Supramolecular Assembly of Hydrogen-Bonded Organic Frameworks with Carbon Dots: Realizing Ultralong Aqueous Room-Temperature Phosphorescence for Anticounterfeiting DOI

Minjuan Cai,

Yijie Qiu,

Feiming Li

и другие.

ACS Applied Materials & Interfaces, Год журнала: 2024, Номер 16(35), С. 46609 - 46618

Опубликована: Авг. 22, 2024

Room-temperature phosphorescent carbon dots (RTP-CDs) have received increasing attention due to their excellent optical properties and potential applications. Nevertheless, the realization of RTP-CDs in aqueous solutions remains a considerable challenge water-molecule- oxygen-induced deactivation triplet excitons, which leads phosphorescence quenching. In this study, ultralong water was achieved by situ self-assembly CDs encapsulated rigid hydrogen-bonded organic framework (HOF). The lifetime reaches an impressive 956.96 ms exhibits long-lasting structural stability for more than 90 days. composite material not only has luminescence life but also two-color emission, as well antiphotobleaching solution, can solve current problem that RTP is easily burst out moisture. addition, study introduced fluorescent dye based on triplet–singlet Förster resonance energy transfer system (TS-FRET) fine-tune afterglow properties. This work will inspire design systems with dual phosphor light sources provide new strategies development smart materials water.

Язык: Английский

Investigating the influence of carbon dots on β-Ca2SiO4:Ce3+ phosphors derived from agro-waste for diverse applications DOI
B.R. Radha Krushna,

G.R. Mamatha,

S.C. Sharma

и другие.

Sustainable materials and technologies, Год журнала: 2024, Номер 41, С. e00993 - e00993

Опубликована: Май 31, 2024

Язык: Английский

Процитировано

3

Quantum Dot Luminescence Microspheres Enable Ultra‐Efficient and Bright Micro‐LEDs DOI Open Access
Ting Gong, Tongtong Xuan, Wenhao Bai

и другие.

Advanced Materials, Год журнала: 2025, Номер unknown

Опубликована: Янв. 21, 2025

Abstract Quantum dot (QD)‐converted micrometer‐scale light‐emitting diodes (micro‐LEDs) are regarded as an effective solution for achieving high‐performance full‐color micro‐LED displays because of their narrow‐band emission, simplified mass transfer, facile drive circuits, and low cost. However, these micro‐LEDs suffer from significant blue light leakage unsatisfactory electroluminescence properties due to the poor conversion efficiency stability QDs. Herein, construction green red QD luminescence microspheres with simultaneously high strong photoluminescence proposed. These exhibit external quantum yields exceeding 46% under 450 nm excitation, along excellent reliability against light, heat, water‐oxygen degradation, owing waveguide spatial confinement effects microspheres. The microsphere‐based achieve world‐record efficiencies 40.8% 22.1%, respectively, brightness values 1.7 × 10 8 7.6 7 cd m −2 , respectively. Finally, 0.6 inch red, green, monochrome demonstrated by integrating microsphere‐converted arrays thin‐film transistor backplanes, which show a pixel resolution 1700 PPI 000 .

Язык: Английский

Процитировано

0

PbTe quantum dots highly packed monolayer fabrication by a spin coating method DOI Creative Commons
Svetlana Lyssenko,

Michal Amar,

Alina Sermiagin

и другие.

PLoS ONE, Год журнала: 2025, Номер 20(2), С. e0317677 - e0317677

Опубликована: Фев. 11, 2025

This study investigates the fabrication of large-area, highly-ordered monolayers PbTe quantum dots (QDs) on TiO 2 /ITO substrate, using a fast, simple, and repeatable spin-coating technique. For first time, real monolayer (a layer with height single QD) covering approximately 3 cm was successfully prepared, achieving root-mean-square roughness (Rq) 1.37 nm. The research systematically explores key parameters such as QD morphology, concentration, conditions, substrate characteristics, wetting properties, solvent effects to optimize thin film deposition. findings reveal that method favors formation layers spherical QDs (6–9 nm) over cubical (10–13 nm). highlight significant influence evaporation rate, viscosity, wettability quality. Chloroform identified optimal for (~90% coverage), while hexane more effective (90%-100% coverage). Beyond monolayers, high-quality bilayers were also fabricated, demonstrating method’s potential multilayer fabrication. rapid efficient bilayer marks breakthrough in producing uniform, large-area films, facilitating seamless integration existing technologies. It offers scalable cost-effective solution, opening door broader applications fields demand

Язык: Английский

Процитировано

0

Supramolecular Assembly of Hydrogen-Bonded Organic Frameworks with Carbon Dots: Realizing Ultralong Aqueous Room-Temperature Phosphorescence for Anticounterfeiting DOI

Minjuan Cai,

Yijie Qiu,

Feiming Li

и другие.

ACS Applied Materials & Interfaces, Год журнала: 2024, Номер 16(35), С. 46609 - 46618

Опубликована: Авг. 22, 2024

Room-temperature phosphorescent carbon dots (RTP-CDs) have received increasing attention due to their excellent optical properties and potential applications. Nevertheless, the realization of RTP-CDs in aqueous solutions remains a considerable challenge water-molecule- oxygen-induced deactivation triplet excitons, which leads phosphorescence quenching. In this study, ultralong water was achieved by situ self-assembly CDs encapsulated rigid hydrogen-bonded organic framework (HOF). The lifetime reaches an impressive 956.96 ms exhibits long-lasting structural stability for more than 90 days. composite material not only has luminescence life but also two-color emission, as well antiphotobleaching solution, can solve current problem that RTP is easily burst out moisture. addition, study introduced fluorescent dye based on triplet–singlet Förster resonance energy transfer system (TS-FRET) fine-tune afterglow properties. This work will inspire design systems with dual phosphor light sources provide new strategies development smart materials water.

Язык: Английский

Процитировано

2