Highly Flexible Polyether for Solid Propellants: Synthesis, Room Temperature Curing, Thermal Analysis, and Mechanical Properties DOI

Q. H. Zhang,

Jinkang Dou, Minghui Xu

и другие.

ACS Applied Polymer Materials, Год журнала: 2024, Номер 6(17), С. 10565 - 10573

Опубликована: Авг. 26, 2024

The nitrile oxide-alkene curing system has attracted attention in the solid propellant field due to its byproduct-free, catalyst-free ligation and room temperature curing. For field, design synthesis of alkenyl-terminated adhesives are extremely important, where controllable distribution quantity alkene groups improve integrity cross-linked network cured elastomers. Compared with traditional for propellants such as poly(ethylene glycol) (PEG) polybutadiene (PB), poly(propylene (PPG) is both highly flexible polar presence ether linkages methyl groups. In this study, PPGs different number-average molecular weights were used raw materials further modified by esterification carbamate reactions successfully obtain two types polymers, 1-PPG 2-PPG. Based on click cycloaddition reaction, elastomers then obtained at temperature. Strikingly, interaction rigid structures, all exhibited excellent low-temperature mechanical properties (at −40 °C), particularly terms elongation break (up a maximum 1126%). This research introduced kinds providing options formulation promoting application system.

Язык: Английский

3D Printing for Explosive and Propellant Applications DOI Creative Commons
Bojun Tan, Jinkang Dou, Yujia Wen

и другие.

Deleted Journal, Год журнала: 2024, Номер 3(3), С. 200151 - 200151

Опубликована: Июль 1, 2024

3D printing technology is considered the perfect modern manufacturing for military/industrial enterprises worldwide. Applying in explosives and propellants fabrication enables precise performance control accurate structure formation, revolutionizing traditional concepts improving continuous, automated, integrated, flexible manufacturing. As key components of propellants, adhesives/binders play a crucial role determining formation rate, stability, structural integrity explosive formulations. This paper provides an overview four major technologies suitable manufacturing: vat photopolymerization, binder jetting, fused deposition modeling, direct ink writing, with their typical production processes, technical characteristics, principles, limitations discussed. Specific solutions to photopolymerization (printing speed), jetting (low accuracy limited applicable materials), modeling (poor mechanical properties dimensional stability), writing (product defects) are presented. Additionally, future development directions prospects discussed, thus providing valuable insights into application fields propellants.

Язык: Английский

Процитировано

4

Precision Preparation of π-Conjugated-Polymer-Based Nanofibers with Shell Tailorability by Combining Living Crystallization-Driven Self-Assembly with Nitrile N-Oxide-Based Cycloaddition DOI
Chen Wang, Fengfeng Huang, Xiaoyu Huang

и другие.

Macromolecules, Год журнала: 2025, Номер unknown

Опубликована: Апрель 15, 2025

Язык: Английский

Процитировано

0

Design, synthesis and curing mechanism of two novel photothermal dual-curing adhesives for propellants and explosives DOI Creative Commons
Bojun Tan,

Hongchang Mo,

Jing Zhang

и другие.

FirePhysChem, Год журнала: 2023, Номер 4(1), С. 63 - 71

Опубликована: Окт. 2, 2023

Photothermal dual-curing adhesive is not only required to realize the basic curing function, but also has characteristics of rapid setting and strong curing, which possesses a vital role in molding speed, stability structure integrity for 3D-printed propellants explosives. Herein, acrylate hydroxyl terminated polybutadiene, as novel photothermal binders, were designed synthesized utilizing cationic ring opening polymerization active monomer mechanism strategy reaction. The mechanical properties thermal elastomers systematically investigated. results suggested that target MAHTPB(Acrylate hydroxy-terminated polybutadiene)-based adhesives could be cured rapidly within 5 s under UV light irradiation completely 1.5 h heating conditions. Specifically, elastomer film formed by MAHTPB-based tensile strength 4.63 MPa an elongation 386%, exhibits stronger than single photo- or thermal-curing. As result, photothermally have performed 3D printing experiments achieved relatively satisfactory effects. Our study aims solve problems short photocuring time, slow rate incomplete traditional photocuring, lays solid foundation achieve prototyping precise performance control

Язык: Английский

Процитировано

3

Efficient metal-free crosslinking of common propellant binders using nitrile oxide–alkene click ligation DOI
Jinkang Dou,

Lijie Cheng,

Bojun Tan

и другие.

Polymer Chemistry, Год журнала: 2023, Номер 14(46), С. 5125 - 5132

Опубликована: Янв. 1, 2023

A promising tritopic nitrile oxide with high stability and reactivity was synthesized easily applied in efficient metal-free crosslinking of alkenyl-terminated binders as a click ligation reagent.

Язык: Английский

Процитировано

3

Highly Flexible Polyether for Solid Propellants: Synthesis, Room Temperature Curing, Thermal Analysis, and Mechanical Properties DOI

Q. H. Zhang,

Jinkang Dou, Minghui Xu

и другие.

ACS Applied Polymer Materials, Год журнала: 2024, Номер 6(17), С. 10565 - 10573

Опубликована: Авг. 26, 2024

The nitrile oxide-alkene curing system has attracted attention in the solid propellant field due to its byproduct-free, catalyst-free ligation and room temperature curing. For field, design synthesis of alkenyl-terminated adhesives are extremely important, where controllable distribution quantity alkene groups improve integrity cross-linked network cured elastomers. Compared with traditional for propellants such as poly(ethylene glycol) (PEG) polybutadiene (PB), poly(propylene (PPG) is both highly flexible polar presence ether linkages methyl groups. In this study, PPGs different number-average molecular weights were used raw materials further modified by esterification carbamate reactions successfully obtain two types polymers, 1-PPG 2-PPG. Based on click cycloaddition reaction, elastomers then obtained at temperature. Strikingly, interaction rigid structures, all exhibited excellent low-temperature mechanical properties (at −40 °C), particularly terms elongation break (up a maximum 1126%). This research introduced kinds providing options formulation promoting application system.

Язык: Английский

Процитировано

0