Enabling highly reversible Zn anode via an interfacial preferentially adsorbed additive containing nucleophilic groups DOI Open Access
Canglong Li,

Hongli Qi,

Jie Huang

и другие.

Microstructures, Год журнала: 2025, Номер 5(2)

Опубликована: Март 21, 2025

The cyclability and reversibility of aqueous zinc-ion batteries (AZIBs) are severely hampered by the safety concerns arising from Zn dendrite growth. Therefore, a stable anode with inhibited dendrites side reactions is crucial for AZIBs. Herein, we utilized methyl acetoacetate (MA) as an additive to prevent growth enable highly reversible anodes. Benefiting nucleophilic groups (carbonyl groups) in MA, MA molecules can preferentially adsorb on anode/electrolyte interface (AEI), forming molecular protective layer. Such layers not only regulate migration deposition zinc ions, but also inhibit induced decomposition free H2O at AEI. symmetric cell addition achieves long-term cycling stability 1,500 h 2 mA cm-2 capacity mAh cm-2. In addition, Zn//NVO full using MA-contained electrolyte demonstrates high specific (138.4 g-1) outstanding retention (92.8% after 600 cycles) 1 A g-1. This work provides principle use ester-based additives suppress durable metal

Язык: Английский

Interfacial dual-modulation through deoxygenation effect and tuning hydrogen-bonding environment toward highly reversible Zn metal anodes DOI
Canglong Li,

Xiaozhi Jiang,

Hongli Qi

и другие.

Energy storage materials, Год журнала: 2025, Номер 75, С. 104012 - 104012

Опубликована: Янв. 9, 2025

Язык: Английский

Процитировано

13

Accelerating Desolvation Process and Achieving Dendrite‐Free Zn Anode Via Dielectric Filler‐assisted Artificial Hybrid Interphase DOI Open Access
Canglong Li, Jie Huang, Dong‐Ping Chen

и другие.

Advanced Sustainable Systems, Год журнала: 2025, Номер unknown

Опубликована: Фев. 2, 2025

Abstract Aqueous zinc‐ion batteries (AZIBs) have garnered significant interest for their potential in large‐scale energy storage, attributed to high safety and low cost. Nonetheless, issues such as limited cycling lifespan coulombic efficiency (CE) associated with dendrite formation uncontrollable side reactions on the Zn metal anode pose challenges that restrict practical applications. Herein, a dielectric filler‐assisted artificial hybrid interphase is constructed surface address faced by aqueous electrolytes. TiO 2 nanoparticles special properties promote solvation process carboxymethyl cellulose (CMC) acts physical barrier suppressing adverse blocking dendrite. Consequently, symmetric cell using modified zinc achieves prolonged cycle life of over 2500 h at 1 mAh cm −2 . Furthermore, full vanadium‐based cathode delivers excellent electrochemical performance (over 600 cycles A g −1 ). This research offers an efficient scalable approach enhance anodes.

Язык: Английский

Процитировано

2

Synergy of constructing robust hybrid interphase and weakly solvating electrolyte for low-temperature aqueous zinc-ion batteries DOI
Wen Liu,

Qiwen Zhao,

Hongli Qi

и другие.

Chinese Chemical Letters, Год журнала: 2025, Номер unknown, С. 110893 - 110893

Опубликована: Янв. 1, 2025

Язык: Английский

Процитировано

0

MOF-based electrode materials for aqueous zinc-ion batteries: design strategy and future challenges DOI
Yingying Wang,

Tao Pan,

Sicong Zhang

и другие.

Inorganic Chemistry Frontiers, Год журнала: 2025, Номер unknown

Опубликована: Янв. 1, 2025

Summary of MOF-based aqueous zinc-ion battery electrode materials design strategies.

Язык: Английский

Процитировано

0

Hydrogen bonding-reinforced multi-component cross-linked hydrogel electrolytes with high ionic conductivity and stretchability for stabilized zinc anodes DOI
Yusheng Wang, Kun Ding,

Xuerong Gong

и другие.

Chinese Chemical Letters, Год журнала: 2025, Номер unknown, С. 111078 - 111078

Опубликована: Март 1, 2025

Язык: Английский

Процитировано

0

Enabling highly reversible Zn anode via an interfacial preferentially adsorbed additive containing nucleophilic groups DOI Open Access
Canglong Li,

Hongli Qi,

Jie Huang

и другие.

Microstructures, Год журнала: 2025, Номер 5(2)

Опубликована: Март 21, 2025

The cyclability and reversibility of aqueous zinc-ion batteries (AZIBs) are severely hampered by the safety concerns arising from Zn dendrite growth. Therefore, a stable anode with inhibited dendrites side reactions is crucial for AZIBs. Herein, we utilized methyl acetoacetate (MA) as an additive to prevent growth enable highly reversible anodes. Benefiting nucleophilic groups (carbonyl groups) in MA, MA molecules can preferentially adsorb on anode/electrolyte interface (AEI), forming molecular protective layer. Such layers not only regulate migration deposition zinc ions, but also inhibit induced decomposition free H2O at AEI. symmetric cell addition achieves long-term cycling stability 1,500 h 2 mA cm-2 capacity mAh cm-2. In addition, Zn//NVO full using MA-contained electrolyte demonstrates high specific (138.4 g-1) outstanding retention (92.8% after 600 cycles) 1 A g-1. This work provides principle use ester-based additives suppress durable metal

Язык: Английский

Процитировано

0