Enzyme-Assisted Solid-Phase Microextraction Coupled with a DNA Nanowalker for Dual-Amplified Detection of Chloramphenicol in Animal-Derived Food Products DOI

Yitong Chen,

Zhuoyue Shen,

Chunxu Tao

и другие.

Journal of Agricultural and Food Chemistry, Год журнала: 2024, Номер unknown

Опубликована: Ноя. 21, 2024

Chloramphenicol (CAP), an aminoalcohol antibiotic, exerts its action on bacterial ribosomes, thereby obstructing protein synthesis. However, the use of CAP in husbandry may lead to excessive accumulation animal-derived food products. This presents potential risks consumer health. study developed a novel dual-amplification fluorescence detection method by integrating enzyme-assisted solid-phase microextraction (SPME) with Fe3O4@Au NP-based DNA nanowalker for food. The combination quartz rod-based SPME biosensor and effectively eliminated matrix interference, enabling conversion enhancement signals through two cyclic amplification processes. strategy demonstrated high sensitivity limit 28.1 aM as well wide linear range from 0.1 fM 1 nM (with R2 > 0.99). also demonstrates robust stability accuracy detecting trace amounts both authentic prepared positive samples.

Язык: Английский

Polysaccharide Hydrogel-Assisted Biosensing Platforms for Point-of-Care Use DOI Creative Commons
Sang‐Uk Kim, Young Jun Kim, Tae Hee Lee

и другие.

Biosensors, Год журнала: 2025, Номер 15(1), С. 13 - 13

Опубликована: Янв. 2, 2025

Point-of-care (POC) use is one of the essential goals biosensing platforms. Because increasing demand for testing cannot be met by a centralized laboratory-based strategy, rapid and frequent at right time place will key to health safety. To date, however, there are still difficulties in developing simple affordable, as well sensitive effective, platform that enables POC use. In terms materials, hydrogels, unique family water-absorbing biocompatible polymers, have emerged promising components development biosensors. Combinations hydrogels various additional applications, such hydrophilic coatings, nanoscale filtration, stimuli-responsive signal enhancement, biodegradation. this review, we highlight recent efforts develop hydrogel-assisted platforms use, especially focusing on polysaccharide like agarose, alginate, chitosan, so on. We first discuss pros cons practical applications then introduce case studies test different formats, paper-based analytical devices (PADs), microfluidic devices, independent believe analysis present review provides information resource-limited settings.

Язык: Английский

Процитировано

0

Bimetallic MOF doped with reduced graphene oxide enables rapid detection of chloramphenicol DOI Open Access

Youheng Pan,

Tianyi Zhang, Lanlan Li

и другие.

Journal of Physics Conference Series, Год журнала: 2025, Номер 2961(1), С. 012020 - 012020

Опубликована: Фев. 1, 2025

Abstract A broad-spectrum antibiotic called chloramphenicol (CAP) stops the creation of bacterial proteins, which bacteria from growing and reproducing. When is misused, it can cause major side effects, secondary infections, resistance, delays in effective treatment, higher treatment costs. As a result, creating an electrochemical sensor that quick sensitive crucial. The electrocatalytic activity CAP determination was enhanced this work by producing reduced graphene oxide doped bimetallic organic framework (Fe/Al-MOF/rGO) nanocomposites single pot, had more active sites better electrical conductivity. constructed has linear range 20 - 1600 μM detection line (LOD) 1.5 nM (S/N=3). Furthermore, sensor’s recovery rate for sample good enough.

Язык: Английский

Процитировано

0

Ratiometric fluorescence biosensing of granzyme B based on biomimetic microspheres DOI
Ji Zheng, Xuewei Li, Hui–Ming Cheng

и другие.

Sensors and Actuators B Chemical, Год журнала: 2025, Номер unknown, С. 137492 - 137492

Опубликована: Фев. 1, 2025

Язык: Английский

Процитировано

0

Combining CRISPR-Cas12a with Microsphere Array-Enhanced Fluorescence for Portable Pathogen Nucleic Acid Detection DOI
Menglu Gao, Chen Yang, Si Wu

и другие.

ACS Applied Materials & Interfaces, Год журнала: 2025, Номер unknown

Опубликована: Март 28, 2025

The detection of food contamination in a swift and sensitive manner is essential for safeguarding public health. Clustered regularly interspaced short palindromic repeats (CRISPR)-based assays nucleic acid are renowned their high specificity convenient, related studies have focused on refining the Cas protein optimizing CRISPR (cr)RNAs design within CRISPR-based enhancing sensitivity detection. Our research offers innovative insights into fluorescence signal output intensity from physical standpoint, thereby presenting practical cost-effective strategy to lower thresholds assays. By layer microsphere arrays was spread onto bottom microfluidic chip enhance sample via self-assembly microspheres. Recombinase polymerase amplification (RPA) used amplify target sequences, followed by crRNA binding activate enzyme, cleaving fluorescein amidite (FAM)-labeled reporters emitting fluorescent signal. method successfully identified SARS-CoV-2 positive samples (10 clinical 8 environmental samples) distinguished them negative samples. Meanwhile, it detected 4 Shigella 5 In this study, developed exhibited limit (LoD) 75 fM (POCT with USB camera: 50 fM) 100 fM). It also demonstrated promising (100%) small-sample validation. Combined portable automated achieved using smartphone receive process signals obtained platform study not only applicable pathogens cold-chain products, but extends pathogen community hospitals resource-limited areas, providing an efficient solution rapid screening different settings. Moreover, can be changing RPA primer crRNA. This provides paradigm studying enhanced signaling holds significant potential advance commercialization use sensors.

Язык: Английский

Процитировано

0

Low-Frequency Optical Signal Enhancement Device Combines CRISPR-Based Assay for Portable S. Pneumoniae Detection DOI
Yang Chen, Menglu Gao, Yifan Wang

и другие.

Analytical Chemistry, Год журнала: 2025, Номер unknown

Опубликована: Апрель 9, 2025

Early detection and treatment of Streptococcus pneumoniae (SPN) is crucial for patients. However, since nucleic acid testing relies on large-scale equipment specialized operators, challenges remain accurate, fast, low-cost SPN detection. Here, we present a point-of-care (POCT) device rapid accurate based low-frequency optical signal enhancement cluster regularly interspaced short palindromic repeats (CRISPR). The spotlight tube enables the fluorescence signal, while combination an artificial intelligence-assisted autoexposure algorithm homomorphic filtering image processing method improves signal-to-noise ratio image, thus realizing highly sensitive Nucleic identification performed using CRISPR-based crRNAs, fluorescent probes were constructed against IytA gene SPN. And they showed high specificity sensitivity gene. This demonstrated excellent in detecting developed strategy. threshold reached 0.1 fM, single time was only 40 min. Specificity validated clinical samples, test 100% agreement with quantitative polymerase chain reaction results from samples. provides device, which, novel DNA probe SPN, indicator option POCT

Язык: Английский

Процитировано

0

Highly sensitive and wash-free human serum albumin detection based on filtration-to-enhancement compound microsphere system DOI
Chen Yang, Xin Zhang,

Minjing Mo

и другие.

Chemical Engineering Journal, Год журнала: 2025, Номер 514, С. 163097 - 163097

Опубликована: Май 3, 2025

Язык: Английский

Процитировано

0

Probe-free and wash-free strategy for on-site testing of chloramphenicol in food based on differential encodable microspheres separation system DOI

Chen Yang,

Guoqing He,

Shukun Zhao

и другие.

Talanta, Год журнала: 2025, Номер 295, С. 128250 - 128250

Опубликована: Май 4, 2025

Язык: Английский

Процитировано

0

Enzyme-Assisted Solid-Phase Microextraction Coupled with a DNA Nanowalker for Dual-Amplified Detection of Chloramphenicol in Animal-Derived Food Products DOI

Yitong Chen,

Zhuoyue Shen,

Chunxu Tao

и другие.

Journal of Agricultural and Food Chemistry, Год журнала: 2024, Номер unknown

Опубликована: Ноя. 21, 2024

Chloramphenicol (CAP), an aminoalcohol antibiotic, exerts its action on bacterial ribosomes, thereby obstructing protein synthesis. However, the use of CAP in husbandry may lead to excessive accumulation animal-derived food products. This presents potential risks consumer health. study developed a novel dual-amplification fluorescence detection method by integrating enzyme-assisted solid-phase microextraction (SPME) with Fe3O4@Au NP-based DNA nanowalker for food. The combination quartz rod-based SPME biosensor and effectively eliminated matrix interference, enabling conversion enhancement signals through two cyclic amplification processes. strategy demonstrated high sensitivity limit 28.1 aM as well wide linear range from 0.1 fM 1 nM (with R2 > 0.99). also demonstrates robust stability accuracy detecting trace amounts both authentic prepared positive samples.

Язык: Английский

Процитировано

1