One-Pot Preparation of Layered Double Hydroxide-Engineered Boric Acid Root and Application in Wastewater DOI Creative Commons

Fengrong Zhang,

Cuilan Zhang,

Kaixuan Zhang

и другие.

Molecules, Год журнала: 2024, Номер 29(13), С. 3204 - 3204

Опубликована: Июль 5, 2024

Heavy metals and organic pollutants are prevalent in water bodies, causing great damage to the environment human beings. Hence, it is urgent develop a kind of adsorbent with good performance. Anion interlacing layered double hydroxides (LDHs) promising for sustainable removal heavy metal ions dyes from wastewater. Using aluminum chloride, zinc chloride ammonium pentaborate tetrahydrate (NH4B5O8 · 4H2O, BA) as raw materials, LDHs complex (BA-LDHs) B5O8− intercalation was prepared by one-step hydrothermal method. The BA-LDHs samples were characterized X-ray powder diffractometer (XRD), scanning electron microscope (SEM), Fourier transform infrared spectrometer (FT-IR) Brunauer–Emmett–Teller (BET) results showed that B5O8- successfully intercalated. Adsorption experimental suggested possess maximum adsorption capacity 18.7, 57.5, 70.2, 3.12 mg·g−1 Cd(II), Cu(II), Cr(VI) Methylene blue (MB) at Cs = 2 g·L−1, respectively. experiment conforms Langmuir Freundlich models, kinetic data well fitted pseudo-second-order equation. as-prepared have potential application prospects More importantly, they also provide strategy preparing selective adsorbents.

Язык: Английский

Preparation of ZnAl layered double hydroxides supported by silica for the treatment of Cr(VI) and Cu(II) in aqueous solution DOI Creative Commons

Fengrong Zhang,

Luxing Liu,

Cuilan Zhang

и другие.

Scientific Reports, Год журнала: 2025, Номер 15(1)

Опубликована: Янв. 20, 2025

A novel adsorbent ZnAl–LDHs/SiO2 (ZA/SiO2) was prepared by blending urea mixture of ZnSO4 and Al2(SO4)3 while using SiO2 as a support form. The adsorption properties ZA/SiO2 for the removal toxic metal ions (Cu(II) Cr(VI)) from water were evaluated. By batch experiment method to investigate Cu(II) Cr(VI) solution treatment effect. sorption kinetics curves on L-shaped. What's more, solid concentration effect found in process kinetics. Langmuir Freundlich isotherm models used analyze data. results showed that conforms models. However, capacity compounds is greatly improved. 158 mg·g−1 176 mg·g−1, which 3.6 1.8 times ZnAl-LDHs (ZA), respectively. Density functional theory (DFT) utilized analysis intrinsic mechanism specific pathways. primary removing mainly included intercalation Cr2O72− exchange between OH−, excluding Cr(OH)3 precipitation. Regarding eliminating water, it involves isomorphic substitution predominant process, except formation Cu(OH)2 precipitates.

Язык: Английский

Процитировано

1

Purification of arsenic-contaminated drinking water by Fe-Al-CO3 layered double hydroxide derived from secondary aluminum dross: adsorption and stabilization studies DOI Creative Commons

Mohammad Bozorgi,

Mostafa Mahinroosta, Ali Allahverdi

и другие.

Scientific Reports, Год журнала: 2025, Номер 15(1)

Опубликована: Янв. 13, 2025

This study aims to utilize secondary aluminum dross waste synthesize Fe-Al layered double hydroxide (Fe-Al LDH) for efficient adsorption of arsenic from drinking water. The synthesis process was based on a multi-step hydrometallurgical approach, in which the content first converted sodium aluminate. followed by transformation into LDH through series processes, including gelation, sol formation, simultaneous precipitation, and aging. A suitable crystal structure adsorbent successfully synthesized at Fe: Al molar ratio 3, pH 7, an aging time 12 h. characterization tests revealed that Fe-Al-LDH had interlayer space 7.5 Å, specific surface area ​​145 m2/g, pore volume 0.57 cm3/g. resulting then used adsorb aqueous solutions. results showed amount adsorbed 0.144 mg/g room temperature, dose 0.5 g/L, = 7 initial concentration 80 µg/L. reduced water below standard value after period 40 min. In addition, can stabilize species its thus prevent their re-release environment.

Язык: Английский

Процитировано

0

In situ engineering 2D/3D CuCo2S4@Co3O4 heterojunction for sensing and photocatalytic degradation of diclofenac sodium in environmental water DOI
Chunmei Chen, Yunjie Yang, Qiong Wang

и другие.

Journal of Environmental Sciences, Год журнала: 2025, Номер unknown

Опубликована: Фев. 1, 2025

Язык: Английский

Процитировано

0

Utilization of Natural Mineral Materials in Environmental Remediation: Processes and Applications DOI Open Access
Dongsheng Xu, Yongkui Yang, Li‐Hua Gan

и другие.

Minerals, Год журнала: 2025, Номер 15(3), С. 318 - 318

Опубликована: Март 19, 2025

The discharge of wastewater containing persistent organic pollutants presents significant ecological and health challenges due to their toxicity resilience. Recent advances in advanced oxidation processes (AOPs) other remediation mechanisms, notably utilizing natural mineral materials (NMMs), offer promising solutions these challenges. NMMs, with cost-effectiveness, accessibility, eco-friendly nature, non-toxicity, unique structural properties, have shown promise environmental could effectively replace conventional catalysts related applications. These minerals enable the activation oxidants, generating reactive oxygen species crucial for degradation pollutants. This article reviews mechanisms NMMs various AOPs, including photocatalysis, Fenton-like reactions, persulfate-activation-based processes, discusses potential enhancing pollutant efficiency, a focus on persulfates photo-induced redox processes. synergy between photocatalytic properties catalytic provided by offers robust approach managing water pollution without drawbacks secondary waste production, thus supporting sustainable efforts.

Язык: Английский

Процитировано

0

Tribocatalysis and self-Fenton reaction of schorl/pyrite mineral composites under stirring conditions DOI
Bingwei Chen, Wangshu Tong, Xinnan Li

и другие.

Materials Science in Semiconductor Processing, Год журнала: 2025, Номер 193, С. 109496 - 109496

Опубликована: Март 24, 2025

Язык: Английский

Процитировано

0

Enhanced sonophotocatalytic degradation of phthalate acid ester using copper-chromium layered double hydroxides on carbon nanotubes and biochar DOI Creative Commons
Tannaz Sadeghi Rad, Alireza Khataee,

Emine Sevval Yazici

и другие.

Ultrasonics Sonochemistry, Год журнала: 2025, Номер unknown, С. 107351 - 107351

Опубликована: Апрель 1, 2025

Язык: Английский

Процитировано

0

Efficient catalytic decomposition of ozone by flake NiFe-LDH with multiple acidic sites DOI

Ruixin Mao,

Fengyu Li,

Yingzhi Bu

и другие.

Applied Surface Science, Год журнала: 2025, Номер 700, С. 163191 - 163191

Опубликована: Апрель 15, 2025

Язык: Английский

Процитировано

0

One-Pot Preparation of Layered Double Hydroxide-Engineered Boric Acid Root and Application in Wastewater DOI Creative Commons

Fengrong Zhang,

Cuilan Zhang,

Kaixuan Zhang

и другие.

Molecules, Год журнала: 2024, Номер 29(13), С. 3204 - 3204

Опубликована: Июль 5, 2024

Heavy metals and organic pollutants are prevalent in water bodies, causing great damage to the environment human beings. Hence, it is urgent develop a kind of adsorbent with good performance. Anion interlacing layered double hydroxides (LDHs) promising for sustainable removal heavy metal ions dyes from wastewater. Using aluminum chloride, zinc chloride ammonium pentaborate tetrahydrate (NH4B5O8 · 4H2O, BA) as raw materials, LDHs complex (BA-LDHs) B5O8− intercalation was prepared by one-step hydrothermal method. The BA-LDHs samples were characterized X-ray powder diffractometer (XRD), scanning electron microscope (SEM), Fourier transform infrared spectrometer (FT-IR) Brunauer–Emmett–Teller (BET) results showed that B5O8- successfully intercalated. Adsorption experimental suggested possess maximum adsorption capacity 18.7, 57.5, 70.2, 3.12 mg·g−1 Cd(II), Cu(II), Cr(VI) Methylene blue (MB) at Cs = 2 g·L−1, respectively. experiment conforms Langmuir Freundlich models, kinetic data well fitted pseudo-second-order equation. as-prepared have potential application prospects More importantly, they also provide strategy preparing selective adsorbents.

Язык: Английский

Процитировано

1