Construction of a Novel Hydrogen-Bond-Assisted Bisulfide Nonmetallic Active Center for Solar Ammonia Fertilizer Production DOI
Wei Cai, Hongbo Jiang,

Qin Zhong

и другие.

ACS Sustainable Chemistry & Engineering, Год журнала: 2024, Номер unknown

Опубликована: Дек. 4, 2024

Solar-driven photocatalytic nitrogen reduction is a promising and effective way to produce NH3 in sustainable manner. The reaction product, ammonium-based nitrogen, can mimic biological fixation for plant growth replace the use of exogenous fertilizers. To address bottleneck N2 activation during reduction, catalyst dithiosalicylic acid (DTSA) with hydrogen-bond-assisted S–S nonmetallic active center was constructed by thiosalicylic this study, which achieved an ammonia yield 278.9 μmol/h/gcat..The innovative application catalytic product as replacement fertilizer Chlorella resulted significant increase concentration without yellowing algal filaments compared blank control group, indicating adequate supply functioning Further mechanistic studies reveal alternating pathway at center. energy barrier rate-determining step (RDS) effectively reduced from 2.79 2.11 eV aid intermolecular hydrogen bonding DTSA. controllable mass production simple synthesis, used cultivation opportunity development NRR catalysts solar Furthermore, proposed novel provides new idea direction future catalysts.

Язык: Английский

Insight into the effect of support properties on DBD plasma-catalytic NH3 synthesis over Ru-Co bimetallic catalysts DOI
Bo Gao, Guoqiang Cao, Donghai Hu

и другие.

Fuel, Год журнала: 2024, Номер 382, С. 133802 - 133802

Опубликована: Ноя. 21, 2024

Язык: Английский

Процитировано

1

Ammonia Can Be Currently Considered One of the Best Green Energy Allies DOI Creative Commons
Rubén González, Xiomar Gómez

Sustainable Chemistry, Год журнала: 2024, Номер 5(2), С. 163 - 195

Опубликована: Июнь 19, 2024

Ammonia can be considered a relevant compound in the future energy sector, playing significant role as an carrier, storage, or carbon-free fuel. However, production of this molecule has high demand, and use natural gas, which is not free controversy due to accidental leakage into atmosphere produced during extraction fact that it nonrenewable source, contributes increasing greenhouse gas emissions. Reducing process’s demand carbon footprint will essential making ammonia clear alternative for economy. Given vast research handling, seems logical step forward evolution sector. current uncertainty global market requires cautiousness decision making. Several factors may impact economic growth human welfare, thus needing careful assessment before any transcendental decisions could affect worldwide prices raw material availability.

Язык: Английский

Процитировано

0

Construction of a Novel Hydrogen-Bond-Assisted Bisulfide Nonmetallic Active Center for Solar Ammonia Fertilizer Production DOI
Wei Cai, Hongbo Jiang,

Qin Zhong

и другие.

ACS Sustainable Chemistry & Engineering, Год журнала: 2024, Номер unknown

Опубликована: Дек. 4, 2024

Solar-driven photocatalytic nitrogen reduction is a promising and effective way to produce NH3 in sustainable manner. The reaction product, ammonium-based nitrogen, can mimic biological fixation for plant growth replace the use of exogenous fertilizers. To address bottleneck N2 activation during reduction, catalyst dithiosalicylic acid (DTSA) with hydrogen-bond-assisted S–S nonmetallic active center was constructed by thiosalicylic this study, which achieved an ammonia yield 278.9 μmol/h/gcat..The innovative application catalytic product as replacement fertilizer Chlorella resulted significant increase concentration without yellowing algal filaments compared blank control group, indicating adequate supply functioning Further mechanistic studies reveal alternating pathway at center. energy barrier rate-determining step (RDS) effectively reduced from 2.79 2.11 eV aid intermolecular hydrogen bonding DTSA. controllable mass production simple synthesis, used cultivation opportunity development NRR catalysts solar Furthermore, proposed novel provides new idea direction future catalysts.

Язык: Английский

Процитировано

0