ACS Applied Materials & Interfaces, Год журнала: 2025, Номер unknown
Опубликована: Май 12, 2025
PtSe2 is notable for its high carrier mobility and exceptional air stability. Its unique thickness-dependent transition from a semiconductor to semimetal renders it particularly promising short-wave infrared (SWIR) detection applications. In this study, single-crystal film with an area approaching 4 in. was fabricated at low temperature under the concurrent modulation of nonuniform gas thermal field in large-diameter tube. Subsequently, p-PtSe2/n--Si/n+-Si 2D-3D PIN photodetectors were constructed. The effect intrinsic layer thickness (0.5 versus 5 μm) on device performance systematically examined. Thinner devices not only deliver wide SWIR range 532 2200 nm but also exhibit metrics, rectification ratio (∼106) ideality factor 1.288, indicating near-ideal performance. contrast, thinner have detectivity as 1.49 × 1011 Jones (approximately double higher), rise fall times 24/71 μs 3-fold faster), 3 dB cutoff frequency 32 kHz (nearly 5-fold higher). addition, display excellent imaging polarization range, dichroic reaching 36.5. This work provides significant insights advancement Si-based integrated detectors.
Язык: Английский