Target and Nontarget Analysis of Organophosphorus Flame Retardants and Plasticizers in a River Impacted by Industrial Activity in Eastern China DOI
Yilin Wu, Yiming Yao, Shijie Chen

и другие.

Environmental Science & Technology, Год журнала: 2024, Номер unknown

Опубликована: Дек. 26, 2024

Industrial activities are a major source of organophosphorus flame retardants (OPFRs) and plasticizers in aquatic environments. This study investigated the distribution 40 OPFRs river impacted by industrial manufacturing plants Eastern China target analysis. Nontarget analysis using high-resolution mass spectrometry was further employed to identify novel compounds (NOPs). Thirty-four were detected water samples, with total concentrations 62.9–1.06 × 103 ng/L (median: 455 ng/L). Triphenylphosphine oxide diphenyl phosphoric acid ubiquitously up 620 127 ng/L, respectively. Among 26 identified NOPs, 17 reported for first time environment, including 14 organophosphate esters (especially 4 heterocycles 3 oligomers), 2 organophosphites, an organophosphonate. Bis(2,4-di-tert-butylphenyl) hydrogen phosphate 2,2-dimethylpropoxy(propyl)phosphinic high predicted persistence or toxicity widely detected, semiquantified 990 1.0 Structurally similar exhibited consistent variation trends, suggesting common emission source. Estimated annual discharges sea 20.6–37.0 kg/yr 30.8–161 NOPs. These findings indicate that contribute NOPs catchment its estuary, posing ecological risks both terrestrial marine

Язык: Английский

Detection and screening of organophosphate esters in infant formula from Shanghai, China: distribution characteristics and risk evaluation DOI

Ruiqi Du,

Jing Zhou,

Shenping Zhang

и другие.

Food Additives & Contaminants Part A, Год журнала: 2025, Номер unknown, С. 1 - 14

Опубликована: Фев. 6, 2025

Organophosphate esters (OPEs) have raised great concerns in recent years. However, information regarding their occurrence infant formula remains limited. Thus, thirty-two OPEs were measured sold Shanghai, China 2023. The results showed that OPE was widespread. median concentrations of organophosphate diesters, triesters, and total 2.28, 5.20, 8.63 ng/g, respectively. Tris(2-chloroisopropyl) phosphate (TCPP) the highest concentration (1.95 ng/g), followed by triethyl phosphate, bis(1-chloro-2-propyl) (BCPP), tri-isobutyl triphenyl (0.532-0.581 ng/g). dominant chloro-OPEs (TCPP BCPP) regional-specific. Compared to corresponding diester often lower, except for bis(2-butoxyethyl) tributoxyethyl phosphate. Additionally, five novel with phenyl groups identified, showing high detection frequencies comparable TCPP. Raw materials food processing methods might affect individual OPEs. estimated daily intakes (EDIs) ranged from 62.3 355 ng/kg bw/day. EDI occurred infants 0-6 months age but posed no obvious health risk toddlers. Further studies are still needed evaluate possible implications arising metabolites, as well potentially synergistic effects.

Язык: Английский

Процитировано

0

Affecting factors and health risks of organophosphate esters in urban soil and surface dust in a typical river valley city based on local bivariate Moran's I and Monte-Carlo simulation DOI
Qian Zhang, Lijun Wang

Journal of Hazardous Materials, Год журнала: 2024, Номер 481, С. 136534 - 136534

Опубликована: Ноя. 16, 2024

Язык: Английский

Процитировано

1

Unveiling the mechanistic in benzoic acid-enhanced hydrated electron reactivity: Synergistic degradation of organic phosphorus flame retardant precursors in UV/sulfite process DOI

Yuxin Guo,

Feifeng Wang,

Zhilei Lu

и другие.

Separation and Purification Technology, Год журнала: 2024, Номер unknown, С. 131323 - 131323

Опубликована: Дек. 1, 2024

Язык: Английский

Процитировано

1

Target and Nontarget Analysis of Organophosphorus Flame Retardants and Plasticizers in a River Impacted by Industrial Activity in Eastern China DOI
Yilin Wu, Yiming Yao, Shijie Chen

и другие.

Environmental Science & Technology, Год журнала: 2024, Номер unknown

Опубликована: Дек. 26, 2024

Industrial activities are a major source of organophosphorus flame retardants (OPFRs) and plasticizers in aquatic environments. This study investigated the distribution 40 OPFRs river impacted by industrial manufacturing plants Eastern China target analysis. Nontarget analysis using high-resolution mass spectrometry was further employed to identify novel compounds (NOPs). Thirty-four were detected water samples, with total concentrations 62.9–1.06 × 103 ng/L (median: 455 ng/L). Triphenylphosphine oxide diphenyl phosphoric acid ubiquitously up 620 127 ng/L, respectively. Among 26 identified NOPs, 17 reported for first time environment, including 14 organophosphate esters (especially 4 heterocycles 3 oligomers), 2 organophosphites, an organophosphonate. Bis(2,4-di-tert-butylphenyl) hydrogen phosphate 2,2-dimethylpropoxy(propyl)phosphinic high predicted persistence or toxicity widely detected, semiquantified 990 1.0 Structurally similar exhibited consistent variation trends, suggesting common emission source. Estimated annual discharges sea 20.6–37.0 kg/yr 30.8–161 NOPs. These findings indicate that contribute NOPs catchment its estuary, posing ecological risks both terrestrial marine

Язык: Английский

Процитировано

0