Self‐assembled small molecule spherulites under mild conditions: High solid‐state quantum yield and unique interconnected structural and fluorescent colors DOI Creative Commons
Cheng Li, Oriol Arteaga,

Florian Ehlers

и другие.

Aggregate, Год журнала: 2024, Номер unknown

Опубликована: Окт. 24, 2024

Abstract Spherulites are generally fabricated from cooling polymer melts, while their fabrication under mild conditions or small molecule materials has been barely reported. Besides, organic luminescent molecules typically suffer low quantum yields in a solid state. Moreover, preparing material with interconnected and simultaneous changes structural fluorescent colors is challenging. Here, we present the first solution‐derived spherulites unique colors, self‐assembled stearoylated monosaccharides at room temperature. D‐galactose stearoyl ester into banded spherulites, containing twisted nanoplates simultaneously changing colors. In comparison, D‐mannose can only form non‐banded which contain oriented uniform Such revealed novel negative correlation between fluorescence birefringence, termed alignment‐promoted quenching propensity. Remarkably, solid‐state of galactose mannose‐derived as high 49 ± 2% 51 respectively, approximately ten times higher than those unmodified monosaccharides. These yield values among highest reported nonconventional fluorophores even comparable to conventional aromatic chromophores. these manifested an unexpected excitation‐dependent multicolor photoluminescence broad‐spectrum emission (410−620 nm). They show multiple peaks photoluminescent spectra broad lifetime distributions, should be attributed clustering variety oxygen‐containing functional groups emissive moieties.

Язык: Английский

A Comprehensive Review on Cellulose Nanofibers, Nanomaterials, and Composites: Manufacturing, Properties, and Applications DOI Creative Commons

Subin Antony Jose,

Neil D. Cowan,

Matthew Davidson

и другие.

Nanomaterials, Год журнала: 2025, Номер 15(5), С. 356 - 356

Опубликована: Фев. 25, 2025

Cellulose nanofibers (CNFs), cellulose nanomaterials (CNMs), and cellulose-based composites represent a convergence of material science, sustainability, advanced engineering, paving the way for innovative eco-friendly materials. This paper presents comprehensive review these materials, encompassing their extraction, preparation methods, properties, applications, future directions. The manufacturing CNFs CNMs leverages diverse techniques-chemical, mechanical, enzymatic-with each offering distinct advantages in tailoring characteristics to meet specific needs. Strategies functionalization surface modification are detailed, highlighting role enhancing properties while addressing challenges scaling production industrial levels. structural, thermal, optical, electrical, biocompatibility CNFs, CNMs, explored, underscoring versatility applications across various industries. Cellulose-based composites, particular, demonstrate exceptional tunable uses, although achieving uniform dispersion remains key technical hurdle. These materials have packaging, automotive, aerospace, biomedical devices, energy storage, environmental remediation. Emerging research trends emphasize integration with technologies, promoting sustainable practices life cycle considerations advancing commercialization potential. rapidly evolving field holds immense promise global by creating high-performance, is crucial understanding nanofibers, nanomaterials, providing valuable insights that will drive development sustainable, high-performance wide range ultimately challenges.

Язык: Английский

Процитировано

3

Tunable and Responsive Circularly Polarized Luminescence of Self‐Organized Cellulose Nanocrystal Chiral Superstructures Loaded with AIE Luminogen DOI Open Access
Baohua Yuan, Q. Jing,

Longxiang He

и другие.

Advanced Functional Materials, Год журнала: 2025, Номер unknown

Опубликована: Фев. 9, 2025

Abstract Circularly polarized luminescence (CPL) holds great potential for next‐generation display techniques. However, dynamic, multicolor CPL with high luminescent quantum yield (PLQY) and tunable dissymmetry factor ( g lum ) based on cost‐effective, sustainable materials is scarcely attainable. Herein, a straightforward approach proposed engineering cellulose nanocrystal (CNC) chiral superstructures loaded aggregation‐induced emission luminogens (AIEgens) through the evaporation‐induced self‐assembly of renewable CNCs tetra‐(4‐pyridylphenyl)ethylene molecules. The judicious design two building blocks as donor–acceptor pairs not only respectively achieves an 86‐fold 2.1‐fold improvement in PLQY resulting systems suspension aggregate states comparison bare AIEgens, but also endows AIEgen‐loaded CNC pH‐tunable, humidity‐responsive, maximal | 0.89. It revealed that induction photonic bandgap effects—which are dominated by interactions homogeneous or heterogeneous processes—are involved mechanisms. Finally, humidity‐responsive multiple changes (structural color, fluorescent CPL) realized both biobased inks films, which paramount importance applications dynamic information encryption. This work offers underlying insights construction dynamically CPL.

Язык: Английский

Процитировано

0

Physical insights into the high radiative cooling power of cellulose-based materials DOI
Zhuo Zhao, Jian Zhang, Yuan Cheng

и другие.

Physical Chemistry Chemical Physics, Год журнала: 2025, Номер unknown

Опубликована: Янв. 1, 2025

Cellulose-based materials exhibit superior spectral properties and high radiative cooling efficiency, making them promising candidates for passive thermal management applications.

Язык: Английский

Процитировано

0

Self‐assembled small molecule spherulites under mild conditions: High solid‐state quantum yield and unique interconnected structural and fluorescent colors DOI Creative Commons
Cheng Li, Oriol Arteaga,

Florian Ehlers

и другие.

Aggregate, Год журнала: 2024, Номер unknown

Опубликована: Окт. 24, 2024

Abstract Spherulites are generally fabricated from cooling polymer melts, while their fabrication under mild conditions or small molecule materials has been barely reported. Besides, organic luminescent molecules typically suffer low quantum yields in a solid state. Moreover, preparing material with interconnected and simultaneous changes structural fluorescent colors is challenging. Here, we present the first solution‐derived spherulites unique colors, self‐assembled stearoylated monosaccharides at room temperature. D‐galactose stearoyl ester into banded spherulites, containing twisted nanoplates simultaneously changing colors. In comparison, D‐mannose can only form non‐banded which contain oriented uniform Such revealed novel negative correlation between fluorescence birefringence, termed alignment‐promoted quenching propensity. Remarkably, solid‐state of galactose mannose‐derived as high 49 ± 2% 51 respectively, approximately ten times higher than those unmodified monosaccharides. These yield values among highest reported nonconventional fluorophores even comparable to conventional aromatic chromophores. these manifested an unexpected excitation‐dependent multicolor photoluminescence broad‐spectrum emission (410−620 nm). They show multiple peaks photoluminescent spectra broad lifetime distributions, should be attributed clustering variety oxygen‐containing functional groups emissive moieties.

Язык: Английский

Процитировано

1