Surface Modification of Polydopamine Particles with Polyethyleneimine Brushes for Enhanced Stability and Reduced Fragmentation DOI Open Access

Su Hyeon Son,

Eun Jin Kim,

Hye Young Koo

и другие.

Polymers, Год журнала: 2025, Номер 17(9), С. 1209 - 1209

Опубликована: Апрель 28, 2025

Polydopamine (Pdop) particles possess unique properties but suffer from inherent instability in aqueous environments due to the gradual release of Pdop fragments. This study demonstrated successful enhancement stability and reduction fragmentation through surface engineering strategies. Specifically, we investigated effects polyelectrolyte multilayer (PEM) coating (PE) brush grafting. Our results showed that PE grafting, particularly with long-chain polyethyleneimine (PEI), was more effective suppressing fragment compared PEM coating. The L-PEI grafted (2.28 chains/nm2) exhibited remarkable across a wide pH range (3–9), inhibition rates exceeding 90% most cases, reaching 93% at 5. Furthermore, direct correlation between PEI grafting density (0.64 2.28 rate observed, higher densities yielding greater stability. These findings offer promising approach for stabilizing diverse applications.

Язык: Английский

Photocatalytic Oxidation of Pesticides with TiO2-CeO2 Thin Films Using Sunlight DOI Open Access

Tania Arelly Tinoco Pérez,

Evaristo Salaya Gerónimo, G. Torres

и другие.

Catalysts, Год журнала: 2025, Номер 15(1), С. 46 - 46

Опубликована: Янв. 6, 2025

TiO2 thin film coatings significantly improve catalyst separation in photocatalytic processes. They can be applied heterogeneous photocatalysis under sunlight by mixing with other oxides, such as CeO2, for the removal of pollutants water. Here, TiO2-CeO2 films deposited on borosilicate slides were analyzed and solar oxidation pesticides. The synthesized sol-gel method spin coating. waste solutions from synthesis used to prepare powders. These XRD XPS explain behavior films. characterized UV-Vis spectroscopy transmittance, RDS, profilometry, AFM SEM. addition CeO2 caused a decrease average crystal size an increase strain index. second layer made thinner. created surface electronic defects titania films, which enhanced their properties mineralization diuron methyl parathion. TiO2-CeO2-5.0% single-layer samples most active this study will undoubtedly larger-scale reaction systems.

Язык: Английский

Процитировано

0

Reductive sulfur mediated Fe2+ fixation and regeneration in valorizing waste activated sludge ash to Fe2+@S-doped sodalite material for emerging contaminants degradation: Performance and mechanism DOI

Yuting Zhou,

Hao Wu,

Jannat Javed

и другие.

Chemical Engineering Science, Год журнала: 2025, Номер unknown, С. 121438 - 121438

Опубликована: Фев. 1, 2025

Язык: Английский

Процитировано

0

Sunlight-Induced Photocatalytic Removal of Paracetamol Using Au-TiO2 Nanoparticles DOI Creative Commons

Lamine Aoudjit,

Joana M. Queirós, A. Castro

и другие.

Nanomaterials, Год журнала: 2025, Номер 15(5), С. 358 - 358

Опубликована: Фев. 26, 2025

Using sunlight as the driving force for photocatalytic processes holds great promise sustainability. As a starting point developing material capable of degrading aquatic pollutants using solar energy stimulus, this work focuses on synthesizing Au-TiO2 nanocomposites deposition-precipitation method. Characterization nanoparticles was performed by X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FTIR), and Transmission Electron Microscopy (TEM). A model pollutant, paracetamol, used to test synergetic effect Au (0.05 wt%) (NPs) with TiO2 activity. The influence parameters pH, loading (0.4, 0.8, 1 g/L), pollutant concentration (20, 30, 40 ppm), contact time (30, 60, 90, 120, 150, 180 min) studied exposing NPs radiation. degradation most effective at 3 h, an initial 20 ppm, pH 6.8. Under these conditions, paracetamol in g/L can be degraded more than 99.17% under irradiation. result composite's ability successfully serve photocatalyst sun radiation, water purification widespread, cost-effective, environmentally friendly.

Язык: Английский

Процитировано

0

The Elimination of N-Chloropiperidine in Aqueous Solution by Using Ni/NiO-C3N4 Under Visible Light Illumination DOI Open Access
Tahani M. Bawazeer,

Amal A. Atran,

Fatmah Alkhatib

и другие.

Catalysts, Год журнала: 2025, Номер 15(3), С. 233 - 233

Опубликована: Фев. 28, 2025

One of the main challenges in environmental remediation is creation stable and effective photocatalysts to eliminate organic contaminants when exposed visible light. For degradation N-chloropiperidine, a persistent pollutant with multiple dangerous issues, we provide synthesis, characterization, photocatalytic evaluation Ni/NiO-incorporating carbon nitride (Ni/NiO-C3N4) composite this work. The Ni/NiO-C3N4 photocatalyst was created by single step thermally polymerizing nickel nitrate melamine. Four samples are ranged Ni concentration from 0% 10%. coexistence NiO phases confirmed structural morphological analyses using X-ray diffraction (XRD), scanning electron microscopy (SEM), transmission (TEM), Fourier-transform infrared spectroscopy (FTIR). UV−Vis diffuse reflectance (DRS) also demonstrated an enhanced capacity absorb A study performance under light illumination showed that degraded N-chloropiperidine at much faster rate than either pure (0.0231 min−1), first-order constant 0.0456 min−1. reaction nearly quadrupled 10% added C3N4 matrix. Furthermore, composite’s activity performed better its counterparts Ni-C3N4 (0.0315 min−1) NiO-C3N4 (0.0386 min−1). synergistic interaction between NiO, which promotes charge separation lowers electron–hole recombination, responsible for higher Ni/NiO-C3N4, increasing production reactive oxygen species. reusability experiments conducted over four successive cycles slight decrease activity, indicating prepared reusable.

Язык: Английский

Процитировано

0

Effect of 3D branched crystalline carbon nitride on nucleic acid amplification techniques in food samples DOI

Yaofang Fan,

Yuxin Xue,

Haoran Wang

и другие.

Food Control, Год журнала: 2025, Номер unknown, С. 111299 - 111299

Опубликована: Март 1, 2025

Язык: Английский

Процитировано

0

Fe2O3@D201 Enhanced Efficiency of Food Waste Degradation by Microbial Inoculum Under Aerobic Condition DOI
Ying Han,

Meiqi Yin,

Qingrui Zhang

и другие.

Current Microbiology, Год журнала: 2025, Номер 82(5)

Опубликована: Апрель 2, 2025

Язык: Английский

Процитировано

0

Recent Advances in the Design and Biocidal Mechanisms of Room-temperature Catalytic Nanomaterials for Efficient Inactivation of Bioaerosols DOI
Wenhui Cheng, Zhenyu Wang, Shiqi Peng

и другие.

Surfaces and Interfaces, Год журнала: 2025, Номер unknown, С. 106449 - 106449

Опубликована: Апрель 1, 2025

Язык: Английский

Процитировано

0

Sustainable Semicrystalline/Nanocrystalline UiO-66-Type Zr-MOFs as Photodegraders of Rhodamine B DOI Creative Commons
Jemal M. Yassin,

Abi M. Taddesse,

Manuel Sánchez‐Sánchez

и другие.

Inorganics, Год журнала: 2025, Номер 13(5), С. 131 - 131

Опубликована: Апрель 24, 2025

UiO-type Zr-BDC MOFs have garnered the interest of scientific community due to their exceptional diversity in composition, structure, and chemical environment, as well high thermal stabilities. This work demonstrates sustainable synthesis a series nanocrystalline/semicrystalline UiO-66(Zr) metal–organic frameworks (MOFs) under facile conditions—specifically at room temperature, water, with yield, without use modulators or toxic byproducts. The involves either deprotonating linker utilizing various ratios water DMF solvents. as-prepared materials obtained from both strategies share key structural features conventional short- medium-range physicochemical properties, while exhibiting significant differences crystallinity textural properties. Nonetheless, generally lack long-range order (semicrystalline), particular these synthesized following deprotonation strategy. However, prepared using mixed solvent strategy seem exhibit characteristics nanocrystalline UiO-66(Zr). Overall, approaches successfully addressed challenges related highly sought-after Zr-based (MOFs). Some MOF were tested for photodegradation rhodamine B (RhB) mercury light irradiation, evidencing photocatalytic efficiency up 75 ± 0.078% within 120 min pseudo-first-order model. suggests an interaction between photocatalyst RhB dye, involving electron injection ability ligand-to-metal charge transfer (LMCT), which enhances efficient degradation RhB. trapping experiments indicated that superoxide radicals (•O2−) photogenerated holes (h+) are crucial Moreover, showed good recyclability across five cycles. A plausible reaction mechanism has been proposed explain findings.

Язык: Английский

Процитировано

0

Defect density of zirconium determines its binding sites and force to antibiotic resistance genes DOI
Ying Han, Yuman Zhang,

Yin Meiqi

и другие.

Chemical Engineering Journal, Год журнала: 2025, Номер unknown, С. 163042 - 163042

Опубликована: Апрель 1, 2025

Язык: Английский

Процитировано

0

Surface Modification of Polydopamine Particles with Polyethyleneimine Brushes for Enhanced Stability and Reduced Fragmentation DOI Open Access

Su Hyeon Son,

Eun Jin Kim,

Hye Young Koo

и другие.

Polymers, Год журнала: 2025, Номер 17(9), С. 1209 - 1209

Опубликована: Апрель 28, 2025

Polydopamine (Pdop) particles possess unique properties but suffer from inherent instability in aqueous environments due to the gradual release of Pdop fragments. This study demonstrated successful enhancement stability and reduction fragmentation through surface engineering strategies. Specifically, we investigated effects polyelectrolyte multilayer (PEM) coating (PE) brush grafting. Our results showed that PE grafting, particularly with long-chain polyethyleneimine (PEI), was more effective suppressing fragment compared PEM coating. The L-PEI grafted (2.28 chains/nm2) exhibited remarkable across a wide pH range (3–9), inhibition rates exceeding 90% most cases, reaching 93% at 5. Furthermore, direct correlation between PEI grafting density (0.64 2.28 rate observed, higher densities yielding greater stability. These findings offer promising approach for stabilizing diverse applications.

Язык: Английский

Процитировано

0