ACS Nano,
Год журнала:
2021,
Номер
15(9), С. 14653 - 14661
Опубликована: Сен. 15, 2021
Owing
to
wearing
and
unpredictable
damage,
the
working
lifetime
of
triboelectric
nanogenerators
(TENGs)
is
largely
limited.
In
this
work,
we
prepared
a
single-electrode
multifunctional
TENG
(MF-TENG)
that
exhibits
fast
self-healing,
human
health
monitoring
capability,
photothermal
properties.
The
device
consists
thin
self-healing
poly(vinyl
alcohol)-based
hydrogel
sandwiched
between
two
silicone
elastomer
films.
MF-TENG
short-circuit
current,
transfer
charge,
open-circuit
voltage
7.98
μA,
78.34
nC,
38.57
V,
respectively.
Furthermore,
owing
repairable
networks
dynamic
imine
bonds
in
charged
layer
borate
ester
electrodes,
could
recover
its
original
state
after
mechanical
damage
within
10
min
at
room
temperature.
can
be
attached
different
joints
for
self-powered
personal
information.
Additionally,
under
near-infrared
laser
irradiation
provide
therapy
assisting
recovery
motion.
It
envisaged
proposed
applied
fields
wearable
electronics
health-monitoring
devices.
Abstract
Wearable
electronics
offer
incredible
benefits
in
mobile
healthcare
monitoring,
sensing,
portable
energy
harvesting
and
storage,
human‐machine
interactions,
etc.,
due
to
the
evolution
of
rigid
structure
flexible
stretchable
devices.
Lately,
transition
metal
carbides
nitrides
(MXenes)
are
highly
regarded
as
a
group
thriving
two‐dimensional
nanomaterials
extraordinary
building
blocks
for
emerging
platforms
because
their
excellent
electrical
conductivity,
enriched
surface
functionalities,
large
area.
This
article
reviews
most
recent
developments
MXene‐enabled
wearable
electronics.
Several
electronic
devices
designed
on
nanometric
scale
highlighted
by
drawing
attention
widely
developed
nonstructural
attributes,
including
3D
configured
devices,
textile
planer
substrates,
bioinspired
structures,
printed
materials.
Furthermore,
unique
progress
these
nanodevices
is
representative
applications
healthcare,
energy,
electromagnetic
interference
(EMI)
shielding,
humanoid
control
machines.
The
prospects
MXene
key
frontier
next‐generation
envisioned
design
challenges
systems
also
discussed,
followed
proposed
solutions.
image
Nano-Micro Letters,
Год журнала:
2022,
Номер
14(1)
Опубликована: Июль 5, 2022
As
an
indispensable
branch
of
wearable
electronics,
flexible
pressure
sensors
are
gaining
tremendous
attention
due
to
their
extensive
applications
in
health
monitoring,
human
–machine
interaction,
artificial
intelligence,
the
internet
things,
and
other
fields.
In
recent
years,
highly
have
been
developed
using
various
materials/structures
transduction
mechanisms.
Morphological
engineering
sensing
materials
at
nanometer
micrometer
scales
is
crucial
obtaining
superior
sensor
performance.
This
review
focuses
on
rapid
development
morphological
technologies
for
sensors.
We
discuss
different
architectures
designs
achieve
high
performance,
including
sensitivity,
broad
working
range,
stable
sensing,
low
hysteresis,
transparency,
directional
or
selective
sensing.
Additionally,
general
fabrication
techniques
summarized,
self-assembly,
patterning,
auxiliary
synthesis
methods.
Furthermore,
we
present
emerging
high-performing
microengineered
healthcare,
smart
homes,
digital
sports,
security
machine
learning-enabled
computational
platform.
Finally,
potential
challenges
prospects
future
developments
discussed
comprehensively.
Abstract
Due
to
their
potential
applications
in
physiological
monitoring,
diagnosis,
human
prosthetics,
haptic
perception,
and
human–machine
interaction,
flexible
tactile
sensors
have
attracted
wide
research
interest
recent
years.
Thanks
the
advances
material
engineering,
high
performance
been
obtained.
Among
representative
pressure
sensing
materials,
2D
layered
nanomaterials
many
properties
that
are
superior
those
of
bulk
more
suitable
for
sensors.
As
a
class
inorganic
compounds
materials
science,
MXene
has
excellent
electrical,
mechanical,
biological
compatibility.
MXene‐based
composites
proven
be
promising
candidates
due
stretchability
metallic
conductivity.
Therefore,
great
efforts
devoted
development
sensor
applications.
In
this
paper,
controllable
preparation
characterization
introduced.
Then,
progresses
on
fabrication
strategies,
operating
mechanisms,
device
composite‐based
sensors,
including
piezoresistive
capacitive
piezoelectric
triboelectric
reviewed.
After
that,
material‐based
electronics
motion
healthcare,
artificial
intelligence
discussed.
Finally,
challenges
perspectives
summarized.
Nano-Micro Letters,
Год журнала:
2022,
Номер
14(1)
Опубликована: Апрель 24, 2022
Although
electrically
conductive
and
hydrophilic
MXene
sheets
are
promising
for
multifunctional
fibers
electronic
textiles,
it
is
still
a
challenge
to
simultaneously
enhance
both
conductivity
mechanical
properties
of
because
the
high
rigidity
insufficient
inter-sheet
interactions.
Herein,
we
demonstrate
core-shell
wet-spinning
methodology
fabricating
highly
conductive,
super-tough,
ultra-strong,
environmentally
stable
Ti3C2Tx
MXene-based
with
cores
tough
aramid
nanofiber
(ANF)
shells.
The
orientated
low-defect
structure
endows
ANF@MXene
fiber
super-toughness
~
48.1
MJ
m-3,
strength
502.9
MPa,
3.0
×
105
S
m-1.
super-tough
can
be
woven
into
exhibiting
an
excellent
electromagnetic
interference
(EMI)
shielding
efficiency
83.4
dB
at
small
thickness
213
μm.
Importantly,
protection
ANF
shells
provides
satisfactory
cyclic
stability
under
dynamic
stretching
bending,
resistance
acid,
alkali,
seawater,
cryogenic
temperatures,
fire.
oxidation
demonstrated
by
their
well-maintained
EMI
performances.
would
in
fields
wearable
electronics
aerospace.
Abstract
MXene
emerged
as
decent
2D
material
and
has
been
exploited
for
numerous
applications
in
the
last
decade.
The
remunerations
of
ideal
metallic
conductivity,
optical
absorbance,
mechanical
stability,
higher
heterogeneous
electron
transfer
rate,
good
redox
capability
have
made
a
potential
candidate
biosensing
applications.
hydrophilic
nature,
biocompatibility,
antifouling,
anti‐toxicity
properties
opened
avenues
to
perform
vitro
vivo
analysis.
In
this
review,
concept,
operating
principle,
detailed
mechanism,
characteristic
are
comprehensively
assessed
compiled
along
with
breakthroughs
fabrication
conjugation
strategies
development
unique
electrochemical
biosensors.
Further,
current
challenges
summarized
suggested
future
aspects.
This
review
article
is
believed
shed
some
light
on
will
open
new
opportunities
advanced
translational
application
bioassays.
Nature Communications,
Год журнала:
2022,
Номер
13(1)
Опубликована: Авг. 5, 2022
Recent
advances
in
MXene
(Ti3C2Tx)
fibers,
prepared
from
electrically
conductive
and
mechanically
strong
nanosheets,
address
the
increasing
demand
of
emerging
yet
promising
electrode
materials
for
development
textile-based
devices
beyond.
However,
to
reveal
full
potential
reaching
a
balance
between
electrical
conductivity
mechanical
property
is
still
fundamental
challenge,
mainly
due
difficulties
further
compact
loose
nanosheets.
In
this
work,
we
demonstrate
continuous
controllable
route
fabricate
ultra-compact
fibers
with
an
in-situ
generated
protective
layer
via
synergy
interfacial
interactions
thermal
drawing-induced
stresses.
The
resulting
high
orientation
low
porosity
exhibit
not
only
excellent
tensile
strength
ultra-high
toughness,
but
also
conductivity.
Then,
construct
meter-scale
textiles
using
these
achieve
high-performance
electromagnetic
interference
shielding
personal
management,
accompanied
by
durability
stability
even
after
multiple
washing
cycles.
demonstrated
generic
strategy
can
be
applied
broad
range
nanostructured
functional
large-scale
applications
both
space
daily
lives.
ACS Nano,
Год журнала:
2022,
Номер
16(5), С. 8161 - 8171
Опубликована: Апрель 28, 2022
Nanocomposite
conductive
fiber
has
been
newly
developed
as
a
lightweight
material
with
high
flexibility
and
strong
weavability,
which
can
meet
the
requirements
of
flexible
wearable
devices.
Herein,
porous
aramid
nanofibers
(ANF)
carbon
nanotube
(CNT)
aerogel
fibers
coated
polypyrrole
(PPy)
layers
are
prepared
by
wet
spinning
method
for
motion
detection
information
transmission.
The
ANF/CNT/PPy
low
density
(56.3
mg/cm3),
conductivity
(6.43
S/m),
tensile
strength
(2.88
MPa)
were
used
sensors
sensitivity
(0.12)
long
life
(1000
cycles).
At
same
time,
differential
is
utilized
to
reduce
transmission
time
(up
46%).
High-
low-temperature-resistant
(-196
100
°C)
also
available
quick
heater
ionic
solution
detector.
In
summary,
be
multifunctional
sensor
human-health
monitoring.