Highly Oriented Nitrogen-Doped Flower-like ZnO Nanostructures for Boosting Photocatalytic and Photoelectrochemical Performance: A Combined Experimental and DFT Study DOI Creative Commons
Riu Riu Wary, Abinash Das,

Emir S. Amirov

и другие.

The Journal of Physical Chemistry Letters, Год журнала: 2025, Номер unknown, С. 5180 - 5187

Опубликована: Май 15, 2025

A facile method to modify the ZnO catalyst by nitrogen doping and synthesis of a highly oriented flower-like structure is reported. The generated system exhibits an enhanced photoinduced charge separation through lightning rod effect. well-aligned high aspect ratio nanorods confirmed XRD, FESEM TEM analyses. Efficient photogenerated transfer achieved upon light irradiation, as PL EIS studies. Density functional theory (DFT) calculations provide atomistic understanding modified electronic N-doped ZnO. with 5 wt % best photocatalytic performance. When applied photoelectrochemical water splitting, optimal can achieve remarkable photocurrent density 4.0 mAcm-2 at lowest onset potential 0.61 V vs Ag/AgCl (1.40 RHE). reported work demonstrates that rational design doped materials opens up new avenues for development.

Язык: Английский

Highly Oriented Nitrogen-Doped Flower-like ZnO Nanostructures for Boosting Photocatalytic and Photoelectrochemical Performance: A Combined Experimental and DFT Study DOI Creative Commons
Riu Riu Wary, Abinash Das,

Emir S. Amirov

и другие.

The Journal of Physical Chemistry Letters, Год журнала: 2025, Номер unknown, С. 5180 - 5187

Опубликована: Май 15, 2025

A facile method to modify the ZnO catalyst by nitrogen doping and synthesis of a highly oriented flower-like structure is reported. The generated system exhibits an enhanced photoinduced charge separation through lightning rod effect. well-aligned high aspect ratio nanorods confirmed XRD, FESEM TEM analyses. Efficient photogenerated transfer achieved upon light irradiation, as PL EIS studies. Density functional theory (DFT) calculations provide atomistic understanding modified electronic N-doped ZnO. with 5 wt % best photocatalytic performance. When applied photoelectrochemical water splitting, optimal can achieve remarkable photocurrent density 4.0 mAcm-2 at lowest onset potential 0.61 V vs Ag/AgCl (1.40 RHE). reported work demonstrates that rational design doped materials opens up new avenues for development.

Язык: Английский

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