,

Bekzat Tynybekov, Akmaral Nurmahanova

и другие.

International Journal of Environmental Health Research, Год журнала: 2025, Номер unknown, С. 1 - 14

Опубликована: Апрель 3, 2025

This study investigates the removal of fluoranthene (Flu) from vehicle-wash wastewater (VWW) using biochar (EWB) derived eucalyptus wood waste. Analytical techniques such as surface area analysis (SAA), scanning electron microscopy (SEM), and fourier transform infrared spectroscopy (FT-IR) were employed to characterize EWB. Optimal conditions for Flu adsorption (98.80%) determined 40 ppm initial concentration, 60 minutes contact time, pH 5, 60°C, 0.4 g adsorbent dosage. The process was evaluated kinetic models isotherms, showing that onto EWB follows a pseudo-second order model. Langmuir isotherm provided best fit experimental data. Thermodynamic revealed is exothermic spontaneous, indicated by values entropy (ΔS°), Gibbs free energy (ΔG°), enthalpy (ΔH°). A comparative with commercial adsorbents demonstrated high efficacy in removing industrial wastewater, achieving over 98% efficiency.

Язык: Английский

Процитировано

0

Non-wood-based biochars as promising and eco-friendly adsorbents for chromium hexavalent Cr (VI) removal from aquatic systems: state-of-the-art, limitations, and potential future directions DOI Creative Commons

Ghulam Murtaza,

Muhammad Usman, Zeeshan Ahmed

и другие.

Environmental Pollutants and Bioavailability, Год журнала: 2024, Номер 36(1)

Опубликована: Авг. 14, 2024

Chromium exists from both natural geological processes and human actions, it has a substantial impact on health ecosystems. This study addresses the major challenges in using biochar as an environmentally friendly, sustainable, economical sorbent for removing chromium hexavalent throughout remediation process. The results exhibited that produced non-woody feedstocks pyrolyzed at (300°C −700°C) significantly large amount of various functional groups, higher pH (7 to 11.10) CEC (27 21.70 cmol kg−1), greater surface area (2–300 m2g−1), O/C H/C ratios with increasing carbonization temperature, adsorption capacities (1.63 435 mg g) superior performance removal compared biochars woody-biomass. use equilibrium isotherm, thermodynamic, kinetic models aids comprehending interactions between biochar, well their processes.

Язык: Английский

Процитировано

3

Removal of hydrocarbon pollutants from refinery wastewater using N-hexadecylchitosan as an efficient adsorptive platform DOI Creative Commons
Sher Bahadar Khan,

Zeenat Haram,

Waqas Ahmad

и другие.

Scientific Reports, Год журнала: 2024, Номер 14(1)

Опубликована: Июль 26, 2024

The negative impact of refinery wastewater is great concern to the aquatic, terrestrial, and aerial environment. In this study, N-hexadecylchitosan (NHDC) was successfully synthesized deal with low mechanical strength, poor adsorption capacity, limited selectivity native chitosan. NHDC characterized by fourier-transform infrared spectroscopy (FTIR), scanning electron microscopy (SEM) X-Ray diffraction analysis (XRD) study its composition, morphology, structural attributes. hydrocarbon pollutants from studied in batch mode experiments. results indicated that removal COD attained chitosan 21 63%, respectively. found be maximal, i.e., 96% using 0.08 g at 60 min a solution pH 6.5 maintained °C. Furthermore, kinetic data revealed system followed pseudo-second order kinetics, whereas equilibrium studies supported both monolayer multilayer mechanisms. designed platform able capture under very mild optimized conditions. demonstrated long term stability when subjected five successive cycles, which contributed sustainability water treatment systems. On basis outcome work, it advocated new biobased can used as an efficient adsorbent for remediation organic contaminants laden streams generated oil refineries.

Язык: Английский

Процитировано

1

Characteristics of Removal of Lead, Cadmium and Chromium from Soil Using Biosorbent and Biochar DOI Creative Commons
Paweł Staroń,

Anita Zawadzka,

Piotr Radomski

и другие.

Applied Sciences, Год журнала: 2024, Номер 14(16), С. 7241 - 7241

Опубликована: Авг. 17, 2024

The study proposed the use of aspen wood sawdust and biochar derived from this for removal Pb(II), Cd(II), Cr(VI) ions soil in systems containing single metals as well a mixture all studied metals. effectiveness applied sorbents was compared with sorptive properties activated carbon. results showed that tested materials reduced metal content soil, obtained able to sorb lead, cadmium, chromium both systems. influence type sorbent, its dose, process duration, impact on efficiency sorption capacity analyzed. A statistical analysis also conducted, determining parameters capabilities ions. highest Pb, Cd Cr ion efficiencies were 36-day at sorbent dose 10%. Aspen sawdust, carbon removed 46%, 50% 71% 35%, 43% 53% Cd(II) 15%, 27% 38% Cr(VI), respectively. In turn, values achieved 2%, obtaining 20.2 mg/g, 22.3 mg/g 23.2 5.1 7.9 11.7 3.8 5.8 8.5 It found raw are effective removing toxic which presents potential solution their presence natural environment.

Язык: Английский

Процитировано

1

A novel thermosensitive porous imprinted polymer for selectively separating ReO4 based on Pickering‐like emulsion polymerization DOI

Xianhang Bu,

Zhengcan Chen,

Xiaoyu Lin

и другие.

Journal of Applied Polymer Science, Год журнала: 2024, Номер 141(42)

Опубликована: Авг. 10, 2024

Abstract In this study, we combined the imprinting technique, temperature‐sensitive polymer, and Pickering emulsion polymerization to prepare a porous imprinted polymer. First, block polymer PDEA‐b‐P (DEA‐co‐AM) was prepared by reversible‐addition fragmentation chain transfer polymerization, then ReO 4 − (ReO ‐TPIP) using Pickering‐like which introduced preparation of The structure morphology were characterized FTIR, SEM‐EDS, BET. adsorption experiments showed that maximum (Q), separation (R), desorption (D) ‐TPIP 0.1568 mmol/g, 3.41, 85.22%, respectively, equilibrium could be reached after 120 min, decreased 0.1212 1.23, 70.01% repeated use for 11 times. These results indicate has good reusability properties. studies conformed zero‐level kinetic model in pre‐adsorption stage, quasi‐one‐level late isothermal process more Langmuir model. addition, secondary leach solution high‐temperature alloys, purity rhenium increased from 35.4119% 53.4812% one adsorption/desorption cycle. provides new material strategy selective purification complex rhenium‐containing solutions industry.

Язык: Английский

Процитировано

0