A Comprehensive and Robust Multiplex-DIA Workflow Profiles Protein Turnover Regulations Associated with Cisplatin Resistance DOI Creative Commons
Barbora Šalovská, Wenxue Li, Oliver M. Bernhardt

и другие.

bioRxiv (Cold Spring Harbor Laboratory), Год журнала: 2024, Номер unknown

Опубликована: Окт. 31, 2024

Summary Measuring protein turnover is essential for understanding cellular biological processes and advancing drug discovery. The multiplex DIA mass spectrometry (DIA-MS) approach, combined with dynamic SILAC labeling (pulse-SILAC, or pSILAC), has proven to be a reliable method analyzing degradation kinetics. Previous DIA-MS workflows have employed various strategies, including leveraging the highest isotopic channels of peptides enhance detection MS signal pairs clusters. In this study, we introduce an improved robust workflow that integrates novel machine learning strategy channel-specific statistical filtering, enabling adaptation systematic temporal variations in channel ratios. This allows comprehensive profiling throughout pSILAC experiment without relying solely on signals. Additionally, developed KdeggeR , data processing analysis package optimized pSILAC-DIA experiments, which estimates visualizes peptide rates profiles. Our integrative was benchmarked both 2-channel 3-channel standard datasets aneuploid cancer cell model before after cisplatin resistance development demonstrated strong negative correlation between transcript regulation major complex subunits. We also identified specific signatures associated resistance.

Язык: Английский

Single-nucleus proteomics identifies regulators of protein transport DOI Creative Commons
Jason Derks,

Tobias Jonson,

Andrew Leduc

и другие.

bioRxiv (Cold Spring Harbor Laboratory), Год журнала: 2024, Номер unknown

Опубликована: Июнь 18, 2024

The physiological response of a cell to stimulation depends on its proteome configuration. Therefore, the abundance variation regulatory proteins across unstimulated single cells can be associatively linked with their stimulation. Here we developed an approach that leverages this association individual and nuclei systematically identify potential regulators biological processes, followed by targeted validation. Specifically, applied nucleocytoplasmic protein transport in macrophages stimulated lipopolysaccharide (LPS). To end, quantified proteomes 3,412 nuclei, sampling dynamic LPS treatment, linking functional variability proteomic variability. Minutes after stimulation, correlated strongly known regulators, thus revealing impact natural cellular response. We found simple biophysical constraints, such as quantity nuclear pores, partially explain LPS-induced transport. Among many newly identified associated response, selected 16 for validation knockdown. knockdown phenotypes confirmed inferences derived from demonstrating (sub-)single-cell proteomics infer regulation. expect generalize broad applications enhance interpretability single-cell omics data.

Язык: Английский

Процитировано

4

Revealing the dynamics of fungal disease with proteomics DOI Creative Commons

Mazmanian Sa,

Manuela Silva, Brianna Ball

и другие.

Molecular Omics, Год журнала: 2025, Номер unknown

Опубликована: Янв. 1, 2025

The occurrence and distribution of new re-emerging fungal pathogens, along with rates antifungal resistance, are rising across the globe, correspondingly, so our awareness call for action to address this public health concern. To effectively detect, monitor, treat infections, biological insights into mechanisms that regulate pathogenesis, influence survival, promote resistance urgently needed. Mass spectrometry-based proteomics is a high-resolution technique enables identification quantification proteins diverse systems better understand biology driving phenotypes. In review, we highlight dynamic innovative applications characterize three critical pathogens (i.e., Candida spp., Cryptococcus Aspergillus spp.) causing disease in humans. We present strategies investigate host-pathogen interface, virulence factor production, protein-level drivers resistance. Through these studies, opportunities biomarker development, drug target discovery, immune system remodeling discussed, supporting use combat plethora diseases threatening global health.

Язык: Английский

Процитировано

0

Global analysis of protein turnover dynamics in single cells DOI Creative Commons
Pierre Sabatier, Maico Lechner, Ulises H. Guzmán

и другие.

Cell, Год журнала: 2025, Номер unknown

Опубликована: Март 1, 2025

Single-cell proteomics (SCPs) has advanced significantly, yet it remains largely unidimensional, focusing primarily on protein abundances. In this study, we employed a pulsed stable isotope labeling by amino acids in cell culture (pSILAC) approach to simultaneously analyze abundance and turnover single cells (SC-pSILAC). Using state-of-the-art SCP workflow, demonstrated that two SILAC labels are detectable from ∼4,000 proteins HeLa recapitulating known biology. We performed large-scale time-series SC-pSILAC analysis of undirected differentiation human induced pluripotent stem (iPSCs) encompassing 6 sampling times over 2 months analyzed >1,000 cells. Protein dynamics highlighted differentiation-specific co-regulation complexes with core histone turnover, discriminating dividing non-dividing Lastly, correlating diameter the individual showed histones some cell-cycle do not scale size. The method provides multidimensional view single-cell

Язык: Английский

Процитировано

0

The plant proteome delivers from discovery to innovation DOI
Jennifer Geddes‐McAlister, R. Glen Uhrig

Trends in Plant Science, Год журнала: 2025, Номер unknown

Опубликована: Апрель 1, 2025

Язык: Английский

Процитировано

0

A Comprehensive and Robust Multiplex-DIA Workflow Profiles Protein Turnover Regulations Associated with Cisplatin Resistance DOI Creative Commons
Barbora Šalovská, Wenxue Li, Oliver M. Bernhardt

и другие.

bioRxiv (Cold Spring Harbor Laboratory), Год журнала: 2024, Номер unknown

Опубликована: Окт. 31, 2024

Summary Measuring protein turnover is essential for understanding cellular biological processes and advancing drug discovery. The multiplex DIA mass spectrometry (DIA-MS) approach, combined with dynamic SILAC labeling (pulse-SILAC, or pSILAC), has proven to be a reliable method analyzing degradation kinetics. Previous DIA-MS workflows have employed various strategies, including leveraging the highest isotopic channels of peptides enhance detection MS signal pairs clusters. In this study, we introduce an improved robust workflow that integrates novel machine learning strategy channel-specific statistical filtering, enabling adaptation systematic temporal variations in channel ratios. This allows comprehensive profiling throughout pSILAC experiment without relying solely on signals. Additionally, developed KdeggeR , data processing analysis package optimized pSILAC-DIA experiments, which estimates visualizes peptide rates profiles. Our integrative was benchmarked both 2-channel 3-channel standard datasets aneuploid cancer cell model before after cisplatin resistance development demonstrated strong negative correlation between transcript regulation major complex subunits. We also identified specific signatures associated resistance.

Язык: Английский

Процитировано

1