Cohesive energy discrepancy drives the fabrication of multimetallic atomically dispersed materials for hydrogen evolution reaction DOI Creative Commons
Xinyi Yang,

Wanqing Song,

Kang Liao

и другие.

Nature Communications, Год журнала: 2024, Номер 15(1)

Опубликована: Сен. 19, 2024

Язык: Английский

Electrocatalytic upcycling of plastic waste: Progress, challenges, and future DOI Creative Commons
Jinzhou Li, J.T. Chen, Luyao Zhang

и другие.

Electron, Год журнала: 2024, Номер 2(3)

Опубликована: Авг. 1, 2024

Abstract The escalating accumulation of plastic waste has been developed into a formidable global environmental challenge. Traditional disposal methods such as landfilling and incineration not only exacerbate degradation by releasing harmful chemicals greenhouse gases, but also squander finite resources that could otherwise be recycled or repurposed. Upcycling is kind recycling technology converts high‐value helps to avoid resource pollution. Electrocatalytic upcycling emerges novel distinguished its mild operational conditions, high transformation efficiency product selectivity. This review commences with an overview the employed in management respective advantages inherent limitations are delineated. different types upcycled electrocatalytic strategy then discussed process examined together mechanisms underlying upcycling. Furthermore, structure‐activity relationships between electrocatalysts performance elucidated. aims furnish readers comprehensive understanding techniques for provide guidance design towards efficient transformation.

Язык: Английский

Процитировано

14

Microenvironment Engineering of Heterogeneous Catalysts for Liquid-Phase Environmental Catalysis DOI

Zhong‐Shuai Zhu,

Shuang Zhong, Cheng Cheng

и другие.

Chemical Reviews, Год журнала: 2024, Номер 124(20), С. 11348 - 11434

Опубликована: Окт. 9, 2024

Environmental catalysis has emerged as a scientific frontier in mitigating water pollution and advancing circular chemistry reaction microenvironment significantly influences the catalytic performance efficiency. This review delves into engineering within liquid-phase environmental catalysis, categorizing microenvironments four scales: atom/molecule-level modulation, nano/microscale-confined structures, interface surface regulation, external field effects. Each category is analyzed for its unique characteristics merits, emphasizing potential to enhance efficiency selectivity. Following this overview, we introduced recent advancements advanced material system design promote (e.g., purification, transformation value-added products, green synthesis), leveraging state-of-the-art technologies. These discussions showcase was applied different reactions fine-tune regimes improve from both thermodynamics kinetics perspectives. Lastly, discussed challenges future directions engineering. underscores of intelligent materials drive development more effective sustainable solutions decontamination.

Язык: Английский

Процитировано

14

Electrocatalytic reduction of CO2 with enhanced C2 liquid products activity by the synergistic effect of Cu single atoms and oxygen vacancies DOI

Quanquan Bie,

Haibo Yin, Yunlong Wang

и другие.

CHINESE JOURNAL OF CATALYSIS (CHINESE VERSION), Год журнала: 2024, Номер 57, С. 96 - 104

Опубликована: Фев. 1, 2024

Язык: Английский

Процитировано

13

Perspectives on sustainable plastic treatment: A shift from linear to circular economy DOI Creative Commons
Xingdong Shi, Zhijie Chen, Wei Wei

и другие.

TrAC Trends in Analytical Chemistry, Год журнала: 2024, Номер 173, С. 117631 - 117631

Опубликована: Март 5, 2024

The pervasive presence of plastics in the environment, particularly microplastics, has become a significant global challenge, demanding innovative solutions for their management and upcycling. While traditional methods including landfill incineration face limitations environmental impact, emerging technologies offer promising pathways conversion into valuable chemicals fuels, operating under ambient conditions often utilizing sustainable energy sources. Considering current research progress plastic upgrading, it is necessary to summarize chemical upcycling waste. To this end, review provides an overall examination methodologies treatment, pyrolysis, hydrogenolysis, photocatalysis, electrocatalysis. Existing knowledge gaps future directions are then proposed. Overall, highlights potential these novel approaches aligning with principles circular economy.

Язык: Английский

Процитировано

13

Cohesive energy discrepancy drives the fabrication of multimetallic atomically dispersed materials for hydrogen evolution reaction DOI Creative Commons
Xinyi Yang,

Wanqing Song,

Kang Liao

и другие.

Nature Communications, Год журнала: 2024, Номер 15(1)

Опубликована: Сен. 19, 2024

Язык: Английский

Процитировано

13