Organic Letters, Год журнала: 2025, Номер unknown
Опубликована: Апрель 11, 2025
DNA-encoded library (DEL) technology is a transformative tool for identifying bioactive compounds in pharmaceutical research. This study presents an optimized copper-mediated reaction to synthesize N-sulfonylamidine derivatives from DNA-conjugated alkynes and sulfonyl azides under mild conditions. Amines serve as nucleophiles, enabling selective functionalization conditions while preserving DNA integrity. Through systematic refinement of substrate evaluation, the approach demonstrated high tolerance diverse functional groups, significantly expanding DEL-accessible chemical space. The developed DNA-compatible method underscores role DELs enhancing drug discovery by facilitating introduction novel pharmacophores into compound libraries.
Язык: Английский