Nonlinear Vortex Dichroism in Chiral Molecules DOI Creative Commons

Luke Cheeseman,

Kayn A. Forbes

Advanced Optical Materials, Год журнала: 2024, Номер unknown

Опубликована: Дек. 15, 2024

Abstract The recent discovery that linearly polarized light with a helical wavefront can exhibit vortex dichroism (also referred to as dichroism) has opened up new horizons in chiroptical spectroscopy structured chiral light. Recent experiments have now pushed optical activity beams into the regime of nonlinear optics. Here theory two‐photon absorption (TPA) focused vortices by molecules: (NVD) is presented. It discovered highly distinct features arise case TPA beams, including ability probe molecular structure not accessible current methods and differential rate significantly influenced orientation state linear polarization. This study provides strong evidence combining improved routes studying chirality.

Язык: Английский

Uniform intensity chiral optical field by multifocal synthesis DOI
Dingyi Wang, Yan Li, Rui Liu

и другие.

Optics Letters, Год журнала: 2024, Номер 49(14), С. 3890 - 3890

Опубликована: Июнь 21, 2024

Chiral optical beams that carry orbital angular momentum (OAM) have a broad range of applications such as tweezers, chiral microstructure fabrication, and communications. However, some inhomogeneous intensity distribution limits the application in these fields. In this Letter, two different types fields with uniform arbitrary length were proposed based on amplitude encoding method multifocal synthesis. The is determined by distance between focal points can greatly extend modulation field. Moreover, since each point contains modulable phase, an interception field be realized selectively retaining part points. By partitioning assigning topological charges, OAM space-division multiplexing independent tunability charges realized. addition, composite multi-petal vortex array formed combining enhance information capacity communications may potential particle manipulation.

Язык: Английский

Процитировано

1

Twisted dynamics in magnetic insulators with structured light DOI
Babak Zare Rameshti, S. Mojtaba Tabatabaei, R. A. Duine

и другие.

Physical review. B./Physical review. B, Год журнала: 2024, Номер 110(9)

Опубликована: Сен. 25, 2024

Язык: Английский

Процитировано

1

Interference Generation of a Reverse Energy Flow with Varying Orbital and Spin Angular Momentum Density DOI Creative Commons

Andrey V. Ustinov,

Alexey P. Porfirev, Svetlana N. Khonina

и другие.

Photonics, Год журнала: 2024, Номер 11(10), С. 962 - 962

Опубликована: Окт. 14, 2024

This paper presents a novel method for generating and shaping reverse energy flow through the interference of light fields from minimal number point sources. Until now, has only been observed using complex fields, such as optical vortices or cylindrical vector beams, limiting formation near axis. We demonstrate both analytically numerically that unbounded regions can be achieved with just two sources, positioned asymmetrically at specific angles (e.g., 90 45 degrees) particular polarization states. The results indicate relative enhanced by increasing sources to three four, adjusting their polarization, introducing vortex phase singularity. presence an initially embedded asymmetry in under consideration leads non-uniform distribution spin orbital angular momentum density. Variations state, well introduction singularity, allow changing density while maintaining flow. also explore feasibility implementing obtained sectional diffractive elements, which will enhance efficiency generated compared

Язык: Английский

Процитировано

1

Calculation of the Transmission Function of a Generalized Spiral Phase Plate to Form a Given Curve DOI

Andrey V. Ustinov,

V. I. Logachev,

Svetlana N. Khonina

и другие.

Optical Memory and Neural Networks, Год журнала: 2024, Номер 33(S1), С. S34 - S42

Опубликована: Дек. 1, 2024

Язык: Английский

Процитировано

1

Nonlinear Vortex Dichroism in Chiral Molecules DOI Creative Commons

Luke Cheeseman,

Kayn A. Forbes

Advanced Optical Materials, Год журнала: 2024, Номер unknown

Опубликована: Дек. 15, 2024

Abstract The recent discovery that linearly polarized light with a helical wavefront can exhibit vortex dichroism (also referred to as dichroism) has opened up new horizons in chiroptical spectroscopy structured chiral light. Recent experiments have now pushed optical activity beams into the regime of nonlinear optics. Here theory two‐photon absorption (TPA) focused vortices by molecules: (NVD) is presented. It discovered highly distinct features arise case TPA beams, including ability probe molecular structure not accessible current methods and differential rate significantly influenced orientation state linear polarization. This study provides strong evidence combining improved routes studying chirality.

Язык: Английский

Процитировано

1