Detection methodologies and mechanisms of reactive oxygen species generated in Fenton/Fenton-like processes

Separation and Purification Technology, Год журнала: 2024, Номер unknown, С. 129578 - 129578

Опубликована: Сен. 1, 2024

Язык: Английский

---

Pilot-scale and large-scale Fenton-like applications with nano-metal catalysts: from catalytic modules to scale-up applications

Water Research, Год журнала: 2024, Номер 266, С. 122425 - 122425

Опубликована: Сен. 10, 2024

Язык: Английский

---

Gambling of homogeneous and heterogeneous Fenton in wastewater treatment

Cell Reports Physical Science, Год журнала: 2024, Номер 5(5), С. 101966 - 101966

Опубликована: Май 1, 2024

Employing Fenton technology for efficiently removing pollutants in water stands as a significant method. Within the domain of traditional techniques, there exist both homogeneous and heterogeneous systems. Homogeneous systems tackle iron sludge concerns through incorporation co-catalysts, whereas adeptly manipulate surface microenvironments adjust active sites, enabling pollutant degradation across wide range pH. Each system boasts distinct advantages limitations. This perspective critically examines existing challenges associated solutions reactions comprehensive analysis typical case studies. The focus is on evaluating industrial potential these systems, forecasting future developmental trends, fostering more robust sustainable advancement within context carbon peaking neutrality goals.

Язык: Английский

---

Single-atom Co-N3 sites induce peroxymonosulfate activation for acetaminophen degradation via nearly 100% internal electron transfer process

Applied Catalysis B Environment and Energy, Год журнала: 2025, Номер unknown, С. 125038 - 125038

Опубликована: Янв. 1, 2025

Язык: Английский

---

Carbonaceous materials in structural dimensions for advanced oxidation processes

Chemical Society Reviews, Год журнала: 2025, Номер unknown

Опубликована: Янв. 1, 2025

Catalytic active sites and mechanisms of various dimensional carbonaceous materials in activation oxidants towards advanced oxidant processes for wastewater/water treatment were reviewed.

Язык: Английский

---

Self-dispersed Fe single-atom anchored biochar derived from hyperaccumulator residues with intrinsic Zn and Fe for selective peroxymonosulfate activation via electron transfer process

Chemical Engineering Journal, Год журнала: 2024, Номер 482, С. 149052 - 149052

Опубликована: Янв. 26, 2024

Язык: Английский

---

Electron transfer-mediated peroxymonosulfate activation through monoatomic Fe–pyridinic N4 moiety in biochar-based catalyst for electron-rich pollutants degradation in groundwater

Chemical Engineering Journal, Год журнала: 2024, Номер 492, С. 152158 - 152158

Опубликована: Май 11, 2024

Язык: Английский

---

Discovery of an End-to-End Pattern for Contaminant-Oriented Advanced Oxidation Processes Catalyzed by Biochar with Explainable Machine Learning

Environmental Science & Technology, Год журнала: 2024, Номер unknown

Опубликована: Авг. 20, 2024

The utilization of biochar-catalyzed peroxymonosulfate in advanced oxidation processes (BC-PMS AOPs) is widely acknowledged as an effective and economical method for mitigating emerging contaminants (ECs). Especially, state-of-the-art machine learning (ML) technology has been employed to accurately predict the reaction rate constants EC degradation BC-PMS AOPs, primarily focusing on three aspects: performance prediction, operating condition optimization, mechanism interpretation. However, its real application specific optimization targeting different ECs seldom considered, hindering realization contaminant-oriented AOPs. Herein, we propose a hierarchical ML pipeline achieve end-to-end (E2E) pattern addressing this issue. First, overall XGB model, trained with comprehensive data set, can perform well predicting additionally providing basis further analysis various ECs. Then, submodels clusters offer strategies selection optimum option AOPs HOMO-LUMO gaps, thus forming E2E This study not only increases our understanding but also successfully bridges gap between model development environmental application.

Язык: Английский

---

Selective oxidation of emerging organic contaminants in heterogeneous Fenton-like systems

Nano Research, Год журнала: 2024, Номер 17(11), С. 9300 - 9325

Опубликована: Авг. 5, 2024

Язык: Английский

---

Nanoconfined catalytic macrostructures for advanced water remediation: From basic understanding to future application strategies

Water Research, Год журнала: 2024, Номер 272, С. 122960 - 122960

Опубликована: Дек. 11, 2024

Язык: Английский

---