Light Absorption and Chromophore Characteristics of Brown Carbon in PM Emitted From Agricultural Machinery in China DOI
Xinyi Wan,

Yubao Chen,

Fan Zhang

и другие.

Journal of Geophysical Research Atmospheres, Год журнала: 2025, Номер 130(11)

Опубликована: Май 28, 2025

Abstract The extensive utilization of agricultural machinery in China has made it a prominent contributor to particulate matter (PM). However, there still exist significant knowledge gaps understanding optical characteristics and molecular composition chromophores brown carbon (BrC) PM emitted from machinery. Therefore, BrC six typical machines were measured investigate the light absorption, chromophore characteristics, influencing factors. Results showed that average emission factors methanol‐soluble organic (MSOC) water‐soluble (WSOC) 0.96 0.21 g (kg fuel) −1 , respectively, exhibiting clear decreasing trends with increasing engine power improving standards. Despite absorption coefficient methanol‐extracted (Abs 365,M ) being approximately 2.2 times higher than water 365,W ), mass efficiency water‐extracted (MAE exhibited significantly greater values MAE . Among detected chromophores, nitro‐aromatic compounds (NACs) highest contribution was about 14.5 more total compared their contributions MSOC (0.04%), followed by polycyclic aromatic hydrocarbons (PAHs) oxygenated PAHs (OPAHs). Besides, integrated simple forcing estimated be 1.5 W for 3.7 WSOC, indicating radiative findings this study not only provide fundamental data climate impact estimation but also propose effective strategies mitigate emissions, such as enhancing standards promoting adoption high‐power

Язык: Английский

A European aerosol phenomenology – 9: Light absorption properties of carbonaceous aerosol particles across surface Europe DOI Creative Commons
Jordi Rovira, Marjan Savadkoohi, Gang Chen

и другие.

Environment International, Год журнала: 2024, Номер 195, С. 109185 - 109185

Опубликована: Дек. 9, 2024

Carbonaceous aerosols (CA), composed of black carbon (BC) and organic matter (OM), significantly impact the climate. Light absorption properties CA, particularly BC brown (BrC), are crucial due to their contribution global regional warming. We present (b

Язык: Английский

Процитировано

4

Influence of ship emitted sulfur and carbonaceous aerosols on East Asian climate in summer DOI
Bingliang Zhuang,

Yinan Zhou,

Yaxin Hu

и другие.

Atmospheric Environment, Год журнала: 2025, Номер 344, С. 121035 - 121035

Опубликована: Янв. 10, 2025

Язык: Английский

Процитировано

0

Global distribution and warming effect of brown carbon from shipping emissions DOI Creative Commons
Yiyang Sun, Junjun Deng, Fan Zhang

и другие.

Carbon Research, Год журнала: 2025, Номер 4(1)

Опубликована: Май 20, 2025

Abstract Emissions of shipping have great influences on atmospheric environment and global climate with the growth maritime trade. Previous studies identified that black carbon (BC) constitutes main aerosol component responsible for light absorption, while organic (OC) was generally considered non-absorbing. Recent indicated components derived from emissions exhibit absorption at short wavelengths (brown carbon, BrC). However, there is a lack quantification regarding effects BrC. This study investigates radiative effect (RAE) BrC, updating models measured BrC ability. Surface concentrations contribute ~ 40% to fossil fuel OC. The annual average RAE +0.15 +0.36 mW m⁻ 2 , peaking in boreal summer. warming 8%–19% relative BC. With low-sulfur standard, increases +0.52 which close BC (+0.52 ) could offset direct cooling sulfate. For aerosols, an important part, whose contribution greater upgrade ship fuels. Graphical

Язык: Английский

Процитировано

0

Light Absorption and Chromophore Characteristics of Brown Carbon in PM Emitted From Agricultural Machinery in China DOI
Xinyi Wan,

Yubao Chen,

Fan Zhang

и другие.

Journal of Geophysical Research Atmospheres, Год журнала: 2025, Номер 130(11)

Опубликована: Май 28, 2025

Abstract The extensive utilization of agricultural machinery in China has made it a prominent contributor to particulate matter (PM). However, there still exist significant knowledge gaps understanding optical characteristics and molecular composition chromophores brown carbon (BrC) PM emitted from machinery. Therefore, BrC six typical machines were measured investigate the light absorption, chromophore characteristics, influencing factors. Results showed that average emission factors methanol‐soluble organic (MSOC) water‐soluble (WSOC) 0.96 0.21 g (kg fuel) −1 , respectively, exhibiting clear decreasing trends with increasing engine power improving standards. Despite absorption coefficient methanol‐extracted (Abs 365,M ) being approximately 2.2 times higher than water 365,W ), mass efficiency water‐extracted (MAE exhibited significantly greater values MAE . Among detected chromophores, nitro‐aromatic compounds (NACs) highest contribution was about 14.5 more total compared their contributions MSOC (0.04%), followed by polycyclic aromatic hydrocarbons (PAHs) oxygenated PAHs (OPAHs). Besides, integrated simple forcing estimated be 1.5 W for 3.7 WSOC, indicating radiative findings this study not only provide fundamental data climate impact estimation but also propose effective strategies mitigate emissions, such as enhancing standards promoting adoption high‐power

Язык: Английский

Процитировано

0