Perspectives for Sustainability Analysis of Scalable Perovskite Photovoltaics
Energy & Environmental Science,
Год журнала:
2024,
Номер
unknown
Опубликована: Янв. 1, 2024
We
propose
a
multi-scale
analytics
and
modeling
framework
to
fill
the
gap
in
integrating
circular
solar
economy
principles
with
ecosystem
climate
commitments,
enabling
holistic
sustainability
analysis
of
perovskite
PVs.
Язык: Английский
Sustainability assessment of rooftop solar photovoltaic systems: A case study
Environmental Impact Assessment Review,
Год журнала:
2024,
Номер
108, С. 107609 - 107609
Опубликована: Июль 24, 2024
Язык: Английский
Life Cycle Assessment of Roll-To-Roll Produced Chemical Vapor Deposition Graphene Transparent Electrodes towards Copper Foil Recycling
Journal of Cleaner Production,
Год журнала:
2024,
Номер
468, С. 143068 - 143068
Опубликована: Авг. 1, 2024
Язык: Английский
Prediction and assessment methods for sustainable solar energy systems within our planetary boundaries: how reliable are they?
Current Opinion in Chemical Engineering,
Год журнала:
2025,
Номер
48, С. 101100 - 101100
Опубликована: Фев. 18, 2025
Язык: Английский
Comparative Life Cycle Assessment of Perovskite Solar Cell Production: Mesoporous n‐i‐p Versus Inverted p‐i‐n Architectures
Advanced Energy and Sustainability Research,
Год журнала:
2025,
Номер
unknown
Опубликована: Март 19, 2025
Perovskite
solar
cells
(PSCs)
offer
a
viable
alternative
to
silicon‐based
technologies.
Assessing
their
environmental
performance
is
essential
for
responsible
development.
This
study
compares
the
life
cycle
impacts
of
two
PSC
architectures,
mesoporous
n‐i‐p
and
inverted
p‐i‐n,
using
assessment
methodology.
The
functional
unit
(FU)
with
an
active
area
2.88
cm
2
.
inventory
uses
primary
production
data
complemented
literature,
EcoInvent
v3.9.1
database,
process
modeling.
Environmental
are
evaluated
ReCiPe
2016
method
in
SimaPro
v9.5.0.1.
Results
indicate
that
producing
PSCs
has
higher
impact
than
PSCs,
due
differences
material
energy
consumption.
Specifically,
require
about
132
MJ/FU
compared
25
leading
carbon
footprints
14.1
kg
CO
eq./FU
2.31
eq./FU,
respectively.
For
consumption
dominates
impacts,
accounting
around
80%
total
impact,
while
depending
on
category,
both
materials
can
dominate.
highlight
critical
could
be
significantly
reduced
by
fully
renewable
electricity
and/or
minimizing
presence
metal
back‐contact.
Язык: Английский
Simultaneous Suppression of Multilayer Ion Migration via Molecular Complexation Strategy toward High‐Performance Regular Perovskite Solar Cells
Angewandte Chemie International Edition,
Год журнала:
2024,
Номер
unknown
Опубликована: Ноя. 4, 2024
The
migration
and
diffusion
of
Li
Язык: Английский
Assessing the Environmental Impact of Pnictogen‐based Perovskite‐Inspired Materials for Indoor Photovoltaics
Advanced Energy Materials,
Год журнала:
2024,
Номер
unknown
Опубликована: Ноя. 17, 2024
Abstract
The
development
of
eco‐friendly
indoor
photovoltaics
(IPVs)
for
Internet‐of‐Things
(IoT)
devices
is
booming.
Emerging
IPVs,
especially
those
based
on
lead
halide
perovskites
(LHPs),
outperform
the
industry
standard
amorphous
hydrogenated
silicon
(a‐Si:H).
However,
toxic
in
LHPs
drives
search
safer
alternatives.
Perovskite‐inspired
materials
(PIMs)
containing
bismuth
(Bi)
and
antimony
(Sb)
have
shown
promise,
achieving
power
conversion
efficiencies
(PCE)
approaching
10%
despite
early
research
stages.
This
promising
due
to
their
eco‐friendlier
light‐harvesting
layers
compared
LHPs.
Yet,
environmental
footprint
pnictogen‐based
PIM
over
lifecycle
remains
unassessed.
study
conducts
a
life‐cycle
assessment
(LCA)
best‐performing
Sb‐
Bi‐PIMs,
considering
PCE,
raw
material
availability,
energy
consumption,
waste
generation.
It
find
that
PCE
plays
decisive
role
identifying
IPVs
with
minimized
impact,
namely
Bi‐Sb
alloy.
Extended
LCA
simulations
industrial‐scale
processing
show
most
Bi‐PIM
has
reduced
burden
a‐Si:H.
also
explore
challenges
solutions
enhancing
Bi‐and
Sb‐PIMs’
sustainability.
Overall,
this
provides
first
evidence
potential
PIMs
as
sustainable
IPV
technology,
addressing
whether
lead‐free
are
truly
eco‐friendly,
thus
contributing
toward
battery‐less
IoT
applications.
Язык: Английский
Simultaneous Suppression of Multilayer Ion Migration via Molecular Complexation Strategy toward High‐Performance Regular Perovskite Solar Cells
Angewandte Chemie,
Год журнала:
2024,
Номер
unknown
Опубликована: Ноя. 4, 2024
Abstract
The
migration
and
diffusion
of
Li
+
,
I
−
Ag
impedes
the
realization
long‐term
operationally
stable
perovskite
solar
cells
(PSCs).
Herein,
we
report
a
multifunctional
universal
molecular
complexation
strategy
to
simultaneously
stabilize
hole
transport
layer
(HTL),
electrode
by
suppression
via
directly
incorporating
bis(2,4,6‐trichlorophenyl)
oxalate
(TCPO)
into
HTL.
Meanwhile,
TCPO
co‐doping
results
in
enhanced
mobility
HTL,
advantageous
energy
band
alignment
mitigated
interfacial
defects,
thereby
leading
facilitated
extraction
minimized
nonradiative
recombination
losses.
TCPO‐doped
regular
device
achieves
peak
power
conversion
efficiency
(PCE)
25.68
%
(certified
25.59
%).
unencapsulated
doped
devices
maintain
over
90
their
initial
efficiencies
after
730
h
continuous
operation
under
one
sun
illumination,
2800
storage
at
30
relative
humidity,
1200
exposure
65
°C,
which
represents
best
stabilities
reported
for
PSCs.
This
work
provides
new
approach
enhance
PCE
stability
PSCs
host–guest
rational
design
ligand
molecules.
Язык: Английский