Effect of the Functional Group Position in Coformers on Ternary Cocrystals: A Case of Sulfamoylbenzoic Acids DOI

Luguang Qi,

Shutian Xuanyuan,

Chang Li

и другие.

Crystal Growth & Design, Год журнала: 2024, Номер 24(18), С. 7455 - 7465

Опубликована: Сен. 3, 2024

Ternary cocrystals are an interesting and important topic of multicomponent crystals in crystal engineering. Although some cases ternary strategies have been reported, the number remains limited, related principles not yet well developed. Herein, 4-chloro-3-sulfamoylbenzoic acid 2,4-dichloro-5-sulfamolybenzoic were selected as model materials, pyridine carboxamides (picolinamide, nicotinamide, isonicotinamide) lactams (2-hydroxy-3-methylpyridine, 2-pyridone, 2-hydroxy-6-methylpyridine) used coformers for synthesizing cocrystals. With help powder X-ray diffraction, thermal analysis, nuclear magnetic resonance spectra, four new found, single structures three them successfully analyzed. The functional group position is found to two effects on On one hand, it affects tendency generate binary products. other there a certain match between types coformers. Further theoretical calculations show that geometrical recognition among components more formation than lattice energy.

Язык: Английский

A novel ADN/TANPDO supramolecular crystal with anti-hygroscopicity and high energy: A promising strategy to construct advanced propellant materials DOI
Shen Qiao, Zening Liu,

Shi Huang

и другие.

Chemical Engineering Journal, Год журнала: 2024, Номер unknown, С. 156152 - 156152

Опубликована: Сен. 1, 2024

Язык: Английский

Процитировано

4

High Energy Density with Low Mechanical Sensitivity: A Novel Energetic Cocrystal Composed of CL-20 and FOX-7 Obtained by Electrostatic Spray Method DOI

Guiyun Hang,

Jintao Wang, Tao Wang

и другие.

Journal of Molecular Structure, Год журнала: 2025, Номер unknown, С. 142138 - 142138

Опубликована: Март 1, 2025

Язык: Английский

Процитировано

0

Development of novel HNIW/N2 host-guest explosives with enhanced stability and performance via pressure-temperature strategy DOI
Xiaomin Song,

Donghan Jia,

Shanhu Sun

и другие.

Chemical Engineering Science, Год журнала: 2025, Номер unknown, С. 121742 - 121742

Опубликована: Апрель 1, 2025

Язык: Английский

Процитировано

0

Polymorphism of CL-20 and the Modification and Inhibition Strategies for Its Crystal Transformation DOI
Hui Wang,

Shifan Xu,

Hongtu Zhao

и другие.

Crystal Growth & Design, Год журнала: 2024, Номер unknown

Опубликована: Окт. 24, 2024

Язык: Английский

Процитировано

3

Pressure-Induced Structural and Electronic Transformations of Energetic Ionic Salt Hydroxylammonium 3,3'-Dinitro-Bis-(1,2,4-Triazole)-1,1'-Diolate DOI
Guozheng Zhao, Dongfang Yang

Опубликована: Янв. 1, 2024

This study explores the structural, molecular, and electronic responses of ionic salt hydroxylammonium 3,3'-dinitro-bis-(1,2,4-triazole)-1,1'-diolate (HDBTD) crystal to external pressure. Utilizing GGA in both PBE PW91 forms, alongside LDA as per CA-PZ, we compared computational results with experimental measurements determine most accurate method for analyzing HDBTD crystal. The reveals anisotropic nature under varying pressures up 200 GPa, detailed observations on behavior lattice constants, unit cell volume, molecular geometry including bond lengths, angles, dihedral angles. formation breaking covalent bonds pressure were highlighted, showing complex effects crystal's structure. Furthermore, impact structure was examined, a dynamic change band gaps density states (DOS) which indicate transitions from semiconductor metallic specific conditions.

Язык: Английский

Процитировано

0

Pressure-Induced Structural and Electronic Transformations of Energetic Ionic Salt Hydroxylammonium 3,3'-Dinitro-Bis-(1,2,4-Triazole)-1,1'-Diolate DOI
Guozheng Zhao, Dongfang Yang

Опубликована: Янв. 1, 2024

Язык: Английский

Процитировано

0

Theoretical investigations on N2H5N5/PDO cocrystal via a first‐principles study DOI
Zhipeng Chen, Junqi Wang,

Qingshan Xie

и другие.

Journal of Physical Organic Chemistry, Год журнала: 2024, Номер 37(11)

Опубликована: Авг. 11, 2024

Abstract The exploration of cyclo ‐N 5 ˉ‐based energetic cocrystals represents a noteworthy avenue within pentazolate chemistry, focusing on leveraging cocrystallization to enhance stability. Recently, novel cocrystal explosive, N 2 H /PDO, was developed by combining with pyrazine 1,4‐dioxide (PDO), exhibiting promising detonation characteristics and reduced sensitivity. This study endeavors elucidate how the structure noncovalent interactions impact performance /PDO through first‐principles investigation. results indicate that enhanced hydrogen bonding wave‐like crystal packing effectively bolster its stability compared . N···H O···H interactions, in conjunction π–π emerge as critical elements driving formation. Compared pure , exhibits slight decline, albeit noticeable reduction

Язык: Английский

Процитировано

0

Effect of the Functional Group Position in Coformers on Ternary Cocrystals: A Case of Sulfamoylbenzoic Acids DOI

Luguang Qi,

Shutian Xuanyuan,

Chang Li

и другие.

Crystal Growth & Design, Год журнала: 2024, Номер 24(18), С. 7455 - 7465

Опубликована: Сен. 3, 2024

Ternary cocrystals are an interesting and important topic of multicomponent crystals in crystal engineering. Although some cases ternary strategies have been reported, the number remains limited, related principles not yet well developed. Herein, 4-chloro-3-sulfamoylbenzoic acid 2,4-dichloro-5-sulfamolybenzoic were selected as model materials, pyridine carboxamides (picolinamide, nicotinamide, isonicotinamide) lactams (2-hydroxy-3-methylpyridine, 2-pyridone, 2-hydroxy-6-methylpyridine) used coformers for synthesizing cocrystals. With help powder X-ray diffraction, thermal analysis, nuclear magnetic resonance spectra, four new found, single structures three them successfully analyzed. The functional group position is found to two effects on On one hand, it affects tendency generate binary products. other there a certain match between types coformers. Further theoretical calculations show that geometrical recognition among components more formation than lattice energy.

Язык: Английский

Процитировано

0