Differences in Performance among ECPs with Different Metal Centers Based on Highly Stable TzTO DOI
Jinhao Zhang, Zhiyuan Jin,

Taichuan Li

и другие.

Crystal Growth & Design, Год журнала: 2024, Номер 24(22), С. 9337 - 9343

Опубликована: Авг. 29, 2024

The stability and detonation properties of energetic coordination polymers (ECPs) are usually directly related to the selection ligands. However, different metals ligands may form structures, which will greatly affect performance ECPs. Three-dimensional (3D) metal–organic frameworks (EMOFs) exhibit enhanced performances modest compared with one-dimensional (1D) two-dimensional (2D) In this work, an internal salt H2TzTO (5-(1H-1,2,4-triazol-4-ium-3-yl)-1H-tetrazol-1-olate) high was selected as ligand coordinated four metal centers, Na(I), K(I), Co(II), Ni(II), three ECPs, named [Na(HTzTO)(H2O)]n·0.5H2O, Co(HTzTO)2(H2O)2, Ni(HTzTO)2(H2O)2·2H2O, one EMOF [K(HTzTO)]n, respectively. compounds showed excellent thermal [decomposition temperature (Td) ≥ 263 °C] [detonation velocity (D) 8587 m·s–1 pressure (P) 33.8 GPa], but their due influence center structure. Among them, [K(HTzTO)]n Co(HTzTO)2(H2O)2 surprising (Td = 344 347 °C, respectively) formation face-to-face π–π stacking in enhances molecules.

Язык: Английский

Synthesizing new Bi-structure energetic coordination compounds using ternary components DOI
Chao Zhang, Tingwei Wang,

Meiqi Xu

и другие.

Inorganic Chemistry Frontiers, Год журнала: 2023, Номер 11(2), С. 624 - 631

Опубликована: Дек. 11, 2023

[Ag(1-APZ-5-HCA)(ClO 4 ) 2 ] n (ECPs-1) has a dual structure of ionic salt and coordination compounds. It also the advantages high ClO − content oxygen balance, acceptable mechanical stimulation excellent explosion performance.

Язык: Английский

Процитировано

6

Two Energetic Framework Materials Based on DNM–TNBI as Host Molecule: Effectively Coordinated by Different Cations DOI

Boqian Yang,

Bibo Li,

Yang Liu

и другие.

Chemistry - An Asian Journal, Год журнала: 2024, Номер 19(9)

Опубликована: Март 6, 2024

Abstract With the demand of develop outstanding‐performance energetic materials, 1‐(dinitromethyl)‐4,4’,5,5’‐tetranitro‐1H,1’H‐2,2’‐biimidazole ( DNM – TNBI ) emerged as a great contender (D: 9102 m ⋅ s −1 ; P: 37.6 GPa). However, relatively poor thermal stability (T d : 142 °C) limits its practical application. In this study, host molecule to synthesize two new open–framework materials by effectively coordinated with different cations. Their supramolecular structures were investigated and indicated that [ 2 − ][ 2NH 4 + ] 2K can be classified hydrogen–bonded ammonium framework (EHAF) an metal organic (EMOF). Meanwhile, their stabilities are higher than have satisfactory detonation performance ([ ], D: 8050 , 26.4 GPa; 8301 30.8

Язык: Английский

Процитировано

1

Metal salts of fused triazole-triazine as Promising energetic materials: Crystal Structures, Energetic Properties and high thermal stability DOI
Shichang Liu, Zhen Dong, Zhiwen Ye

и другие.

New Journal of Chemistry, Год журнала: 2024, Номер 48(37), С. 16331 - 16336

Опубликована: Янв. 1, 2024

Novel metal salt energetic material with good properties and high thermal stability.

Язык: Английский

Процитировано

1

Differences in Performance among ECPs with Different Metal Centers Based on Highly Stable TzTO DOI
Jinhao Zhang, Zhiyuan Jin,

Taichuan Li

и другие.

Crystal Growth & Design, Год журнала: 2024, Номер 24(22), С. 9337 - 9343

Опубликована: Авг. 29, 2024

The stability and detonation properties of energetic coordination polymers (ECPs) are usually directly related to the selection ligands. However, different metals ligands may form structures, which will greatly affect performance ECPs. Three-dimensional (3D) metal–organic frameworks (EMOFs) exhibit enhanced performances modest compared with one-dimensional (1D) two-dimensional (2D) In this work, an internal salt H2TzTO (5-(1H-1,2,4-triazol-4-ium-3-yl)-1H-tetrazol-1-olate) high was selected as ligand coordinated four metal centers, Na(I), K(I), Co(II), Ni(II), three ECPs, named [Na(HTzTO)(H2O)]n·0.5H2O, Co(HTzTO)2(H2O)2, Ni(HTzTO)2(H2O)2·2H2O, one EMOF [K(HTzTO)]n, respectively. compounds showed excellent thermal [decomposition temperature (Td) ≥ 263 °C] [detonation velocity (D) 8587 m·s–1 pressure (P) 33.8 GPa], but their due influence center structure. Among them, [K(HTzTO)]n Co(HTzTO)2(H2O)2 surprising (Td = 344 347 °C, respectively) formation face-to-face π–π stacking in enhances molecules.

Язык: Английский

Процитировано

0