Nature Synthesis,
Год журнала:
2024,
Номер
3(5), С. 606 - 614
Опубликована: Апрель 9, 2024
Abstract
Efficient
synthesis
recipes
are
needed
to
streamline
the
manufacturing
of
complex
materials
and
accelerate
realization
theoretically
predicted
materials.
Often,
solid-state
multicomponent
oxides
is
impeded
by
undesired
by-product
phases,
which
can
kinetically
trap
reactions
in
an
incomplete
non-equilibrium
state.
Here
we
report
a
thermodynamic
strategy
navigate
high-dimensional
phase
diagrams
search
precursors
that
circumvent
low-energy,
competing
by-products,
while
maximizing
reaction
energy
drive
fast
transformation
kinetics.
Using
robotic
inorganic
laboratory,
perform
large-scale
experimental
validation
our
precursor
selection
principles.
For
set
35
target
quaternary
oxides,
with
chemistries
representative
intercalation
battery
cathodes
electrolytes,
robot
performs
224
spanning
27
elements
28
unique
precursors,
operated
1
human
experimentalist.
Our
frequently
yield
higher
purity
than
traditional
precursors.
Robotic
laboratories
offer
exciting
platform
for
data-driven
science,
from
develop
fundamental
insights
guide
both
chemists.
World Journal of Advanced Research and Reviews,
Год журнала:
2024,
Номер
21(1), С. 2009 - 2020
Опубликована: Янв. 25, 2024
The
integration
of
embedded
systems
in
autonomous
vehicles
represents
a
transformative
paradigm
shift
the
automotive
industry,
offering
unprecedented
opportunities
for
enhanced
safety,
efficiency,
and
user
experience.
This
comprehensive
review
explores
current
landscape
vehicles,
delving
into
emerging
trends,
persistent
challenges,
future
directions
that
shape
trajectory
this
rapidly
evolving
field.
begins
by
examining
foundational
concepts
context
elucidating
intricate
interplay
between
hardware
software
components.
It
surveys
state-of-the-art
technologies
empower
these
systems,
including
advanced
sensors,
actuators,
communication
protocols,
highlighting
their
pivotal
roles
perception,
decision-making,
control
aspects
driving.
One
prominent
trends
discussed
is
increasing
reliance
on
artificial
intelligence
(AI)
machine
learning
algorithms
within
systems.
incorporation
intelligent
enables
to
adapt
learn
from
real-world
scenarios,
enhancing
ability
navigate
diverse
dynamic
environments.
Additionally,
sheds
light
growing
emphasis
connectivity
edge
computing,
illustrating
how
leverage
facilitate
seamless
surrounding
infrastructure.
Despite
promising
advancements,
critically
examines
challenges
impede
widespread
adoption
vehicles.
Issues
such
as
safety
concerns,
cybersecurity
threats,
regulatory
frameworks
are
analyzed,
providing
insights
complex
ecosystem
which
operate.
In
addressing
envisions
marked
continuous
innovation
collaboration
across
industries.
anticipates
evolution
towards
more
robust,
adaptive,
fault-tolerant
architectures,
paving
way
increased
autonomy
deployment
provides
holistic
understanding
encapsulating
directions.
As
undergoes
shift,
serves
valuable
resource
researchers,
practitioners,
policymakers
seeking
terrain
vehicle
technology.
Contemporary
materials
discovery
requires
intricate
sequences
of
synthesis,
formulation,
and
characterization
that
often
span
multiple
locations
with
specialized
expertise
or
instrumentation.
To
accelerate
these
workflows,
we
present
a
cloud-based
strategy
enabled
delocalized
asynchronous
design-make-test-analyze
cycles.
We
showcased
this
approach
through
the
exploration
molecular
gain
for
organic
solid-state
lasers
as
frontier
application
in
optoelectronics.
Distributed
robotic
synthesis
in-line
property
characterization,
orchestrated
by
artificial
intelligence
experiment
planner,
resulted
21
new
state-of-the-art
materials.
Gram-scale
ultimately
allowed
verification
best-in-class
stimulated
emission
thin-film
device.
Demonstrating
integration
five
laboratories
across
globe,
workflow
provides
blueprint
delocalizing-and
democratizing-scientific
discovery.
Nature Communications,
Год журнала:
2024,
Номер
15(1)
Опубликована: Янв. 23, 2024
Abstract
The
ability
to
integrate
resources
and
share
knowledge
across
organisations
empowers
scientists
expedite
the
scientific
discovery
process.
This
is
especially
crucial
in
addressing
emerging
global
challenges
that
require
solutions.
In
this
work,
we
develop
an
architecture
for
distributed
self-driving
laboratories
within
World
Avatar
project,
which
seeks
create
all-encompassing
digital
twin
based
on
a
dynamic
graph.
We
employ
ontologies
capture
data
material
flows
design-make-test-analyse
cycles,
utilising
autonomous
agents
as
executable
components
carry
out
experimentation
workflow.
Data
provenance
recorded
ensure
its
findability,
accessibility,
interoperability,
reusability.
demonstrate
practical
application
of
our
framework
by
linking
two
robots
Cambridge
Singapore
collaborative
closed-loop
optimisation
pharmaceutically-relevant
aldol
condensation
reaction
real-time.
graph
autonomously
evolves
toward
scientist’s
research
goals,
with
effectively
generating
Pareto
front
cost-yield
three
days.
Nature Communications,
Год журнала:
2024,
Номер
15(1)
Опубликована: Май 21, 2024
Abstract
Energy
absorbing
efficiency
is
a
key
determinant
of
structure’s
ability
to
provide
mechanical
protection
and
defined
by
the
amount
energy
that
can
be
absorbed
prior
stresses
increasing
level
damages
system
protected.
Here,
we
explore
additively
manufactured
polymer
structures
using
self-driving
lab
(SDL)
perform
>25,000
physical
experiments
on
generalized
cylindrical
shells.
We
use
human-SDL
collaborative
approach
where
are
selected
from
over
trillions
candidates
in
an
11-dimensional
parameter
space
Bayesian
optimization
then
automatically
performed
while
human
team
monitors
progress
periodically
modify
aspects
system.
The
result
this
campaign
discovery
structure
with
75.2%
library
experimental
data
reveals
transferable
principles
for
designing
tough
structures.
Nature Synthesis,
Год журнала:
2024,
Номер
3(5), С. 606 - 614
Опубликована: Апрель 9, 2024
Abstract
Efficient
synthesis
recipes
are
needed
to
streamline
the
manufacturing
of
complex
materials
and
accelerate
realization
theoretically
predicted
materials.
Often,
solid-state
multicomponent
oxides
is
impeded
by
undesired
by-product
phases,
which
can
kinetically
trap
reactions
in
an
incomplete
non-equilibrium
state.
Here
we
report
a
thermodynamic
strategy
navigate
high-dimensional
phase
diagrams
search
precursors
that
circumvent
low-energy,
competing
by-products,
while
maximizing
reaction
energy
drive
fast
transformation
kinetics.
Using
robotic
inorganic
laboratory,
perform
large-scale
experimental
validation
our
precursor
selection
principles.
For
set
35
target
quaternary
oxides,
with
chemistries
representative
intercalation
battery
cathodes
electrolytes,
robot
performs
224
spanning
27
elements
28
unique
precursors,
operated
1
human
experimentalist.
Our
frequently
yield
higher
purity
than
traditional
precursors.
Robotic
laboratories
offer
exciting
platform
for
data-driven
science,
from
develop
fundamental
insights
guide
both
chemists.