Scientific Reports,
Год журнала:
2024,
Номер
14(1)
Опубликована: Июль 17, 2024
Abstract
Direct
air
capture
(DAC)
in
combination
with
storage
of
CO
2
can
lower
atmospheric
concentrations.
This
study
investigates
the
environmental
impact
a
new
fast-swing
solid
sorbent
DAC
system,
including
transport
and
storage,
over
its
life
cycle,
using
prospective
cycle
assessment.
technology
is
currently
on
readiness
level
5
expected
to
operate
an
industrial
scale
by
2030.
The
was
upscaled
future
changes
background
lifetime
system
were
included,
such
as
electricity
grid
mix
decarbonization.
Environmental
trade-offs
for
assessed
comparing
benefits
from
sequestration
burdens
production,
operation
decommissioning.
We
considered
three
generation
configurations:
grid-connected,
wind-connected,
hybrid
configuration.
found
net
all
configurations
scenarios
ecosystem
damage
climate
change.
Net
human
health
observed
when
decarbonizes
quickly
without
use
battery.
increase
decreasing
footprint
are
comparable
other
technologies.
illustrates
that
help
meet
goals.
Joule,
Год журнала:
2024,
Номер
8(4), С. 979 - 999
Опубликована: Март 1, 2024
Several
low-carbon
technologies,
such
as
solar
photovoltaics
or
batteries,
have
experienced
massive
cost
reductions
in
the
recent
past.
However,
non-mature
technologies
will
also
be
required
to
meet
Paris
climate
targets.
The
of
novel
like
direct
air
capture
(DAC)
remains
highly
uncertain.
Here,
we
introduce
a
new
method
project
future
costs
by
assigning
empirically
grounded
experience
rates
technology
components
based
on
their
similarity
mature
terms
design
complexity
and
customization
needs.
After
an
ex-post
validation
this
method,
apply
it
three
DAC
combined
with
CO2
transport
storage
(DACCS)
provide
probabilistic
estimates
net
removed.
At
1
Gt-CO2/year
cumulative
capacity,
DACCS
at
$341/tCO2
($226–$544
90%
confidence)
for
liquid
solvent
DACCS,
$374/tCO2
($281–$579)
solid
sorbent
$371/tCO2
($230–$835)
CaO
ambient
weathering
DACCS.
Journal of the American Chemical Society,
Год журнала:
2025,
Номер
unknown
Опубликована: Фев. 7, 2025
Escalating
carbon
dioxide
(CO2)
emissions
have
intensified
the
greenhouse
effect,
posing
a
significant
long-term
threat
to
environmental
sustainability.
Direct
air
capture
(DAC)
has
emerged
as
promising
approach
achieving
net-zero
future,
which
offers
several
practical
advantages,
such
independence
from
specific
CO2
emission
sources,
economic
feasibility,
flexible
deployment,
and
minimal
risk
of
leakage.
The
design
optimization
DAC
sorbents
are
crucial
for
accelerating
industrial
adoption.
Metal-organic
frameworks
(MOFs),
with
high
structural
order
tunable
pore
sizes,
present
an
ideal
solution
strong
guest-host
interactions
under
trace
conditions.
This
perspective
highlights
recent
advancements
in
using
MOFs
DAC,
examines
molecular-level
effects
water
vapor
on
capture,
reviews
data-driven
computational
screening
methods
develop
molecularly
programmable
MOF
platform
identifying
optimal
sorbents,
discusses
scale-up
cost
DAC.
Environmental Science & Technology,
Год журнала:
2025,
Номер
unknown
Опубликована: Фев. 11, 2025
This
study
integrates
high-resolution
thermal
and
biological
modeling
with
techno-economic
analysis
life
cycle
assessment
to
evaluate
compare
two
different
microalgae
biorefinery
configurations
targeting
renewable
diesel
(RD)
sustainable
aviation
fuel
(SAF)
production
in
the
United
States
at
county
level.
A
dynamic
engineering
process
model
captures
mass
energy
balances
for
biomass
growth,
storage,
dewatering,
conversion
hourly
resolution.
The
modeled
enable
large-scale
biofuel
by
supporting
facilities
remote
locations
cultivation
on
marginal
lands.
pathways
under
examination
share
identical
harvesting
assumptions
but
differ
their
processes.
first
pathway
evaluates
hydrothermal
liquefaction
(HTL)
produce
RD,
while
second
explores
hydroprocessed
esters
fatty
acids
(HEFA)
SAF.
Results
indicate
that
minimum
selling
price
(MFSP)
HTL
could
decrease
from
3.72-$7.26
1.48-$4.10
per
liter
of
gasoline
equivalent
(LGE-1),
HEFA
5.79-$10.93
1.73-$4.48
LGE-1
future
scenarios
increased
lipid
content
reduced
CO2
delivery
costs.
Optimization
analyses
reveal
achieve
a
MFSP
$0.75
70%
greenhouse
gas
emissions
reductions
compared
petroleum
fuels
both
pathways.
also
examines
water
footprint,
land-use
change
emissions,
additional
environmental
impacts.
Discussion
focuses
outlining
strategic
research
development
investments
reduce
costs
burdens
biofuels.
Nature Chemical Engineering,
Год журнала:
2024,
Номер
1(3), С. 208 - 215
Опубликована: Март 5, 2024
Water
plays
a
pivotal
role
in
direct
air
capture
technologies,
impacting
materials,
regeneration
processes
and
product
streams.
CO2
removal
methods,
including
absorption,
adsorption
electrochemical
techniques,
encounter
challenges
associated
with
water,
thus
reducing
their
efficacy.
fluxes
into
out
of
aqueous
solvents
affect
the
concentration
overall
performance.
Solid
adsorbents
co-adsorb
water
greater
quantities
than
will
require
effective
strategies
to
address
substantial
energy
penalty
desorption
each
cycle.
Water-management
are
imperative
for
economic
viability
minimizing
environmental
impact,
but
high
intensity
necessitates
heat
recovery
techniques.
Feed
dehydration
can
be
combined
strategic
integration
process
streams
standard
techniques
front-end
management.
For
back-end
approaches,
mechanical
vapor
compression
is
viable
solution
coupling
management,
we
highlight
potential
benefits
three
implementation
methods.
Further
research
variable
climate
conditions
quality
impacts
essential
success
technologies.
management
crucial
enhancing
impact
(DAC)
This
Perspective
discusses
several
DAC
processes.
Energy & Environmental Science,
Год журнала:
2024,
Номер
17(13), С. 4544 - 4559
Опубликована: Янв. 1, 2024
A
direct
air
capture
(DAC)
economic
model
that
accounts
for
sorbent
degradation
is
developed.
Experimentally-measured
parameters
are
then
integrated
to
identify
and
process
features
minimize
both
the
DAC
carbon
footprint
cost.
MRS Energy & Sustainability,
Год журнала:
2024,
Номер
unknown
Опубликована: Июль 9, 2024
Abstract
Amid
a
relentless
global
climate
crisis,
the
28th
Conference
of
Parties
(COP28)
spotlighted
Direct
Air
Carbon
Capture
(DACC)
as
key
intervention
to
mitigate
escalating
temperatures
and
CO
2
levels.
The
Intergovernmental
Panel
on
Climate
Change
(IPCC)
underscores
urgency
this
challenge,
stipulating
need
for
robust
removal
strategies.
It
sets
daunting
yet
crucial
target:
capture
85
million
metric
tons
by
2030,
980
2050,
achieve
net-zero
emissions
(IEA,
Executive
Summary—Direct
2022—Analysis.
https://www.iea.org/reports/direct-air-capture-2022/executive-summary
).
Despite
imperative,
existing
19
operational
DAC
facilities
globally
face
significant
barriers,
including
prohibitive
costs
stringent
regulations,
which
impede
their
large-scale
application
(Ozkan
et
al.).
Current
status
pillars
direct
air
technologies.
Iscience
(2022).
While
COP28
stopped
short
delineating
definitive
roadmap
DAC,
article
addresses
vital
aspect
technology:
processes’
substantial
energy
heat
requirements,
are
integral
efficiency
economic
viability.
This
illuminates
pathways
future
technological
evolution
cost
optimization
through
an
in-depth
analysis
these
thereby
charting
course
toward
more
effective
scalable
infrastructure.
Graphical
abstract
Highlights
With
atmospheric
exceeding
420
ppm,
clock
is
ticking
crisis.
offers
revolutionary
approach
directly
remove
excess
,
acting
critical
tool
in
our
fight
sustainable
future.
However,
current
systems
challenge
high
consumption.
Continuous
fan
operation
intake
sorbent
material
regeneration,
consuming
nearly
2000–3000
kWh
per
ton
captured,
major
contributors.
Optimizing
processes
crucial.
Advancements
efficiency,
system
design
that
minimizes
parasitic
losses,
seamless
integration
with
renewable
sources
slashing
DAC’s
demands.
By
reducing
its
carbon
footprint
enhancing
viability,
advancements
can
unlock
full
potential
become
game-changer
combating
change
securing
cleaner
planet.
Discussion
Given
requirements
DACC
processes,
what
innovations
necessary
make
efficient
economically
viable?
Considering
demands
most
promising
avenues
enhance
technology's
scalability
cost-effectiveness?
How
limitations
be
overcome
scale
up
effectively?
What
role
could
play
meeting
facilities,
how
might
impact
overall
process?
do
technologies
influence
location
infrastructure
needs,
particularly
relation
sinks?
or
currently
being
explored
optimize
challenges
they
terms
implementation
scaling?
achieving
targets,
policy
regulatory
frameworks
designed
support
development
deployment
energy-efficient
solutions?
Communications Engineering,
Год журнала:
2024,
Номер
3(1)
Опубликована: Янв. 16, 2024
Abstract
Large-scale
deployment
of
direct
air
carbon
capture
and
storage
(DACS)
is
required
to
offset
CO
2
emissions.
To
guide
decision-making,
a
combined
assessment
costs
environmental
impacts
for
DACS
systems
necessary.
Here
we
present
cost
model
life
cycle
several
combinations
off-grid
DACSs,
powered
by
photovoltaic
(PV)
energy
heat
pumps
with
battery
storages
mitigate
intermittency
the
PV
source.
Utilization
factors
DACSs
are
estimated
different
locations,
power
capacities.
We
find
that
optimal
layout
in
Nevada
(USA)
nominal
removal
capacity
100,000tCO
per
year
consists
100
MW
300MWh
battery.
Costs
$755
$877
gross
net
1tCO
.
The
difference
explained
efficiency
(CRE)
88%.
Of
16
evaluated
impact
categories
mineral
resource
use
most
problematic.
conceive
dashboard
which
allows
track
how
changes
technical
parameters,
such
as
consumption
or
adsorbent
degradation,
costs,
CRE
impacts.
In
an
optimized
scenario
including
tax
credits,
net-removal
will
be
$216
at
93%.
Environmental Science & Technology,
Год журнала:
2024,
Номер
58(24), С. 10567 - 10581
Опубликована: Июнь 3, 2024
Direct
air
capture
with
CO2
storage
(DACCS)
is
among
the
carbon
dioxide
removal
(CDR)
options,
largest
gap
between
current
deployment
and
needed
upscaling.
Here,
we
present
a
geospatial
analysis
of
techno-economic
performance
large-scale
DACCS
in
Europe
using
two
indicators:
CDR
costs
potential.
Different
low-temperature
heat
configurations
are
considered,
i.e.,
coupled
to
national
power
grid,
waste
powered
by
curtailed
electricity.
Our
findings
reveal
that
potential
systems
mainly
driven
(i)
availability
energy
sources,
(ii)
location-specific
climate
conditions,
(iii)
price
GHG
intensity
electricity,
(iv)
transport
distance
nearest
location.
The
results
further
highlight
following
key
findings:
limited
heat,
only
Sweden
potentially
compensating
nearly
10%
emissions
through
CDR,
need
for
considering
comprehensive
assessment
DACCS.
Finally,
our
reveals
substantial
differences
regions
due
useful
information
elements
consistent
insights
will
contribute
feasibility
studies
toward
effective
implementation.